Femtosecond all-optical synchronization of an X-ray free-electron laser

Many advanced applications of X-ray free-electron lasers require pulse durations and time resolutions of only a few femtoseconds. To generate these pulses and to apply them in time-resolved experiments, synchronization techniques that can simultaneously lock all independent components, including all...

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Main Authors: Schulz, S., Grguraš, I., Behrens, C., Bromberger, H., Costello, J. T., Czwalinna, M. K., Felber, M., Hoffmann, M. C., Ilchen, M., Liu, H. Y., Mazza, T., Meyer, M., Pfeiffer, S., Prędki, P., Schefer, S., Schmidt, C., Wegner, U., Schlarb, H., Cavalieri, A. L.
Format: Online
Language:English
Published: Nature Pub. Group 2015
Online Access:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC4309427/
id pubmed-4309427
recordtype oai_dc
spelling pubmed-43094272015-02-09 Femtosecond all-optical synchronization of an X-ray free-electron laser Schulz, S. Grguraš, I. Behrens, C. Bromberger, H. Costello, J. T. Czwalinna, M. K. Felber, M. Hoffmann, M. C. Ilchen, M. Liu, H. Y. Mazza, T. Meyer, M. Pfeiffer, S. Prędki, P. Schefer, S. Schmidt, C. Wegner, U. Schlarb, H. Cavalieri, A. L. Article Many advanced applications of X-ray free-electron lasers require pulse durations and time resolutions of only a few femtoseconds. To generate these pulses and to apply them in time-resolved experiments, synchronization techniques that can simultaneously lock all independent components, including all accelerator modules and all external optical lasers, to better than the delivered free-electron laser pulse duration, are needed. Here we achieve all-optical synchronization at the soft X-ray free-electron laser FLASH and demonstrate facility-wide timing to better than 30 fs r.m.s. for 90 fs X-ray photon pulses. Crucially, our analysis indicates that the performance of this optical synchronization is limited primarily by the free-electron laser pulse duration, and should naturally scale to the sub-10 femtosecond level with shorter X-ray pulses. Nature Pub. Group 2015-01-20 /pmc/articles/PMC4309427/ /pubmed/25600823 http://dx.doi.org/10.1038/ncomms6938 Text en Copyright © 2015, Nature Publishing Group, a division of Macmillan Publishers Limited. All Rights Reserved. http://creativecommons.org/licenses/by/4.0/ This work is licensed under a Creative Commons Attribution 4.0 International License. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in the credit line; if the material is not included under the Creative Commons license, users will need to obtain permission from the license holder to reproduce the material. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/
repository_type Open Access Journal
institution_category Foreign Institution
institution US National Center for Biotechnology Information
building NCBI PubMed
collection Online Access
language English
format Online
author Schulz, S.
Grguraš, I.
Behrens, C.
Bromberger, H.
Costello, J. T.
Czwalinna, M. K.
Felber, M.
Hoffmann, M. C.
Ilchen, M.
Liu, H. Y.
Mazza, T.
Meyer, M.
Pfeiffer, S.
Prędki, P.
Schefer, S.
Schmidt, C.
Wegner, U.
Schlarb, H.
Cavalieri, A. L.
spellingShingle Schulz, S.
Grguraš, I.
Behrens, C.
Bromberger, H.
Costello, J. T.
Czwalinna, M. K.
Felber, M.
Hoffmann, M. C.
Ilchen, M.
Liu, H. Y.
Mazza, T.
Meyer, M.
Pfeiffer, S.
Prędki, P.
Schefer, S.
Schmidt, C.
Wegner, U.
Schlarb, H.
Cavalieri, A. L.
Femtosecond all-optical synchronization of an X-ray free-electron laser
author_facet Schulz, S.
Grguraš, I.
Behrens, C.
Bromberger, H.
Costello, J. T.
Czwalinna, M. K.
Felber, M.
Hoffmann, M. C.
Ilchen, M.
Liu, H. Y.
Mazza, T.
Meyer, M.
Pfeiffer, S.
Prędki, P.
Schefer, S.
Schmidt, C.
Wegner, U.
Schlarb, H.
Cavalieri, A. L.
author_sort Schulz, S.
title Femtosecond all-optical synchronization of an X-ray free-electron laser
title_short Femtosecond all-optical synchronization of an X-ray free-electron laser
title_full Femtosecond all-optical synchronization of an X-ray free-electron laser
title_fullStr Femtosecond all-optical synchronization of an X-ray free-electron laser
title_full_unstemmed Femtosecond all-optical synchronization of an X-ray free-electron laser
title_sort femtosecond all-optical synchronization of an x-ray free-electron laser
description Many advanced applications of X-ray free-electron lasers require pulse durations and time resolutions of only a few femtoseconds. To generate these pulses and to apply them in time-resolved experiments, synchronization techniques that can simultaneously lock all independent components, including all accelerator modules and all external optical lasers, to better than the delivered free-electron laser pulse duration, are needed. Here we achieve all-optical synchronization at the soft X-ray free-electron laser FLASH and demonstrate facility-wide timing to better than 30 fs r.m.s. for 90 fs X-ray photon pulses. Crucially, our analysis indicates that the performance of this optical synchronization is limited primarily by the free-electron laser pulse duration, and should naturally scale to the sub-10 femtosecond level with shorter X-ray pulses.
publisher Nature Pub. Group
publishDate 2015
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC4309427/
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