Synthesis of CdS sensitized TiO2 photocatalysts: methylene blue adsorption and enhanced photocatalytic activities

A series of CdS/ nanocomposites with different Cd to Ti molar ratio were synthesized from P25- nanopowder using microwave-assisted hydrothermal method. The as-produced powders were characterized by XRD, electron microscopy, EDX, and UV-Vis diffuse reflectance spectroscopy. The adsorption capacity an...

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Main Authors: Makama, Abdullahi B., Ali, Salmiaton, Saion, Elias, Choong, Thomas Shean Yaw, Abdullah, Norhafizah
Format: Article
Language:English
Published: Hindawi Publishing Corporation 2016
Subjects:
Online Access:http://psasir.upm.edu.my/id/eprint/53964/
http://psasir.upm.edu.my/id/eprint/53964/1/Synthesis%20of%20CdS%20sensitized%20TiO2%20photocatalysts.pdf
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author Makama, Abdullahi B.
Ali, Salmiaton
Saion, Elias
Choong, Thomas Shean Yaw
Abdullah, Norhafizah
author_facet Makama, Abdullahi B.
Ali, Salmiaton
Saion, Elias
Choong, Thomas Shean Yaw
Abdullah, Norhafizah
author_sort Makama, Abdullahi B.
building UPM Institutional Repository
collection Online Access
description A series of CdS/ nanocomposites with different Cd to Ti molar ratio were synthesized from P25- nanopowder using microwave-assisted hydrothermal method. The as-produced powders were characterized by XRD, electron microscopy, EDX, and UV-Vis diffuse reflectance spectroscopy. The adsorption capacity and photocatalytic activity of the samples were investigated using methylene blue as a model pollutant. Sorption tests revealed that the adsorption of MB onto the samples obeys the Freundlich-Langmuir isotherm model. The sorption capacity decreased as follows: . The results of the photocatalytic tests under high-intensity discharge (HID) lamp revealed that CdS/ powders with low Cd to Ti molar ratios exhibited much higher activities than P25-. The CdS/ sample with 20% CdS/(TCd2) showed the most activity among all these samples. The results also show that the Cd to Ti molar ratio of the nanocomposite has a significant effect on the photodegradation of MB and the enhanced activities exhibited by the nanocomposites are because of the low rate of electron-hole recombination.
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spelling upm-539642018-02-22T08:19:03Z http://psasir.upm.edu.my/id/eprint/53964/ Synthesis of CdS sensitized TiO2 photocatalysts: methylene blue adsorption and enhanced photocatalytic activities Makama, Abdullahi B. Ali, Salmiaton Saion, Elias Choong, Thomas Shean Yaw Abdullah, Norhafizah A series of CdS/ nanocomposites with different Cd to Ti molar ratio were synthesized from P25- nanopowder using microwave-assisted hydrothermal method. The as-produced powders were characterized by XRD, electron microscopy, EDX, and UV-Vis diffuse reflectance spectroscopy. The adsorption capacity and photocatalytic activity of the samples were investigated using methylene blue as a model pollutant. Sorption tests revealed that the adsorption of MB onto the samples obeys the Freundlich-Langmuir isotherm model. The sorption capacity decreased as follows: . The results of the photocatalytic tests under high-intensity discharge (HID) lamp revealed that CdS/ powders with low Cd to Ti molar ratios exhibited much higher activities than P25-. The CdS/ sample with 20% CdS/(TCd2) showed the most activity among all these samples. The results also show that the Cd to Ti molar ratio of the nanocomposite has a significant effect on the photodegradation of MB and the enhanced activities exhibited by the nanocomposites are because of the low rate of electron-hole recombination. Hindawi Publishing Corporation 2016 Article PeerReviewed text en http://psasir.upm.edu.my/id/eprint/53964/1/Synthesis%20of%20CdS%20sensitized%20TiO2%20photocatalysts.pdf Makama, Abdullahi B. and Ali, Salmiaton and Saion, Elias and Choong, Thomas Shean Yaw and Abdullah, Norhafizah (2016) Synthesis of CdS sensitized TiO2 photocatalysts: methylene blue adsorption and enhanced photocatalytic activities. International Journal of Photoenergy, 2016. art. no. 2947510. pp. 1-14. ISSN 1110-662X; ESSN: 1687-529X https://www.hindawi.com/journals/ijp/2016/2947510/abs/ CdS/TiO2; Photocatalysts; Methylene blue adsorption; Photocatalytic activities 10.1155/2016/2947510
spellingShingle CdS/TiO2; Photocatalysts; Methylene blue adsorption; Photocatalytic activities
Makama, Abdullahi B.
Ali, Salmiaton
Saion, Elias
Choong, Thomas Shean Yaw
Abdullah, Norhafizah
Synthesis of CdS sensitized TiO2 photocatalysts: methylene blue adsorption and enhanced photocatalytic activities
title Synthesis of CdS sensitized TiO2 photocatalysts: methylene blue adsorption and enhanced photocatalytic activities
title_full Synthesis of CdS sensitized TiO2 photocatalysts: methylene blue adsorption and enhanced photocatalytic activities
title_fullStr Synthesis of CdS sensitized TiO2 photocatalysts: methylene blue adsorption and enhanced photocatalytic activities
title_full_unstemmed Synthesis of CdS sensitized TiO2 photocatalysts: methylene blue adsorption and enhanced photocatalytic activities
title_short Synthesis of CdS sensitized TiO2 photocatalysts: methylene blue adsorption and enhanced photocatalytic activities
title_sort synthesis of cds sensitized tio2 photocatalysts: methylene blue adsorption and enhanced photocatalytic activities
topic CdS/TiO2; Photocatalysts; Methylene blue adsorption; Photocatalytic activities
url http://psasir.upm.edu.my/id/eprint/53964/
http://psasir.upm.edu.my/id/eprint/53964/
http://psasir.upm.edu.my/id/eprint/53964/
http://psasir.upm.edu.my/id/eprint/53964/1/Synthesis%20of%20CdS%20sensitized%20TiO2%20photocatalysts.pdf