Synthesis of waste cooking oil based biodiesel via ferric-manganese promoted molybdenum oxide / zirconia nanoparticle solid acid catalyst: influence of ferric and manganese dopants

The utilization of ferric-manganese promoted molybdenum oxide/zirconia (Fe-Mn- MoO3/ZrO2) (FMMZ) solid acid catalyst for production of biodiesel was demonstrated. FMMZ is produced through impregnation reaction followed by calcination at 600°C for 3 h. The characterization of FMMZ had been done using...

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Main Authors: Alhassan, Fatah H., Rashid, Umer, Yap, Taufiq Yun Hin
Format: Article
Language:English
Published: Japan Oil Chemists' Society 2015
Online Access:http://psasir.upm.edu.my/id/eprint/46475/
http://psasir.upm.edu.my/id/eprint/46475/1/Synthesis%20of%20waste%20cooking%20oil%20based%20biodiesel%20via%20ferric-manganese%20promoted%20molybdenum%20oxide%20%20zirconia%20nanoparticle%20solid%20acid%20catalyst%20influence%20of%20ferric%20and%20manganese%20dopants.pdf
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author Alhassan, Fatah H.
Rashid, Umer
Yap, Taufiq Yun Hin
author_facet Alhassan, Fatah H.
Rashid, Umer
Yap, Taufiq Yun Hin
author_sort Alhassan, Fatah H.
building UPM Institutional Repository
collection Online Access
description The utilization of ferric-manganese promoted molybdenum oxide/zirconia (Fe-Mn- MoO3/ZrO2) (FMMZ) solid acid catalyst for production of biodiesel was demonstrated. FMMZ is produced through impregnation reaction followed by calcination at 600°C for 3 h. The characterization of FMMZ had been done using X-ray diffraction (XRD), X-ray photoelectron spectroscopy (XPS), thermal gravimetric analysis (TGA), temperature programmed desorption of NH3 (TPD-NH3), transmission electron microscopy(TEM) and Brunner-Emmett-Teller (BET) surface area measurement. The effect of waste cooking oil methyl esters (WCOME's) yield on the reactions variables such as reaction temperature, catalyst loading, molar ratio of methanol/oil and reusability were also assessed. The catalyst was used to convert the waste cooking oil into corresponding methyl esters (95.6%±0.15) within 5 h at 200℃ reaction temperature, 600 rpm stirring speed, 1:25 molar ratio of oil to alcohol and 4% w/w catalyst loading. The reported catalyst was successfully recycled in six connective experiments without loss in activity. Moreover, the fuel properties of WCOME's were also reported using ASTM D 6751 methods.
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spelling upm-464752018-02-27T04:17:57Z http://psasir.upm.edu.my/id/eprint/46475/ Synthesis of waste cooking oil based biodiesel via ferric-manganese promoted molybdenum oxide / zirconia nanoparticle solid acid catalyst: influence of ferric and manganese dopants Alhassan, Fatah H. Rashid, Umer Yap, Taufiq Yun Hin The utilization of ferric-manganese promoted molybdenum oxide/zirconia (Fe-Mn- MoO3/ZrO2) (FMMZ) solid acid catalyst for production of biodiesel was demonstrated. FMMZ is produced through impregnation reaction followed by calcination at 600°C for 3 h. The characterization of FMMZ had been done using X-ray diffraction (XRD), X-ray photoelectron spectroscopy (XPS), thermal gravimetric analysis (TGA), temperature programmed desorption of NH3 (TPD-NH3), transmission electron microscopy(TEM) and Brunner-Emmett-Teller (BET) surface area measurement. The effect of waste cooking oil methyl esters (WCOME's) yield on the reactions variables such as reaction temperature, catalyst loading, molar ratio of methanol/oil and reusability were also assessed. The catalyst was used to convert the waste cooking oil into corresponding methyl esters (95.6%±0.15) within 5 h at 200℃ reaction temperature, 600 rpm stirring speed, 1:25 molar ratio of oil to alcohol and 4% w/w catalyst loading. The reported catalyst was successfully recycled in six connective experiments without loss in activity. Moreover, the fuel properties of WCOME's were also reported using ASTM D 6751 methods. Japan Oil Chemists' Society 2015 Article PeerReviewed text en http://psasir.upm.edu.my/id/eprint/46475/1/Synthesis%20of%20waste%20cooking%20oil%20based%20biodiesel%20via%20ferric-manganese%20promoted%20molybdenum%20oxide%20%20zirconia%20nanoparticle%20solid%20acid%20catalyst%20influence%20of%20ferric%20and%20manganese%20dopants.pdf Alhassan, Fatah H. and Rashid, Umer and Yap, Taufiq Yun Hin (2015) Synthesis of waste cooking oil based biodiesel via ferric-manganese promoted molybdenum oxide / zirconia nanoparticle solid acid catalyst: influence of ferric and manganese dopants. Journal of Oleo Science, 64 (5). pp. 505-514. ISSN 1345-8957; ESSN: 1347-3352 http://www.jstage.jst.go.jp/browse/jos/ 10.5650/jos.ess14228
spellingShingle Alhassan, Fatah H.
Rashid, Umer
Yap, Taufiq Yun Hin
Synthesis of waste cooking oil based biodiesel via ferric-manganese promoted molybdenum oxide / zirconia nanoparticle solid acid catalyst: influence of ferric and manganese dopants
title Synthesis of waste cooking oil based biodiesel via ferric-manganese promoted molybdenum oxide / zirconia nanoparticle solid acid catalyst: influence of ferric and manganese dopants
title_full Synthesis of waste cooking oil based biodiesel via ferric-manganese promoted molybdenum oxide / zirconia nanoparticle solid acid catalyst: influence of ferric and manganese dopants
title_fullStr Synthesis of waste cooking oil based biodiesel via ferric-manganese promoted molybdenum oxide / zirconia nanoparticle solid acid catalyst: influence of ferric and manganese dopants
title_full_unstemmed Synthesis of waste cooking oil based biodiesel via ferric-manganese promoted molybdenum oxide / zirconia nanoparticle solid acid catalyst: influence of ferric and manganese dopants
title_short Synthesis of waste cooking oil based biodiesel via ferric-manganese promoted molybdenum oxide / zirconia nanoparticle solid acid catalyst: influence of ferric and manganese dopants
title_sort synthesis of waste cooking oil based biodiesel via ferric-manganese promoted molybdenum oxide / zirconia nanoparticle solid acid catalyst: influence of ferric and manganese dopants
url http://psasir.upm.edu.my/id/eprint/46475/
http://psasir.upm.edu.my/id/eprint/46475/
http://psasir.upm.edu.my/id/eprint/46475/
http://psasir.upm.edu.my/id/eprint/46475/1/Synthesis%20of%20waste%20cooking%20oil%20based%20biodiesel%20via%20ferric-manganese%20promoted%20molybdenum%20oxide%20%20zirconia%20nanoparticle%20solid%20acid%20catalyst%20influence%20of%20ferric%20and%20manganese%20dopants.pdf