Modification of commercial activated carbon for the removal of 2,4-dichlorophenol from simulated wastewater

In this study, modification of commercial activated carbon (AC) has been examined for the removal of 2,4-dichlorophenol (2,4-DCP) from aqueous solutions. The modified process involves impregnation of phosphoric acid at ratios of 0.6–2.4 followed by 500 °C and 700 °C for 2 h. The effect of different...

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Main Authors: Yap, Taufiq Yun Hin, Anisuzzaman, S. M., Joseph, Collin G., Krishnaiah, Duduku, Tay, V. V.
Format: Article
Language:English
Published: King Saud University 2015
Online Access:http://psasir.upm.edu.my/id/eprint/45512/
http://psasir.upm.edu.my/id/eprint/45512/1/CARBON.pdf
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author Yap, Taufiq Yun Hin
Anisuzzaman, S. M.
Joseph, Collin G.
Krishnaiah, Duduku
Tay, V. V.
author_facet Yap, Taufiq Yun Hin
Anisuzzaman, S. M.
Joseph, Collin G.
Krishnaiah, Duduku
Tay, V. V.
author_sort Yap, Taufiq Yun Hin
building UPM Institutional Repository
collection Online Access
description In this study, modification of commercial activated carbon (AC) has been examined for the removal of 2,4-dichlorophenol (2,4-DCP) from aqueous solutions. The modified process involves impregnation of phosphoric acid at ratios of 0.6–2.4 followed by 500 °C and 700 °C for 2 h. The effect of different impregnation ratios and activation temperatures was studied. Physical and chemical characterization of modified AC was conducted including percentage yield, moisture content, ash content, pH, morphology study and functional groups. The adsorption of 2,4-DCP by modified AC was also investigated. Various tests were conducted on the unmodified AC and chemically modified AC at different contact times (5–60 min) and adsorbent dosages (0.1–0.9 g). Results revealed that the modified AC (AC2) prepared with impregnation ratio, Xp value of 1.2 at 500 °C for 2 h was found to have the highest percentage removal of 2,4-DCP (50 ppm), which is 93.63%. The modified AC showed better capability to adsorb 2,4-DCP from aqueous solutions, the percentage removal was improved to 20.40%. Elovich and intraparticle diffusion kinetic models were used to test the adsorption kinetics. The adsorption of 2,4-DCP proved to fit better in the intraparticle diffusion model compared to Elovich equation. The mechanism of the adsorption process was determined by the intraparticle model.
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spelling upm-455122021-01-23T22:00:35Z http://psasir.upm.edu.my/id/eprint/45512/ Modification of commercial activated carbon for the removal of 2,4-dichlorophenol from simulated wastewater Yap, Taufiq Yun Hin Anisuzzaman, S. M. Joseph, Collin G. Krishnaiah, Duduku Tay, V. V. In this study, modification of commercial activated carbon (AC) has been examined for the removal of 2,4-dichlorophenol (2,4-DCP) from aqueous solutions. The modified process involves impregnation of phosphoric acid at ratios of 0.6–2.4 followed by 500 °C and 700 °C for 2 h. The effect of different impregnation ratios and activation temperatures was studied. Physical and chemical characterization of modified AC was conducted including percentage yield, moisture content, ash content, pH, morphology study and functional groups. The adsorption of 2,4-DCP by modified AC was also investigated. Various tests were conducted on the unmodified AC and chemically modified AC at different contact times (5–60 min) and adsorbent dosages (0.1–0.9 g). Results revealed that the modified AC (AC2) prepared with impregnation ratio, Xp value of 1.2 at 500 °C for 2 h was found to have the highest percentage removal of 2,4-DCP (50 ppm), which is 93.63%. The modified AC showed better capability to adsorb 2,4-DCP from aqueous solutions, the percentage removal was improved to 20.40%. Elovich and intraparticle diffusion kinetic models were used to test the adsorption kinetics. The adsorption of 2,4-DCP proved to fit better in the intraparticle diffusion model compared to Elovich equation. The mechanism of the adsorption process was determined by the intraparticle model. King Saud University 2015 Article PeerReviewed text en http://psasir.upm.edu.my/id/eprint/45512/1/CARBON.pdf Yap, Taufiq Yun Hin and Anisuzzaman, S. M. and Joseph, Collin G. and Krishnaiah, Duduku and Tay, V. V. (2015) Modification of commercial activated carbon for the removal of 2,4-dichlorophenol from simulated wastewater. Journal of King Saud University Science, 27 (4). pp. 318-330. ISSN 1018-3647 https://www.sciencedirect.com/science/article/pii/S101836471500004X 10.1016/j.jksus.2015.01.002
spellingShingle Yap, Taufiq Yun Hin
Anisuzzaman, S. M.
Joseph, Collin G.
Krishnaiah, Duduku
Tay, V. V.
Modification of commercial activated carbon for the removal of 2,4-dichlorophenol from simulated wastewater
title Modification of commercial activated carbon for the removal of 2,4-dichlorophenol from simulated wastewater
title_full Modification of commercial activated carbon for the removal of 2,4-dichlorophenol from simulated wastewater
title_fullStr Modification of commercial activated carbon for the removal of 2,4-dichlorophenol from simulated wastewater
title_full_unstemmed Modification of commercial activated carbon for the removal of 2,4-dichlorophenol from simulated wastewater
title_short Modification of commercial activated carbon for the removal of 2,4-dichlorophenol from simulated wastewater
title_sort modification of commercial activated carbon for the removal of 2,4-dichlorophenol from simulated wastewater
url http://psasir.upm.edu.my/id/eprint/45512/
http://psasir.upm.edu.my/id/eprint/45512/
http://psasir.upm.edu.my/id/eprint/45512/
http://psasir.upm.edu.my/id/eprint/45512/1/CARBON.pdf