Optimization of lipase-catalyzed synthesis of N-trans-feruloyltyramine using response surface methodology (RSM)

Enzymatic synthesis of N-trans-feruloyltyramine amide was optimized by response surface methodology (RSM) using 4-hydroxy-3-methoxycinnamic acid and tyramine hydrochloride in a one-step lipase catalyzed reaction using Lipozyme TL IM. Response surface methodology (RSM) based on five-level, four-varia...

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Main Authors: Basri, Mahiran, Alrub, Mohammad Abu, Abd Malek, Emilia, Alang Ahmad, Shahrul Ainliah, Salleh, Abu Bakar, Abdul Rahman, Mohd Basyaruddin
Format: Article
Published: Taylor & Francis 2014
Online Access:http://psasir.upm.edu.my/id/eprint/34773/
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author Basri, Mahiran
Alrub, Mohammad Abu
Abd Malek, Emilia
Alang Ahmad, Shahrul Ainliah
Salleh, Abu Bakar
Abdul Rahman, Mohd Basyaruddin
author_facet Basri, Mahiran
Alrub, Mohammad Abu
Abd Malek, Emilia
Alang Ahmad, Shahrul Ainliah
Salleh, Abu Bakar
Abdul Rahman, Mohd Basyaruddin
author_sort Basri, Mahiran
building UPM Institutional Repository
collection Online Access
description Enzymatic synthesis of N-trans-feruloyltyramine amide was optimized by response surface methodology (RSM) using 4-hydroxy-3-methoxycinnamic acid and tyramine hydrochloride in a one-step lipase catalyzed reaction using Lipozyme TL IM. Response surface methodology (RSM) based on five-level, four-variable central composite rotatable design (CCRD) was used to evaluate the interaction of synthesis, reaction time (24–96 h), temperature (30°–50°C), amount of enzyme (50–500 mg, 12.5–125.0 IUN), and substrate molar ratio (cinnamic acid:tyramine HCl) 1:1–8:1 mmol on the percentage yield of N-trans-feruloyltyramine amide. The optimum conditions derived via RSM were: reaction time 52 h, temperature 43°C, amount of enzyme 260 mg (65.0 IUN), and substrate molar ratio (cinnamic acid:tyramine HCl) 6.2:1. The actual experimental yield was 96.3% under optimum conditions, which compared well to the maximum predicted value of 97.2%.
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spelling upm-347732015-12-23T00:44:22Z http://psasir.upm.edu.my/id/eprint/34773/ Optimization of lipase-catalyzed synthesis of N-trans-feruloyltyramine using response surface methodology (RSM) Basri, Mahiran Alrub, Mohammad Abu Abd Malek, Emilia Alang Ahmad, Shahrul Ainliah Salleh, Abu Bakar Abdul Rahman, Mohd Basyaruddin Enzymatic synthesis of N-trans-feruloyltyramine amide was optimized by response surface methodology (RSM) using 4-hydroxy-3-methoxycinnamic acid and tyramine hydrochloride in a one-step lipase catalyzed reaction using Lipozyme TL IM. Response surface methodology (RSM) based on five-level, four-variable central composite rotatable design (CCRD) was used to evaluate the interaction of synthesis, reaction time (24–96 h), temperature (30°–50°C), amount of enzyme (50–500 mg, 12.5–125.0 IUN), and substrate molar ratio (cinnamic acid:tyramine HCl) 1:1–8:1 mmol on the percentage yield of N-trans-feruloyltyramine amide. The optimum conditions derived via RSM were: reaction time 52 h, temperature 43°C, amount of enzyme 260 mg (65.0 IUN), and substrate molar ratio (cinnamic acid:tyramine HCl) 6.2:1. The actual experimental yield was 96.3% under optimum conditions, which compared well to the maximum predicted value of 97.2%. Taylor & Francis 2014 Article PeerReviewed Basri, Mahiran and Alrub, Mohammad Abu and Abd Malek, Emilia and Alang Ahmad, Shahrul Ainliah and Salleh, Abu Bakar and Abdul Rahman, Mohd Basyaruddin (2014) Optimization of lipase-catalyzed synthesis of N-trans-feruloyltyramine using response surface methodology (RSM). Chemical Engineering Communications, 201 (12). pp. 1582-1592. ISSN 0098-6445; ESSN: 1563-5201 http://www.tandfonline.com/doi/abs/10.1080/00986445.2013.821060 10.1080/00986445.2013.821060
spellingShingle Basri, Mahiran
Alrub, Mohammad Abu
Abd Malek, Emilia
Alang Ahmad, Shahrul Ainliah
Salleh, Abu Bakar
Abdul Rahman, Mohd Basyaruddin
Optimization of lipase-catalyzed synthesis of N-trans-feruloyltyramine using response surface methodology (RSM)
title Optimization of lipase-catalyzed synthesis of N-trans-feruloyltyramine using response surface methodology (RSM)
title_full Optimization of lipase-catalyzed synthesis of N-trans-feruloyltyramine using response surface methodology (RSM)
title_fullStr Optimization of lipase-catalyzed synthesis of N-trans-feruloyltyramine using response surface methodology (RSM)
title_full_unstemmed Optimization of lipase-catalyzed synthesis of N-trans-feruloyltyramine using response surface methodology (RSM)
title_short Optimization of lipase-catalyzed synthesis of N-trans-feruloyltyramine using response surface methodology (RSM)
title_sort optimization of lipase-catalyzed synthesis of n-trans-feruloyltyramine using response surface methodology (rsm)
url http://psasir.upm.edu.my/id/eprint/34773/
http://psasir.upm.edu.my/id/eprint/34773/
http://psasir.upm.edu.my/id/eprint/34773/