Effect of chemical surface treatment on the mechanical properties of reinforced plasticized poly(lactic acid) biodegradable composites

Biodegradable composites were prepared by melt-blending technique using 30 wt% kenaf bast fiber (KBF) to reinforce 70 wt% plasticized poly(lactic acid) (PLA). The KBF was treated with various percentages of sodium hydroxide (NaOH), whereas 5% triacetin was used as plasticizer. The effects of the KBF...

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Main Authors: Ibrahim, Nor Azowa, Wan Yunus, Wan Md. Zin, Osman, Maizatul, Abdan, Khalina
Format: Article
Language:English
Published: SAGE Publications 2011
Online Access:http://psasir.upm.edu.my/id/eprint/25049/
http://psasir.upm.edu.my/id/eprint/25049/1/Effect%20of%20chemical%20surface%20treatment%20on%20the%20mechanical%20properties%20of%20reinforced%20plasticized%20poly.pdf
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author Ibrahim, Nor Azowa
Wan Yunus, Wan Md. Zin
Osman, Maizatul
Abdan, Khalina
author_facet Ibrahim, Nor Azowa
Wan Yunus, Wan Md. Zin
Osman, Maizatul
Abdan, Khalina
author_sort Ibrahim, Nor Azowa
building UPM Institutional Repository
collection Online Access
description Biodegradable composites were prepared by melt-blending technique using 30 wt% kenaf bast fiber (KBF) to reinforce 70 wt% plasticized poly(lactic acid) (PLA). The KBF was treated with various percentages of sodium hydroxide (NaOH), whereas 5% triacetin was used as plasticizer. The effects of the KBF surface treatments on the tensile, flexural, impact strength, and DMA of the biocomposites were investigated. Tensile, flexural, and impact testing results reveal that 4% of NaOH-treated KBF produced composites with optimum tensile strength (62 MPa), flexural strength (67 MPa), and the impact strength (42 kJ/m2). The removal of the lignin from the fiber during the surface treatment caused the increment in the modulus result. This finding is also supported by the dynamic mechanical analysis. The storage modulus of plasticized PLA/treated KBF is higher than the storage modulus of plasticized PLA/untreated KBF which is attributed to the enhancement of the fiber—matrix adhesion. The loss modulus results showed that the Tg of the plasticized composites was shifting to higher temperature, from 55°C for plasticized PLA/untreated KBF to 65°C for plasticized PLA/treated KBF. The increase in Tg shows that the plasticized PLA has low chain mobility when reinforced with treated KBF, indicating better interaction.
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spelling upm-250492019-11-20T02:10:48Z http://psasir.upm.edu.my/id/eprint/25049/ Effect of chemical surface treatment on the mechanical properties of reinforced plasticized poly(lactic acid) biodegradable composites Ibrahim, Nor Azowa Wan Yunus, Wan Md. Zin Osman, Maizatul Abdan, Khalina Biodegradable composites were prepared by melt-blending technique using 30 wt% kenaf bast fiber (KBF) to reinforce 70 wt% plasticized poly(lactic acid) (PLA). The KBF was treated with various percentages of sodium hydroxide (NaOH), whereas 5% triacetin was used as plasticizer. The effects of the KBF surface treatments on the tensile, flexural, impact strength, and DMA of the biocomposites were investigated. Tensile, flexural, and impact testing results reveal that 4% of NaOH-treated KBF produced composites with optimum tensile strength (62 MPa), flexural strength (67 MPa), and the impact strength (42 kJ/m2). The removal of the lignin from the fiber during the surface treatment caused the increment in the modulus result. This finding is also supported by the dynamic mechanical analysis. The storage modulus of plasticized PLA/treated KBF is higher than the storage modulus of plasticized PLA/untreated KBF which is attributed to the enhancement of the fiber—matrix adhesion. The loss modulus results showed that the Tg of the plasticized composites was shifting to higher temperature, from 55°C for plasticized PLA/untreated KBF to 65°C for plasticized PLA/treated KBF. The increase in Tg shows that the plasticized PLA has low chain mobility when reinforced with treated KBF, indicating better interaction. SAGE Publications 2011 Article PeerReviewed application/pdf en http://psasir.upm.edu.my/id/eprint/25049/1/Effect%20of%20chemical%20surface%20treatment%20on%20the%20mechanical%20properties%20of%20reinforced%20plasticized%20poly.pdf Ibrahim, Nor Azowa and Wan Yunus, Wan Md. Zin and Osman, Maizatul and Abdan, Khalina (2011) Effect of chemical surface treatment on the mechanical properties of reinforced plasticized poly(lactic acid) biodegradable composites. Journal of Reinforced Plastics and Composites, 30 (5). pp. 381-388. ISSN 0731-6844 https://journals.sagepub.com/doi/10.1177/0731684410396595 10.1177/0731684410396595
spellingShingle Ibrahim, Nor Azowa
Wan Yunus, Wan Md. Zin
Osman, Maizatul
Abdan, Khalina
Effect of chemical surface treatment on the mechanical properties of reinforced plasticized poly(lactic acid) biodegradable composites
title Effect of chemical surface treatment on the mechanical properties of reinforced plasticized poly(lactic acid) biodegradable composites
title_full Effect of chemical surface treatment on the mechanical properties of reinforced plasticized poly(lactic acid) biodegradable composites
title_fullStr Effect of chemical surface treatment on the mechanical properties of reinforced plasticized poly(lactic acid) biodegradable composites
title_full_unstemmed Effect of chemical surface treatment on the mechanical properties of reinforced plasticized poly(lactic acid) biodegradable composites
title_short Effect of chemical surface treatment on the mechanical properties of reinforced plasticized poly(lactic acid) biodegradable composites
title_sort effect of chemical surface treatment on the mechanical properties of reinforced plasticized poly(lactic acid) biodegradable composites
url http://psasir.upm.edu.my/id/eprint/25049/
http://psasir.upm.edu.my/id/eprint/25049/
http://psasir.upm.edu.my/id/eprint/25049/
http://psasir.upm.edu.my/id/eprint/25049/1/Effect%20of%20chemical%20surface%20treatment%20on%20the%20mechanical%20properties%20of%20reinforced%20plasticized%20poly.pdf