Identification of the anti-epileptic effect of speciogynine through molecular network-aided metabolite profiling of M. speciosa alkaloids using zebrafish

Mitragyna speciosa is a native plant to Southeast Asian countries, known its medicinal use as an analgesic and stimulant. Apart from the indole-type alkaloids, which have been shown to be responsible for its pharmacological properties, there is still limited information on other classes of compounds...

Full description

Bibliographic Details
Main Authors: Garba, Suleiman Abubakar, Swain, Puspanjali, Shaari, Khozirah, Afzan, Adlin, Lee, Soo Yee, Kim, Cheol-Hee, Mohd Faudzi, Siti Munirah
Format: Article
Language:English
Published: Elsevier B.V. 2025
Online Access:http://psasir.upm.edu.my/id/eprint/120720/
http://psasir.upm.edu.my/id/eprint/120720/1/120720.pdf
_version_ 1848868221677993984
author Garba, Suleiman Abubakar
Swain, Puspanjali
Shaari, Khozirah
Afzan, Adlin
Lee, Soo Yee
Kim, Cheol-Hee
Mohd Faudzi, Siti Munirah
author_facet Garba, Suleiman Abubakar
Swain, Puspanjali
Shaari, Khozirah
Afzan, Adlin
Lee, Soo Yee
Kim, Cheol-Hee
Mohd Faudzi, Siti Munirah
author_sort Garba, Suleiman Abubakar
building UPM Institutional Repository
collection Online Access
description Mitragyna speciosa is a native plant to Southeast Asian countries, known its medicinal use as an analgesic and stimulant. Apart from the indole-type alkaloids, which have been shown to be responsible for its pharmacological properties, there is still limited information on other classes of compounds present in various parts of the plant. In an effort to fill this knowledge gap, the present study applied tandem liquid chromatography-mass spectrometry (LC-MS/MS)-based molecular networking to obtain more information on the chemodiversity of M. speciosa. Analysis of the generated molecular map obtained from methanol extracts of leaves (green- and red-veined), stem bark, stem tissue and fruits, revealed the putative presence of not only the characteristic indole-type alkaloids, but also flavoalkaloids, iridoids, triterpenoid saponins, glycoside derivatives, phenolic acids, flavonoids, and polyphenols, pervading all different parts of the plant. The class of flavoalkaloids is reported herein as new for M. speciosa. Continuing our interest in the biological properties of the chemical constituents of the plant, two minor indole alkaloids, speciogynine and isopaynantheine, purified from the leaf extract were evaluated for their toxicity and antiepileptic potential in zebrafish animal model. Interestingly, speciogynine exhibited a significant dose-dependent effect in reducing hyperactive movements in a zebrafish epilepsy model with mild toxic effects, indicating that it could be a promising anti-epileptic lead compound for further exploration.
first_indexed 2025-11-15T14:48:57Z
format Article
id upm-120720
institution Universiti Putra Malaysia
institution_category Local University
language English
last_indexed 2025-11-15T14:48:57Z
publishDate 2025
publisher Elsevier B.V.
recordtype eprints
repository_type Digital Repository
spelling upm-1207202025-10-08T08:24:18Z http://psasir.upm.edu.my/id/eprint/120720/ Identification of the anti-epileptic effect of speciogynine through molecular network-aided metabolite profiling of M. speciosa alkaloids using zebrafish Garba, Suleiman Abubakar Swain, Puspanjali Shaari, Khozirah Afzan, Adlin Lee, Soo Yee Kim, Cheol-Hee Mohd Faudzi, Siti Munirah Mitragyna speciosa is a native plant to Southeast Asian countries, known its medicinal use as an analgesic and stimulant. Apart from the indole-type alkaloids, which have been shown to be responsible for its pharmacological properties, there is still limited information on other classes of compounds present in various parts of the plant. In an effort to fill this knowledge gap, the present study applied tandem liquid chromatography-mass spectrometry (LC-MS/MS)-based molecular networking to obtain more information on the chemodiversity of M. speciosa. Analysis of the generated molecular map obtained from methanol extracts of leaves (green- and red-veined), stem bark, stem tissue and fruits, revealed the putative presence of not only the characteristic indole-type alkaloids, but also flavoalkaloids, iridoids, triterpenoid saponins, glycoside derivatives, phenolic acids, flavonoids, and polyphenols, pervading all different parts of the plant. The class of flavoalkaloids is reported herein as new for M. speciosa. Continuing our interest in the biological properties of the chemical constituents of the plant, two minor indole alkaloids, speciogynine and isopaynantheine, purified from the leaf extract were evaluated for their toxicity and antiepileptic potential in zebrafish animal model. Interestingly, speciogynine exhibited a significant dose-dependent effect in reducing hyperactive movements in a zebrafish epilepsy model with mild toxic effects, indicating that it could be a promising anti-epileptic lead compound for further exploration. Elsevier B.V. 2025 Article PeerReviewed text en http://psasir.upm.edu.my/id/eprint/120720/1/120720.pdf Garba, Suleiman Abubakar and Swain, Puspanjali and Shaari, Khozirah and Afzan, Adlin and Lee, Soo Yee and Kim, Cheol-Hee and Mohd Faudzi, Siti Munirah (2025) Identification of the anti-epileptic effect of speciogynine through molecular network-aided metabolite profiling of M. speciosa alkaloids using zebrafish. Fitoterapia, 184. art. no. 106667. pp. 1-17. ISSN 0367-326X; eISSN: 1873-6971 https://www.sciencedirect.com/science/article/pii/S0367326X25002928?via%3Dihub 10.1016/j.fitote.2025.106667
spellingShingle Garba, Suleiman Abubakar
Swain, Puspanjali
Shaari, Khozirah
Afzan, Adlin
Lee, Soo Yee
Kim, Cheol-Hee
Mohd Faudzi, Siti Munirah
Identification of the anti-epileptic effect of speciogynine through molecular network-aided metabolite profiling of M. speciosa alkaloids using zebrafish
title Identification of the anti-epileptic effect of speciogynine through molecular network-aided metabolite profiling of M. speciosa alkaloids using zebrafish
title_full Identification of the anti-epileptic effect of speciogynine through molecular network-aided metabolite profiling of M. speciosa alkaloids using zebrafish
title_fullStr Identification of the anti-epileptic effect of speciogynine through molecular network-aided metabolite profiling of M. speciosa alkaloids using zebrafish
title_full_unstemmed Identification of the anti-epileptic effect of speciogynine through molecular network-aided metabolite profiling of M. speciosa alkaloids using zebrafish
title_short Identification of the anti-epileptic effect of speciogynine through molecular network-aided metabolite profiling of M. speciosa alkaloids using zebrafish
title_sort identification of the anti-epileptic effect of speciogynine through molecular network-aided metabolite profiling of m. speciosa alkaloids using zebrafish
url http://psasir.upm.edu.my/id/eprint/120720/
http://psasir.upm.edu.my/id/eprint/120720/
http://psasir.upm.edu.my/id/eprint/120720/
http://psasir.upm.edu.my/id/eprint/120720/1/120720.pdf