Influence of surface passivation on indium arsenide nanowire band gap energies

The interplay between surface chemistry and quantum confinement on the band gap energies of indium arsenide (InAs) nanowires is investigated by first principle computations as the surface-to-volume ratio increases with decreasing cross section. Electronic band structures are presented as determined...

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Main Authors: Razavi, Pedram, Greer, James C.
Format: Article
Language:English
Published: Springer 2019
Online Access:https://eprints.nottingham.ac.uk/57323/
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author Razavi, Pedram
Greer, James C.
author_facet Razavi, Pedram
Greer, James C.
author_sort Razavi, Pedram
building Nottingham Research Data Repository
collection Online Access
description The interplay between surface chemistry and quantum confinement on the band gap energies of indium arsenide (InAs) nanowires is investigated by first principle computations as the surface-to-volume ratio increases with decreasing cross section. Electronic band structures are presented as determined by both density functional and hybrid density functional theory (DFT) calculations; the latter are used to provide improved band gap energy estimates over those from standard approximate DFT methods. Different monovalent chemical species with varying electron affinity are used to eliminate surface states to enable direct comparison between surface chemistry and quantum confinement. The influence of these effects on energy band gaps and electron effective masses is highlighted. It is found that many desirable properties in terms of electronic properties and the elimination of surface states for nanoscale field effect transistors fabricated using [100]-oriented InAs can be achieved. © 2019, The Minerals, Metals & Materials Society.
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spelling nottingham-573232020-07-31T04:30:13Z https://eprints.nottingham.ac.uk/57323/ Influence of surface passivation on indium arsenide nanowire band gap energies Razavi, Pedram Greer, James C. The interplay between surface chemistry and quantum confinement on the band gap energies of indium arsenide (InAs) nanowires is investigated by first principle computations as the surface-to-volume ratio increases with decreasing cross section. Electronic band structures are presented as determined by both density functional and hybrid density functional theory (DFT) calculations; the latter are used to provide improved band gap energy estimates over those from standard approximate DFT methods. Different monovalent chemical species with varying electron affinity are used to eliminate surface states to enable direct comparison between surface chemistry and quantum confinement. The influence of these effects on energy band gaps and electron effective masses is highlighted. It is found that many desirable properties in terms of electronic properties and the elimination of surface states for nanoscale field effect transistors fabricated using [100]-oriented InAs can be achieved. © 2019, The Minerals, Metals & Materials Society. Springer 2019-10-31 Article PeerReviewed application/pdf en https://eprints.nottingham.ac.uk/57323/1/combinepdf.pdf Razavi, Pedram and Greer, James C. (2019) Influence of surface passivation on indium arsenide nanowire band gap energies. Journal of Electronic Materials, 48 (10). pp. 6654-6660. ISSN 0361-5235 https://link.springer.com/article/10.1007%2Fs11664-019-07476-0 doi:10.1007/s11664-019-07476-0 doi:10.1007/s11664-019-07476-0
spellingShingle Razavi, Pedram
Greer, James C.
Influence of surface passivation on indium arsenide nanowire band gap energies
title Influence of surface passivation on indium arsenide nanowire band gap energies
title_full Influence of surface passivation on indium arsenide nanowire band gap energies
title_fullStr Influence of surface passivation on indium arsenide nanowire band gap energies
title_full_unstemmed Influence of surface passivation on indium arsenide nanowire band gap energies
title_short Influence of surface passivation on indium arsenide nanowire band gap energies
title_sort influence of surface passivation on indium arsenide nanowire band gap energies
url https://eprints.nottingham.ac.uk/57323/
https://eprints.nottingham.ac.uk/57323/
https://eprints.nottingham.ac.uk/57323/