Significant enhancement of structural stability of the hyperhalophilic ADH from Haloferax volcanii via entrapment on metal organic framework support

The use of an in-situ immobilization procedure for the immobilization of hyperhalophilic alcohol dehydrogenase in a metal organic framework material is described. The easy and rapid in situ immobilization process enables retention of activity over a broad range of pH and temperature together with a...

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Main Authors: Carucci, Cristina, Bruen, Larah, Gascón, Victoria, Paradisi, Francesca, Magner, Edmond
Format: Article
Published: ACS Publications 2018
Online Access:https://eprints.nottingham.ac.uk/52945/
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author Carucci, Cristina
Bruen, Larah
Gascón, Victoria
Paradisi, Francesca
Magner, Edmond
author_facet Carucci, Cristina
Bruen, Larah
Gascón, Victoria
Paradisi, Francesca
Magner, Edmond
author_sort Carucci, Cristina
building Nottingham Research Data Repository
collection Online Access
description The use of an in-situ immobilization procedure for the immobilization of hyperhalophilic alcohol dehydrogenase in a metal organic framework material is described. The easy and rapid in situ immobilization process enables retention of activity over a broad range of pH and temperature together with a decrease in the halophilicity of the enzyme. The catalytic activity of the immobilized enzyme was studied in non-aqueous solvent mixtures with the highest retention of activity in aqueous solutions of methanol and acetonitrile. The approach demonstrates that this immobilization method can be extended to hyperhalophilic enzymes with enhancements in activity and stability.
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spelling nottingham-529452020-05-04T19:41:17Z https://eprints.nottingham.ac.uk/52945/ Significant enhancement of structural stability of the hyperhalophilic ADH from Haloferax volcanii via entrapment on metal organic framework support Carucci, Cristina Bruen, Larah Gascón, Victoria Paradisi, Francesca Magner, Edmond The use of an in-situ immobilization procedure for the immobilization of hyperhalophilic alcohol dehydrogenase in a metal organic framework material is described. The easy and rapid in situ immobilization process enables retention of activity over a broad range of pH and temperature together with a decrease in the halophilicity of the enzyme. The catalytic activity of the immobilized enzyme was studied in non-aqueous solvent mixtures with the highest retention of activity in aqueous solutions of methanol and acetonitrile. The approach demonstrates that this immobilization method can be extended to hyperhalophilic enzymes with enhancements in activity and stability. ACS Publications 2018-06-19 Article PeerReviewed Carucci, Cristina, Bruen, Larah, Gascón, Victoria, Paradisi, Francesca and Magner, Edmond (2018) Significant enhancement of structural stability of the hyperhalophilic ADH from Haloferax volcanii via entrapment on metal organic framework support. Langmuir . ISSN 0743-7463 https://pubs.acs.org/doi/abs/10.1021/acs.langmuir.8b01037 doi:10.1021/acs.langmuir.8b01037 doi:10.1021/acs.langmuir.8b01037
spellingShingle Carucci, Cristina
Bruen, Larah
Gascón, Victoria
Paradisi, Francesca
Magner, Edmond
Significant enhancement of structural stability of the hyperhalophilic ADH from Haloferax volcanii via entrapment on metal organic framework support
title Significant enhancement of structural stability of the hyperhalophilic ADH from Haloferax volcanii via entrapment on metal organic framework support
title_full Significant enhancement of structural stability of the hyperhalophilic ADH from Haloferax volcanii via entrapment on metal organic framework support
title_fullStr Significant enhancement of structural stability of the hyperhalophilic ADH from Haloferax volcanii via entrapment on metal organic framework support
title_full_unstemmed Significant enhancement of structural stability of the hyperhalophilic ADH from Haloferax volcanii via entrapment on metal organic framework support
title_short Significant enhancement of structural stability of the hyperhalophilic ADH from Haloferax volcanii via entrapment on metal organic framework support
title_sort significant enhancement of structural stability of the hyperhalophilic adh from haloferax volcanii via entrapment on metal organic framework support
url https://eprints.nottingham.ac.uk/52945/
https://eprints.nottingham.ac.uk/52945/
https://eprints.nottingham.ac.uk/52945/