Assessment of time-dependent density functional theory with the restricted excitation space approximation for excited state calculations of large systems

The restricted excitation subspace approximation is explored as a basis to reduce the memory storage required in linear response time-dependent density functional theory (TDDFT) calculations within the Tamm-Dancoff approximation. It is shown that excluding the core orbitals and up to 70% of the virt...

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Bibliographic Details
Main Authors: Hanson-Heine, Magnus W.D., George, Michael W., Besley, Nicholas A.
Format: Article
Language:English
Published: Taylor & Francis 2018
Subjects:
Online Access:https://eprints.nottingham.ac.uk/49206/