Excitonic mobility edge and ultra-short photoluminescence decay time in n-type GaAsN

We use time-resolved photoluminescence (PL) spectroscopy to study the recombination dynamics in Si-doped GaAsN semiconductor alloys with a nitrogen content up to 0.2%. The PL decay is predominantly monoexponential and exhibits a strong energy dispersion. We find ultra-short decay times on the high-e...

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Main Authors: Eßer, F., Winner, S., Patanè, Amalia, Helm, M., Schneider, H.
Format: Article
Published: American Institute of Physics 2016
Online Access:https://eprints.nottingham.ac.uk/39577/
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author Eßer, F.
Winner, S.
Patanè, Amalia
Helm, M.
Schneider, H.
author_facet Eßer, F.
Winner, S.
Patanè, Amalia
Helm, M.
Schneider, H.
author_sort Eßer, F.
building Nottingham Research Data Repository
collection Online Access
description We use time-resolved photoluminescence (PL) spectroscopy to study the recombination dynamics in Si-doped GaAsN semiconductor alloys with a nitrogen content up to 0.2%. The PL decay is predominantly monoexponential and exhibits a strong energy dispersion. We find ultra-short decay times on the high-energy side and long decay times on the low-energy side of the photoluminescence spectrum. This asymmetry can be explained by the existence of an additional non-radiative energy transfer channel and is consistent with previous studies on intrinsic GaAsN epilayers. However, the determined maximum decay times of GaAsN:Si are significantly reduced in comparison to undoped GaAsN. The determined excitonic mobility edge energy constantly decreases with an increase in the N content, in agreement with the two-level band anticrossing model.
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spelling nottingham-395772020-05-04T18:22:33Z https://eprints.nottingham.ac.uk/39577/ Excitonic mobility edge and ultra-short photoluminescence decay time in n-type GaAsN Eßer, F. Winner, S. Patanè, Amalia Helm, M. Schneider, H. We use time-resolved photoluminescence (PL) spectroscopy to study the recombination dynamics in Si-doped GaAsN semiconductor alloys with a nitrogen content up to 0.2%. The PL decay is predominantly monoexponential and exhibits a strong energy dispersion. We find ultra-short decay times on the high-energy side and long decay times on the low-energy side of the photoluminescence spectrum. This asymmetry can be explained by the existence of an additional non-radiative energy transfer channel and is consistent with previous studies on intrinsic GaAsN epilayers. However, the determined maximum decay times of GaAsN:Si are significantly reduced in comparison to undoped GaAsN. The determined excitonic mobility edge energy constantly decreases with an increase in the N content, in agreement with the two-level band anticrossing model. American Institute of Physics 2016-11-03 Article PeerReviewed Eßer, F., Winner, S., Patanè, Amalia, Helm, M. and Schneider, H. (2016) Excitonic mobility edge and ultra-short photoluminescence decay time in n-type GaAsN. Applied Physics Letters, 109 (18). 182113/1-182113/4. ISSN 1077-3118 http://aip.scitation.org/doi/10.1063/1.4966949 doi: 10.1063/1.4966949 doi: 10.1063/1.4966949
spellingShingle Eßer, F.
Winner, S.
Patanè, Amalia
Helm, M.
Schneider, H.
Excitonic mobility edge and ultra-short photoluminescence decay time in n-type GaAsN
title Excitonic mobility edge and ultra-short photoluminescence decay time in n-type GaAsN
title_full Excitonic mobility edge and ultra-short photoluminescence decay time in n-type GaAsN
title_fullStr Excitonic mobility edge and ultra-short photoluminescence decay time in n-type GaAsN
title_full_unstemmed Excitonic mobility edge and ultra-short photoluminescence decay time in n-type GaAsN
title_short Excitonic mobility edge and ultra-short photoluminescence decay time in n-type GaAsN
title_sort excitonic mobility edge and ultra-short photoluminescence decay time in n-type gaasn
url https://eprints.nottingham.ac.uk/39577/
https://eprints.nottingham.ac.uk/39577/
https://eprints.nottingham.ac.uk/39577/