Mass spectrometry insights into a tandem ubiquitin-binding domain hybrid engineered for the selective recognition of unanchored polyubiquitin

Unanchored polyubiquitin chains are emerging as importanregulators of cellular physiology with diverse roles paralleling those of substrate-conjugated polyubiquitin. However tools able to discriminate unanchored polyubiquitin chains of different isopeptide linkages have not been described. We descri...

Full description

Bibliographic Details
Main Authors: Scott, Daniel, Garner, Tom P., Long, Jed, Strachan, Jo, Mistry, Sharad C., Bottrill, Andrew R., Tooth, David J., Searle, Mark S., Oldham, Neil J., Layfield, Rob
Format: Article
Published: Wiley-VCH Verlag 2016
Online Access:https://eprints.nottingham.ac.uk/32622/
_version_ 1848794451434012672
author Scott, Daniel
Garner, Tom P.
Long, Jed
Strachan, Jo
Mistry, Sharad C.
Bottrill, Andrew R.
Tooth, David J.
Searle, Mark S.
Oldham, Neil J.
Layfield, Rob
author_facet Scott, Daniel
Garner, Tom P.
Long, Jed
Strachan, Jo
Mistry, Sharad C.
Bottrill, Andrew R.
Tooth, David J.
Searle, Mark S.
Oldham, Neil J.
Layfield, Rob
author_sort Scott, Daniel
building Nottingham Research Data Repository
collection Online Access
description Unanchored polyubiquitin chains are emerging as importanregulators of cellular physiology with diverse roles paralleling those of substrate-conjugated polyubiquitin. However tools able to discriminate unanchored polyubiquitin chains of different isopeptide linkages have not been described. We describe the design of a linker-optimised ubiquitin-binding domain hybrid (t-UBD) containing two UBDs, a ZnF-UBP domain in tandem with a linkage-selective UBA domain, which exploits avidity effects to afford selective recognition of unanchored Lys48-linked polyubiquitin chains. Utilising native MS to quantitatively probe binding affinities we confirm cooperative binding of the UBDs within the synthetic protein, and desired binding specificity for Lys48-linked ubiquitin dimers. Furthermore MS/MS analyses indicate that the t-UBD, when applied as an affinity enrichment reagent, can be used to favour the purification of endogenous unanchored Lys48-linked polyubiquitin chains from mammalian cell extracts. Our study indicates that strategies for the rational design and engineering of polyubiquitin chain-selective binding in non-biological polymers are possible, paving the way for the generation of reagents to probe unanchored polyubiquitin chains of different linkages and more broadly the ‘ubiquitome’.
first_indexed 2025-11-14T19:16:24Z
format Article
id nottingham-32622
institution University of Nottingham Malaysia Campus
institution_category Local University
last_indexed 2025-11-14T19:16:24Z
publishDate 2016
publisher Wiley-VCH Verlag
recordtype eprints
repository_type Digital Repository
spelling nottingham-326222020-05-04T18:00:15Z https://eprints.nottingham.ac.uk/32622/ Mass spectrometry insights into a tandem ubiquitin-binding domain hybrid engineered for the selective recognition of unanchored polyubiquitin Scott, Daniel Garner, Tom P. Long, Jed Strachan, Jo Mistry, Sharad C. Bottrill, Andrew R. Tooth, David J. Searle, Mark S. Oldham, Neil J. Layfield, Rob Unanchored polyubiquitin chains are emerging as importanregulators of cellular physiology with diverse roles paralleling those of substrate-conjugated polyubiquitin. However tools able to discriminate unanchored polyubiquitin chains of different isopeptide linkages have not been described. We describe the design of a linker-optimised ubiquitin-binding domain hybrid (t-UBD) containing two UBDs, a ZnF-UBP domain in tandem with a linkage-selective UBA domain, which exploits avidity effects to afford selective recognition of unanchored Lys48-linked polyubiquitin chains. Utilising native MS to quantitatively probe binding affinities we confirm cooperative binding of the UBDs within the synthetic protein, and desired binding specificity for Lys48-linked ubiquitin dimers. Furthermore MS/MS analyses indicate that the t-UBD, when applied as an affinity enrichment reagent, can be used to favour the purification of endogenous unanchored Lys48-linked polyubiquitin chains from mammalian cell extracts. Our study indicates that strategies for the rational design and engineering of polyubiquitin chain-selective binding in non-biological polymers are possible, paving the way for the generation of reagents to probe unanchored polyubiquitin chains of different linkages and more broadly the ‘ubiquitome’. Wiley-VCH Verlag 2016-07-21 Article PeerReviewed Scott, Daniel, Garner, Tom P., Long, Jed, Strachan, Jo, Mistry, Sharad C., Bottrill, Andrew R., Tooth, David J., Searle, Mark S., Oldham, Neil J. and Layfield, Rob (2016) Mass spectrometry insights into a tandem ubiquitin-binding domain hybrid engineered for the selective recognition of unanchored polyubiquitin. Proteomics, 16 (14). pp. 1961-1969. ISSN 1615-9861 http://onlinelibrary.wiley.com/doi/10.1002/pmic.201600067/abstract doi:10.1002/pmic.201600067 doi:10.1002/pmic.201600067
spellingShingle Scott, Daniel
Garner, Tom P.
Long, Jed
Strachan, Jo
Mistry, Sharad C.
Bottrill, Andrew R.
Tooth, David J.
Searle, Mark S.
Oldham, Neil J.
Layfield, Rob
Mass spectrometry insights into a tandem ubiquitin-binding domain hybrid engineered for the selective recognition of unanchored polyubiquitin
title Mass spectrometry insights into a tandem ubiquitin-binding domain hybrid engineered for the selective recognition of unanchored polyubiquitin
title_full Mass spectrometry insights into a tandem ubiquitin-binding domain hybrid engineered for the selective recognition of unanchored polyubiquitin
title_fullStr Mass spectrometry insights into a tandem ubiquitin-binding domain hybrid engineered for the selective recognition of unanchored polyubiquitin
title_full_unstemmed Mass spectrometry insights into a tandem ubiquitin-binding domain hybrid engineered for the selective recognition of unanchored polyubiquitin
title_short Mass spectrometry insights into a tandem ubiquitin-binding domain hybrid engineered for the selective recognition of unanchored polyubiquitin
title_sort mass spectrometry insights into a tandem ubiquitin-binding domain hybrid engineered for the selective recognition of unanchored polyubiquitin
url https://eprints.nottingham.ac.uk/32622/
https://eprints.nottingham.ac.uk/32622/
https://eprints.nottingham.ac.uk/32622/