Electrochemical oxidation of D-fructose solution using the Box–Behnken design methodology

The electrochemical oxidation of D-fructose solution was studied using a Box–Behnken design. Seventeen batch runs of electrochemical oxidation were conducted based on three sets of operating conditions generated using Design-Expert software. The effects of D-fructose concentration, applied voltage a...

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Main Authors: Tay, Chen Lim, Fam, S.L.
Format: Journal Article
Published: Taylor & Francis Ltd. 2014
Subjects:
Online Access:http://hdl.handle.net/20.500.11937/9420
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author Tay, Chen Lim
Fam, S.L.
author_facet Tay, Chen Lim
Fam, S.L.
author_sort Tay, Chen Lim
building Curtin Institutional Repository
collection Online Access
description The electrochemical oxidation of D-fructose solution was studied using a Box–Behnken design. Seventeen batch runs of electrochemical oxidation were conducted based on three sets of operating conditions generated using Design-Expert software. The effects of D-fructose concentration, applied voltage and NaOH concentration on oxidation percentage and oxidation rate were studied. As revealed by ANOVA, the D-fructose and NaOH concentrations significantly affected the oxidation percentage, and the applied voltage and NaOH concentration significantly affected the oxidation rate. Functional models for the oxidation percentage and oxidation rate were generated and reported. The electrochemical oxidation of D-fructose was optimised by maximising the D-fructose concentration and minimising the applied voltage and NaOH concentration. The models were validated by comparing the adjusted optimised solution with the experimental data. A 62.78% electrochemical oxidation percentage and an oxidation rate of 12.20 mM/L h were achieved using 82% D-fructose with 0.14 M NaOH and a 10 V applied voltage.
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institution Curtin University Malaysia
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spelling curtin-20.500.11937-94202017-09-13T14:52:44Z Electrochemical oxidation of D-fructose solution using the Box–Behnken design methodology Tay, Chen Lim Fam, S.L. Box–Behnken Electrochemical oxidation Wastewater treatment D-fructose Optimisation Modelling The electrochemical oxidation of D-fructose solution was studied using a Box–Behnken design. Seventeen batch runs of electrochemical oxidation were conducted based on three sets of operating conditions generated using Design-Expert software. The effects of D-fructose concentration, applied voltage and NaOH concentration on oxidation percentage and oxidation rate were studied. As revealed by ANOVA, the D-fructose and NaOH concentrations significantly affected the oxidation percentage, and the applied voltage and NaOH concentration significantly affected the oxidation rate. Functional models for the oxidation percentage and oxidation rate were generated and reported. The electrochemical oxidation of D-fructose was optimised by maximising the D-fructose concentration and minimising the applied voltage and NaOH concentration. The models were validated by comparing the adjusted optimised solution with the experimental data. A 62.78% electrochemical oxidation percentage and an oxidation rate of 12.20 mM/L h were achieved using 82% D-fructose with 0.14 M NaOH and a 10 V applied voltage. 2014 Journal Article http://hdl.handle.net/20.500.11937/9420 10.1080/19443994.2014.880380 Taylor & Francis Ltd. restricted
spellingShingle Box–Behnken
Electrochemical oxidation
Wastewater treatment
D-fructose
Optimisation
Modelling
Tay, Chen Lim
Fam, S.L.
Electrochemical oxidation of D-fructose solution using the Box–Behnken design methodology
title Electrochemical oxidation of D-fructose solution using the Box–Behnken design methodology
title_full Electrochemical oxidation of D-fructose solution using the Box–Behnken design methodology
title_fullStr Electrochemical oxidation of D-fructose solution using the Box–Behnken design methodology
title_full_unstemmed Electrochemical oxidation of D-fructose solution using the Box–Behnken design methodology
title_short Electrochemical oxidation of D-fructose solution using the Box–Behnken design methodology
title_sort electrochemical oxidation of d-fructose solution using the box–behnken design methodology
topic Box–Behnken
Electrochemical oxidation
Wastewater treatment
D-fructose
Optimisation
Modelling
url http://hdl.handle.net/20.500.11937/9420