Photocatalytic study of two-dimensional ZnO nanopellets in the decomposition of methylene blue

We report several significant photodecomposition rates of methylene blue (MB) obtained before and after the refluxing process of own-synthesized two-dimensional (2D) zinc oxide (ZnO) nanopellets. Each photodecomposition rate of MB was found highly dependent on the weight of photocatalyst. The existi...

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Main Authors: Chiu, Wee Siong, Khiew, Poi Sim, Cloke, Michael, Isa, Dino, Tan, Thian Khoon, Radiman, Shahidan, Abd Shukor, Roslan, Abdul Hamid, Muhammad Azmi, Huang, Nay Ming, Lim, Hong Ngee, Chia, Chin Hua
Format: Article
Language:English
Published: Elsevier 2010
Online Access:http://psasir.upm.edu.my/id/eprint/25158/
http://psasir.upm.edu.my/id/eprint/25158/
http://psasir.upm.edu.my/id/eprint/25158/1/Photocatalytic%20study%20of%20two.pdf
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spelling upm-251582016-03-03T13:12:24Z http://psasir.upm.edu.my/id/eprint/25158/ Photocatalytic study of two-dimensional ZnO nanopellets in the decomposition of methylene blue Chiu, Wee Siong Khiew, Poi Sim Cloke, Michael Isa, Dino Tan, Thian Khoon Radiman, Shahidan Abd Shukor, Roslan Abdul Hamid, Muhammad Azmi Huang, Nay Ming Lim, Hong Ngee Chia, Chin Hua We report several significant photodecomposition rates of methylene blue (MB) obtained before and after the refluxing process of own-synthesized two-dimensional (2D) zinc oxide (ZnO) nanopellets. Each photodecomposition rate of MB was found highly dependent on the weight of photocatalyst. The existing photodecomposition rate has been successfully improved to a factor of 22.0 times through refluxing process in excessive pyridine where the surface capping ligand (oleic acid) is removed from the 2D ZnO nanopellets. On the other hand, the refluxed photocatalyst (0.04 g) in this study was found to exhibit excellent recyclability up to three cycles. Furthermore, X-ray powder diffraction spectrums for the refluxed photocatatalyst, respectively, before and after three cycles of photocatalytic reactions, has generated the same patterns showing that the photocatalyst is stable and feasible to be used as an efficient photocatalyst material. Hence, these 2D ZnO nanopellets would provide a new alternative route as a highly efficient photocatalyst for wastewater treatment. Elsevier 2010-04-01 Article PeerReviewed application/pdf en http://psasir.upm.edu.my/id/eprint/25158/1/Photocatalytic%20study%20of%20two.pdf Chiu, Wee Siong and Khiew, Poi Sim and Cloke, Michael and Isa, Dino and Tan, Thian Khoon and Radiman, Shahidan and Abd Shukor, Roslan and Abdul Hamid, Muhammad Azmi and Huang, Nay Ming and Lim, Hong Ngee and Chia, Chin Hua (2010) Photocatalytic study of two-dimensional ZnO nanopellets in the decomposition of methylene blue. Chemical Engineering Journal, 158 (2). pp. 345-352. ISSN 1385-8947; ESSN: 1873-3212 10.1016/j.cej.2010.01.052
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description We report several significant photodecomposition rates of methylene blue (MB) obtained before and after the refluxing process of own-synthesized two-dimensional (2D) zinc oxide (ZnO) nanopellets. Each photodecomposition rate of MB was found highly dependent on the weight of photocatalyst. The existing photodecomposition rate has been successfully improved to a factor of 22.0 times through refluxing process in excessive pyridine where the surface capping ligand (oleic acid) is removed from the 2D ZnO nanopellets. On the other hand, the refluxed photocatalyst (0.04 g) in this study was found to exhibit excellent recyclability up to three cycles. Furthermore, X-ray powder diffraction spectrums for the refluxed photocatatalyst, respectively, before and after three cycles of photocatalytic reactions, has generated the same patterns showing that the photocatalyst is stable and feasible to be used as an efficient photocatalyst material. Hence, these 2D ZnO nanopellets would provide a new alternative route as a highly efficient photocatalyst for wastewater treatment.
format Article
author Chiu, Wee Siong
Khiew, Poi Sim
Cloke, Michael
Isa, Dino
Tan, Thian Khoon
Radiman, Shahidan
Abd Shukor, Roslan
Abdul Hamid, Muhammad Azmi
Huang, Nay Ming
Lim, Hong Ngee
Chia, Chin Hua
spellingShingle Chiu, Wee Siong
Khiew, Poi Sim
Cloke, Michael
Isa, Dino
Tan, Thian Khoon
Radiman, Shahidan
Abd Shukor, Roslan
Abdul Hamid, Muhammad Azmi
Huang, Nay Ming
Lim, Hong Ngee
Chia, Chin Hua
Photocatalytic study of two-dimensional ZnO nanopellets in the decomposition of methylene blue
author_facet Chiu, Wee Siong
Khiew, Poi Sim
Cloke, Michael
Isa, Dino
Tan, Thian Khoon
Radiman, Shahidan
Abd Shukor, Roslan
Abdul Hamid, Muhammad Azmi
Huang, Nay Ming
Lim, Hong Ngee
Chia, Chin Hua
author_sort Chiu, Wee Siong
title Photocatalytic study of two-dimensional ZnO nanopellets in the decomposition of methylene blue
title_short Photocatalytic study of two-dimensional ZnO nanopellets in the decomposition of methylene blue
title_full Photocatalytic study of two-dimensional ZnO nanopellets in the decomposition of methylene blue
title_fullStr Photocatalytic study of two-dimensional ZnO nanopellets in the decomposition of methylene blue
title_full_unstemmed Photocatalytic study of two-dimensional ZnO nanopellets in the decomposition of methylene blue
title_sort photocatalytic study of two-dimensional zno nanopellets in the decomposition of methylene blue
publisher Elsevier
publishDate 2010
url http://psasir.upm.edu.my/id/eprint/25158/
http://psasir.upm.edu.my/id/eprint/25158/
http://psasir.upm.edu.my/id/eprint/25158/1/Photocatalytic%20study%20of%20two.pdf
first_indexed 2018-09-07T14:55:03Z
last_indexed 2018-09-07T14:55:03Z
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