Selective interlayer ferromagnetic coupling between the Cu spins in YBa2Cu3O7−x grown on top of La0.7Ca0.3MnO3

Studies to date on ferromagnet/d-wave superconductor heterostructures focus mainly on the effects at or near the interfaces while the response of bulk properties to heterostructuring is overlooked. Here we use resonant soft x-ray scattering spectroscopy to reveal a novel c-axis ferromagnetic couplin...

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Main Authors: Huang, S. W., Wray, L. Andrew, Jeng, Horng-Tay, Tra, V. T., Lee, J. M., Langner, M. C., Chen, J. M., Roy, S., Chu, Y. H., Schoenlein, R. W., Chuang, Y.-D., Lin, J.-Y.
Format: Online
Language:English
Published: Nature Publishing Group 2015
Online Access:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC4648077/
id pubmed-4648077
recordtype oai_dc
spelling pubmed-46480772015-11-23 Selective interlayer ferromagnetic coupling between the Cu spins in YBa2Cu3O7−x grown on top of La0.7Ca0.3MnO3 Huang, S. W. Wray, L. Andrew Jeng, Horng-Tay Tra, V. T. Lee, J. M. Langner, M. C. Chen, J. M. Roy, S. Chu, Y. H. Schoenlein, R. W. Chuang, Y.-D. Lin, J.-Y. Article Studies to date on ferromagnet/d-wave superconductor heterostructures focus mainly on the effects at or near the interfaces while the response of bulk properties to heterostructuring is overlooked. Here we use resonant soft x-ray scattering spectroscopy to reveal a novel c-axis ferromagnetic coupling between the in-plane Cu spins in YBa2Cu3O7−x (YBCO) superconductor when it is grown on top of ferromagnetic La0.7Ca0.3MnO3 (LCMO) manganite layer. This coupling, present in both normal and superconducting states of YBCO, is sensitive to the interfacial termination such that it is only observed in bilayers with MnO2 but not with La0.7Ca0.3O interfacial termination. Such contrasting behaviors, we propose, are due to distinct energetic of CuO chain and CuO2 plane at the La0.7Ca0.3O and MnO2 terminated interfaces respectively, therefore influencing the transfer of spin-polarized electrons from manganite to cuprate differently. Our findings suggest that the superconducting/ferromagnetic bilayers with proper interfacial engineering can be good candidates for searching the theorized Fulde-Ferrel-Larkin-Ovchinnikov (FFLO) state in cuprates and studying the competing quantum orders in highly correlated electron systems. Nature Publishing Group 2015-11-17 /pmc/articles/PMC4648077/ /pubmed/26573394 http://dx.doi.org/10.1038/srep16690 Text en Copyright © 2015, Macmillan Publishers Limited http://creativecommons.org/licenses/by/4.0/ This work is licensed under a Creative Commons Attribution 4.0 International License. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in the credit line; if the material is not included under the Creative Commons license, users will need to obtain permission from the license holder to reproduce the material. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/
repository_type Open Access Journal
institution_category Foreign Institution
institution US National Center for Biotechnology Information
building NCBI PubMed
collection Online Access
language English
format Online
author Huang, S. W.
Wray, L. Andrew
Jeng, Horng-Tay
Tra, V. T.
Lee, J. M.
Langner, M. C.
Chen, J. M.
Roy, S.
Chu, Y. H.
Schoenlein, R. W.
Chuang, Y.-D.
Lin, J.-Y.
spellingShingle Huang, S. W.
Wray, L. Andrew
Jeng, Horng-Tay
Tra, V. T.
Lee, J. M.
Langner, M. C.
Chen, J. M.
Roy, S.
Chu, Y. H.
Schoenlein, R. W.
Chuang, Y.-D.
Lin, J.-Y.
Selective interlayer ferromagnetic coupling between the Cu spins in YBa2Cu3O7−x grown on top of La0.7Ca0.3MnO3
author_facet Huang, S. W.
Wray, L. Andrew
Jeng, Horng-Tay
Tra, V. T.
Lee, J. M.
Langner, M. C.
Chen, J. M.
Roy, S.
Chu, Y. H.
Schoenlein, R. W.
Chuang, Y.-D.
Lin, J.-Y.
author_sort Huang, S. W.
title Selective interlayer ferromagnetic coupling between the Cu spins in YBa2Cu3O7−x grown on top of La0.7Ca0.3MnO3
title_short Selective interlayer ferromagnetic coupling between the Cu spins in YBa2Cu3O7−x grown on top of La0.7Ca0.3MnO3
title_full Selective interlayer ferromagnetic coupling between the Cu spins in YBa2Cu3O7−x grown on top of La0.7Ca0.3MnO3
title_fullStr Selective interlayer ferromagnetic coupling between the Cu spins in YBa2Cu3O7−x grown on top of La0.7Ca0.3MnO3
title_full_unstemmed Selective interlayer ferromagnetic coupling between the Cu spins in YBa2Cu3O7−x grown on top of La0.7Ca0.3MnO3
title_sort selective interlayer ferromagnetic coupling between the cu spins in yba2cu3o7−x grown on top of la0.7ca0.3mno3
description Studies to date on ferromagnet/d-wave superconductor heterostructures focus mainly on the effects at or near the interfaces while the response of bulk properties to heterostructuring is overlooked. Here we use resonant soft x-ray scattering spectroscopy to reveal a novel c-axis ferromagnetic coupling between the in-plane Cu spins in YBa2Cu3O7−x (YBCO) superconductor when it is grown on top of ferromagnetic La0.7Ca0.3MnO3 (LCMO) manganite layer. This coupling, present in both normal and superconducting states of YBCO, is sensitive to the interfacial termination such that it is only observed in bilayers with MnO2 but not with La0.7Ca0.3O interfacial termination. Such contrasting behaviors, we propose, are due to distinct energetic of CuO chain and CuO2 plane at the La0.7Ca0.3O and MnO2 terminated interfaces respectively, therefore influencing the transfer of spin-polarized electrons from manganite to cuprate differently. Our findings suggest that the superconducting/ferromagnetic bilayers with proper interfacial engineering can be good candidates for searching the theorized Fulde-Ferrel-Larkin-Ovchinnikov (FFLO) state in cuprates and studying the competing quantum orders in highly correlated electron systems.
publisher Nature Publishing Group
publishDate 2015
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC4648077/
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