Coherence in the presence of absorption and heating in a molecule interferometer

Matter-wave interferometry can be used to probe the foundations of physics and to enable precise measurements of particle properties and fundamental constants. It relies on beam splitters that coherently divide the wave function. In atom interferometers, such elements are often realised using lasers...

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Main Authors: Cotter, J. P., Eibenberger, S., Mairhofer, L., Cheng, X., Asenbaum, P., Arndt, M., Walter, K., Nimmrichter, S., Hornberger, K.
Format: Online
Language:English
Published: Nature Pub. Group 2015
Online Access:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC4477035/
id pubmed-4477035
recordtype oai_dc
spelling pubmed-44770352015-07-13 Coherence in the presence of absorption and heating in a molecule interferometer Cotter, J. P. Eibenberger, S. Mairhofer, L. Cheng, X. Asenbaum, P. Arndt, M. Walter, K. Nimmrichter, S. Hornberger, K. Article Matter-wave interferometry can be used to probe the foundations of physics and to enable precise measurements of particle properties and fundamental constants. It relies on beam splitters that coherently divide the wave function. In atom interferometers, such elements are often realised using lasers by exploiting the dipole interaction or through photon absorption. It is intriguing to extend these ideas to complex molecules where the energy of an absorbed photon can rapidly be redistributed across many internal degrees of freedom. Here, we provide evidence that center-of-mass coherence can be maintained even when the internal energy and entropy of the interfering particle are substantially increased by absorption of photons from a standing light wave. Each photon correlates the molecular center-of-mass wave function with its internal temperature and splits it into a superposition with opposite momenta in addition to the beam-splitting action of the optical dipole potential. Nature Pub. Group 2015-06-11 /pmc/articles/PMC4477035/ /pubmed/26066053 http://dx.doi.org/10.1038/ncomms8336 Text en Copyright © 2015, Nature Publishing Group, a division of Macmillan Publishers Limited. All Rights Reserved. http://creativecommons.org/licenses/by/4.0/ This work is licensed under a Creative Commons Attribution 4.0 International License. The images or other third party material in this article are included in the article's Creative Commons license, unless indicated otherwise in the credit line; if the material is not included under the Creative Commons license, users will need to obtain permission from the license holder to reproduce the material. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/
repository_type Open Access Journal
institution_category Foreign Institution
institution US National Center for Biotechnology Information
building NCBI PubMed
collection Online Access
language English
format Online
author Cotter, J. P.
Eibenberger, S.
Mairhofer, L.
Cheng, X.
Asenbaum, P.
Arndt, M.
Walter, K.
Nimmrichter, S.
Hornberger, K.
spellingShingle Cotter, J. P.
Eibenberger, S.
Mairhofer, L.
Cheng, X.
Asenbaum, P.
Arndt, M.
Walter, K.
Nimmrichter, S.
Hornberger, K.
Coherence in the presence of absorption and heating in a molecule interferometer
author_facet Cotter, J. P.
Eibenberger, S.
Mairhofer, L.
Cheng, X.
Asenbaum, P.
Arndt, M.
Walter, K.
Nimmrichter, S.
Hornberger, K.
author_sort Cotter, J. P.
title Coherence in the presence of absorption and heating in a molecule interferometer
title_short Coherence in the presence of absorption and heating in a molecule interferometer
title_full Coherence in the presence of absorption and heating in a molecule interferometer
title_fullStr Coherence in the presence of absorption and heating in a molecule interferometer
title_full_unstemmed Coherence in the presence of absorption and heating in a molecule interferometer
title_sort coherence in the presence of absorption and heating in a molecule interferometer
description Matter-wave interferometry can be used to probe the foundations of physics and to enable precise measurements of particle properties and fundamental constants. It relies on beam splitters that coherently divide the wave function. In atom interferometers, such elements are often realised using lasers by exploiting the dipole interaction or through photon absorption. It is intriguing to extend these ideas to complex molecules where the energy of an absorbed photon can rapidly be redistributed across many internal degrees of freedom. Here, we provide evidence that center-of-mass coherence can be maintained even when the internal energy and entropy of the interfering particle are substantially increased by absorption of photons from a standing light wave. Each photon correlates the molecular center-of-mass wave function with its internal temperature and splits it into a superposition with opposite momenta in addition to the beam-splitting action of the optical dipole potential.
publisher Nature Pub. Group
publishDate 2015
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC4477035/
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