Effects of phase inversion and rheological factors on formation of defect-free and ultrathin-skinned asymmetric polysulfone membranes for gas separation

Development of defect-free and ultrathin-skinned asymmetric membranes for gas separation process without requiring any additional post-treatments such as curing or coating is a major breakthrough in membrane technology. Correlation of primary dry/wet phase inversion process with rheology aspects is...

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Main Authors: Ismail, A. F., Lai, P. Y.
Format: Article
Published: Elsevier 2003
Subjects:
Online Access:http://eprints.utm.my/773/
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author Ismail, A. F.
Lai, P. Y.
author_facet Ismail, A. F.
Lai, P. Y.
author_sort Ismail, A. F.
building UTeM Institutional Repository
collection Online Access
description Development of defect-free and ultrathin-skinned asymmetric membranes for gas separation process without requiring any additional post-treatments such as curing or coating is a major breakthrough in membrane technology. Correlation of primary dry/wet phase inversion process with rheology aspects is a novel approach in membrane research that provides a potential platform to improve membrane performance. The former controls general morphology of membrane, whereas the latter further affects molecular orientation in membrane. Casting solution developed in this study consisted of polysulfone, tetrahydrofuran (THF), N,N-dimethylacetamide (DMAc) and ethanol (EtOH). The produced membranes were tested with hydrogen and nitrogen as test gases. Essentially defect-free and ultrathin skin layer was achieved for asymmetric polysulfone membranes. Selectivity of these membranes was relatively higher compared to conventional membranes, some of them even surpassed the intrinsic selectivity.
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spelling utm-7732010-10-26T08:28:30Z http://eprints.utm.my/773/ Effects of phase inversion and rheological factors on formation of defect-free and ultrathin-skinned asymmetric polysulfone membranes for gas separation Ismail, A. F. Lai, P. Y. TP Chemical technology Development of defect-free and ultrathin-skinned asymmetric membranes for gas separation process without requiring any additional post-treatments such as curing or coating is a major breakthrough in membrane technology. Correlation of primary dry/wet phase inversion process with rheology aspects is a novel approach in membrane research that provides a potential platform to improve membrane performance. The former controls general morphology of membrane, whereas the latter further affects molecular orientation in membrane. Casting solution developed in this study consisted of polysulfone, tetrahydrofuran (THF), N,N-dimethylacetamide (DMAc) and ethanol (EtOH). The produced membranes were tested with hydrogen and nitrogen as test gases. Essentially defect-free and ultrathin skin layer was achieved for asymmetric polysulfone membranes. Selectivity of these membranes was relatively higher compared to conventional membranes, some of them even surpassed the intrinsic selectivity. Elsevier 2003-10 Article PeerReviewed Ismail, A. F. and Lai, P. Y. (2003) Effects of phase inversion and rheological factors on formation of defect-free and ultrathin-skinned asymmetric polysulfone membranes for gas separation. Separation and Purification Technology, 33 (2). pp. 127-143. ISSN 1383-5866 http://dx.doi.org/10.1016/S1383-5866(02)00201-0 doi:10.1016/S1383-5866(02)00201-0
spellingShingle TP Chemical technology
Ismail, A. F.
Lai, P. Y.
Effects of phase inversion and rheological factors on formation of defect-free and ultrathin-skinned asymmetric polysulfone membranes for gas separation
title Effects of phase inversion and rheological factors on formation of defect-free and ultrathin-skinned asymmetric polysulfone membranes for gas separation
title_full Effects of phase inversion and rheological factors on formation of defect-free and ultrathin-skinned asymmetric polysulfone membranes for gas separation
title_fullStr Effects of phase inversion and rheological factors on formation of defect-free and ultrathin-skinned asymmetric polysulfone membranes for gas separation
title_full_unstemmed Effects of phase inversion and rheological factors on formation of defect-free and ultrathin-skinned asymmetric polysulfone membranes for gas separation
title_short Effects of phase inversion and rheological factors on formation of defect-free and ultrathin-skinned asymmetric polysulfone membranes for gas separation
title_sort effects of phase inversion and rheological factors on formation of defect-free and ultrathin-skinned asymmetric polysulfone membranes for gas separation
topic TP Chemical technology
url http://eprints.utm.my/773/
http://eprints.utm.my/773/
http://eprints.utm.my/773/