Morphological and mechanical properties of rubber-toughened polyamide 6/ polypropylene nanocomposites prepared by different methods of compounding

The nanocomposites based on polyamide 6/polypropylene blends (PA6/PP), polypropylene grafted with maleic anhydride (PPgMAH), ethylene octene copolymer (POE), and organically modified montmorillonite (organoclay) are prepared through different mixing sequences of melt intercalation technique. The pro...

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Main Authors: Wahit, Mat Uzir, Hassan, Azman, Rahmat, Abd Razak, Mohd Ishak, Zarifin Ariffin
Format: Article
Published: Sage Publication 2006
Subjects:
Online Access:http://eprints.utm.my/7440/
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author Wahit, Mat Uzir
Hassan, Azman
Rahmat, Abd Razak
Mohd Ishak, Zarifin Ariffin
author_facet Wahit, Mat Uzir
Hassan, Azman
Rahmat, Abd Razak
Mohd Ishak, Zarifin Ariffin
author_sort Wahit, Mat Uzir
building UTeM Institutional Repository
collection Online Access
description The nanocomposites based on polyamide 6/polypropylene blends (PA6/PP), polypropylene grafted with maleic anhydride (PPgMAH), ethylene octene copolymer (POE), and organically modified montmorillonite (organoclay) are prepared through different mixing sequences of melt intercalation technique. The processes used are: (1) direct melt intercalation single extrusion process (SD), (2) two times direct melt intercalation (S2x), (3) two steps melt intercalation i.e., mixing of preblend PA6/organoclay with preblend PP/PPgMAH/POE (S2sa), and (4) two steps melt intercalation i.e., mixing of preblend PA6/PP/PPgMAH/organoclay with POE (S2sb). The effect of various processing techniques on the structural, morphological, and mechanical properties of nanocomposites is characterized by X-ray diffraction (XRD), scanning electron microscope (SEM), tensile, flexural, and Izod impact testing. The results show that all the methods give generally exfoliated structures based on XRD. It is also found that the melt intercalation technique significantly influences the dispersion behavior of POE in the PA6/PP matrix and thus the impact properties. However, no significant blending sequence effect is found for tensile and flexural properties of nanocomposites. Overall, the method S2sa gives the best mechanical properties due to its good dispersion of organoclays and elastomer in the continuous PA6/PP matrix.
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spelling utm-74402009-01-05T03:14:41Z http://eprints.utm.my/7440/ Morphological and mechanical properties of rubber-toughened polyamide 6/ polypropylene nanocomposites prepared by different methods of compounding Wahit, Mat Uzir Hassan, Azman Rahmat, Abd Razak Mohd Ishak, Zarifin Ariffin TP Chemical technology The nanocomposites based on polyamide 6/polypropylene blends (PA6/PP), polypropylene grafted with maleic anhydride (PPgMAH), ethylene octene copolymer (POE), and organically modified montmorillonite (organoclay) are prepared through different mixing sequences of melt intercalation technique. The processes used are: (1) direct melt intercalation single extrusion process (SD), (2) two times direct melt intercalation (S2x), (3) two steps melt intercalation i.e., mixing of preblend PA6/organoclay with preblend PP/PPgMAH/POE (S2sa), and (4) two steps melt intercalation i.e., mixing of preblend PA6/PP/PPgMAH/organoclay with POE (S2sb). The effect of various processing techniques on the structural, morphological, and mechanical properties of nanocomposites is characterized by X-ray diffraction (XRD), scanning electron microscope (SEM), tensile, flexural, and Izod impact testing. The results show that all the methods give generally exfoliated structures based on XRD. It is also found that the melt intercalation technique significantly influences the dispersion behavior of POE in the PA6/PP matrix and thus the impact properties. However, no significant blending sequence effect is found for tensile and flexural properties of nanocomposites. Overall, the method S2sa gives the best mechanical properties due to its good dispersion of organoclays and elastomer in the continuous PA6/PP matrix. Sage Publication 2006-07 Article PeerReviewed Wahit, Mat Uzir and Hassan, Azman and Rahmat, Abd Razak and Mohd Ishak, Zarifin Ariffin (2006) Morphological and mechanical properties of rubber-toughened polyamide 6/ polypropylene nanocomposites prepared by different methods of compounding. Journal of Elastomers and Plastics, 38 (3). pp. 231-247. http://dx.doi.org/10.1177/0095244306063852 10.1177/0095244306063852
spellingShingle TP Chemical technology
Wahit, Mat Uzir
Hassan, Azman
Rahmat, Abd Razak
Mohd Ishak, Zarifin Ariffin
Morphological and mechanical properties of rubber-toughened polyamide 6/ polypropylene nanocomposites prepared by different methods of compounding
title Morphological and mechanical properties of rubber-toughened polyamide 6/ polypropylene nanocomposites prepared by different methods of compounding
title_full Morphological and mechanical properties of rubber-toughened polyamide 6/ polypropylene nanocomposites prepared by different methods of compounding
title_fullStr Morphological and mechanical properties of rubber-toughened polyamide 6/ polypropylene nanocomposites prepared by different methods of compounding
title_full_unstemmed Morphological and mechanical properties of rubber-toughened polyamide 6/ polypropylene nanocomposites prepared by different methods of compounding
title_short Morphological and mechanical properties of rubber-toughened polyamide 6/ polypropylene nanocomposites prepared by different methods of compounding
title_sort morphological and mechanical properties of rubber-toughened polyamide 6/ polypropylene nanocomposites prepared by different methods of compounding
topic TP Chemical technology
url http://eprints.utm.my/7440/
http://eprints.utm.my/7440/
http://eprints.utm.my/7440/