Capability Of Adsorptive Expoxified Poly(Ethersulfone) Membrane To Separate Chromium Ions

A microporous epoxy resin epoxified-polyethersulfone (EPES) blend membrane (EPES membrane) was prepared through dry-wet phase inversion. This study attempts to correlate the changes in membrane physical and chemical properties when different composition (30wt%, 50wt%, 70wt% and 90wt %) of bisphenol...

Full description

Bibliographic Details
Main Author: Tan, Ying Shien
Format: Monograph
Language:English
Published: Universiti Sains Malaysia 2017
Subjects:
Online Access:http://eprints.usm.my/53138/
http://eprints.usm.my/53138/1/Capability%20Of%20Adsorptive%20Expoxified%20Poly%28Ethersulfone%29%20Membrane%20To%20Separate%20Chromium%20Ions_Tan%20Ying%20Shien_K4_2017.pdf
_version_ 1848882443192369152
author Tan, Ying Shien
author_facet Tan, Ying Shien
author_sort Tan, Ying Shien
building USM Institutional Repository
collection Online Access
description A microporous epoxy resin epoxified-polyethersulfone (EPES) blend membrane (EPES membrane) was prepared through dry-wet phase inversion. This study attempts to correlate the changes in membrane physical and chemical properties when different composition (30wt%, 50wt%, 70wt% and 90wt %) of bisphenol A diglycidyl ether (BADGE) were added into the PES membrane. The synthesised membrane was used to separate the carcinogen chromium (VI). Analysis from fourier transform infrared spectroscopy (FTIR) has proved the present of the epoxy peak which indicated the successful integration of the epoxy resin into the polymer matrix. Scanning electron microscopy (SEM) showed the finger-like pore structure in neat PES and sponge structure pore in EPES membrane. Also, the macrovoid became more significant as the composition of BADGE increases. Moreover, the viscosity of the dope solution of each formula were found lower when more BADGE added which explain the phenomenon observe in SEM as viscosity will affect the rate of diffusion of NMP solvent during phase inversion. The lower viscosity allow the rate of diffusion higher and thus increased the macrovoid phenomenon. As the performances of the membranes, permeate flux increased with reduction of fouling when composition of BADGE was increased. 30wt% of BADGE/PES membrane show highest rejection of Cr (VI) ions at 83.734% with permeated flux of 1.52 L/m2.min. In this work, another type of epoxy resin- Glycidyl methacrylate (GMA) was also used as the additive and compare the performance with BADGE/PES membrane. The GMA-PES membrane demonstrated very high initial flux of 89.312 L/m2.min but very low rejection at 19.067%. Through FTIR analysis, GMA peak was failed to appear, indicated most of the epoxy resin was fluxed out during the membrane synthesis. It was due to the high solubility of GMA in water as compared to BADGE.
first_indexed 2025-11-15T18:35:00Z
format Monograph
id usm-53138
institution Universiti Sains Malaysia
institution_category Local University
language English
last_indexed 2025-11-15T18:35:00Z
publishDate 2017
publisher Universiti Sains Malaysia
recordtype eprints
repository_type Digital Repository
spelling usm-531382022-06-27T10:25:40Z http://eprints.usm.my/53138/ Capability Of Adsorptive Expoxified Poly(Ethersulfone) Membrane To Separate Chromium Ions Tan, Ying Shien T Technology TP155-156 Chemical engineering A microporous epoxy resin epoxified-polyethersulfone (EPES) blend membrane (EPES membrane) was prepared through dry-wet phase inversion. This study attempts to correlate the changes in membrane physical and chemical properties when different composition (30wt%, 50wt%, 70wt% and 90wt %) of bisphenol A diglycidyl ether (BADGE) were added into the PES membrane. The synthesised membrane was used to separate the carcinogen chromium (VI). Analysis from fourier transform infrared spectroscopy (FTIR) has proved the present of the epoxy peak which indicated the successful integration of the epoxy resin into the polymer matrix. Scanning electron microscopy (SEM) showed the finger-like pore structure in neat PES and sponge structure pore in EPES membrane. Also, the macrovoid became more significant as the composition of BADGE increases. Moreover, the viscosity of the dope solution of each formula were found lower when more BADGE added which explain the phenomenon observe in SEM as viscosity will affect the rate of diffusion of NMP solvent during phase inversion. The lower viscosity allow the rate of diffusion higher and thus increased the macrovoid phenomenon. As the performances of the membranes, permeate flux increased with reduction of fouling when composition of BADGE was increased. 30wt% of BADGE/PES membrane show highest rejection of Cr (VI) ions at 83.734% with permeated flux of 1.52 L/m2.min. In this work, another type of epoxy resin- Glycidyl methacrylate (GMA) was also used as the additive and compare the performance with BADGE/PES membrane. The GMA-PES membrane demonstrated very high initial flux of 89.312 L/m2.min but very low rejection at 19.067%. Through FTIR analysis, GMA peak was failed to appear, indicated most of the epoxy resin was fluxed out during the membrane synthesis. It was due to the high solubility of GMA in water as compared to BADGE. Universiti Sains Malaysia 2017-05-01 Monograph NonPeerReviewed application/pdf en http://eprints.usm.my/53138/1/Capability%20Of%20Adsorptive%20Expoxified%20Poly%28Ethersulfone%29%20Membrane%20To%20Separate%20Chromium%20Ions_Tan%20Ying%20Shien_K4_2017.pdf Tan, Ying Shien (2017) Capability Of Adsorptive Expoxified Poly(Ethersulfone) Membrane To Separate Chromium Ions. Project Report. Universiti Sains Malaysia, Pusat Pengajian Kejuruteraan Kimia. (Submitted)
spellingShingle T Technology
TP155-156 Chemical engineering
Tan, Ying Shien
Capability Of Adsorptive Expoxified Poly(Ethersulfone) Membrane To Separate Chromium Ions
title Capability Of Adsorptive Expoxified Poly(Ethersulfone) Membrane To Separate Chromium Ions
title_full Capability Of Adsorptive Expoxified Poly(Ethersulfone) Membrane To Separate Chromium Ions
title_fullStr Capability Of Adsorptive Expoxified Poly(Ethersulfone) Membrane To Separate Chromium Ions
title_full_unstemmed Capability Of Adsorptive Expoxified Poly(Ethersulfone) Membrane To Separate Chromium Ions
title_short Capability Of Adsorptive Expoxified Poly(Ethersulfone) Membrane To Separate Chromium Ions
title_sort capability of adsorptive expoxified poly(ethersulfone) membrane to separate chromium ions
topic T Technology
TP155-156 Chemical engineering
url http://eprints.usm.my/53138/
http://eprints.usm.my/53138/1/Capability%20Of%20Adsorptive%20Expoxified%20Poly%28Ethersulfone%29%20Membrane%20To%20Separate%20Chromium%20Ions_Tan%20Ying%20Shien_K4_2017.pdf