Activated Rice Husk-Based Adsorbents For Chlorophenol Removal And Their Bioregeneration

The objectives of this study are to develop rice husk-based adsorbents activated with different activating agents, namely potassium hydroxide (KRH), nitric acid and methanol (ARH), and ethylenediamine (MRH), and compare their adsorption capacities and bioregeneration efficiencies to remove 4-c...

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Main Author: Khor, Siok Moi
Format: Thesis
Language:English
Published: 2013
Subjects:
Online Access:http://eprints.usm.my/43534/
http://eprints.usm.my/43534/1/Khor%20Siok%20Moi24.pdf
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author Khor, Siok Moi
author_facet Khor, Siok Moi
author_sort Khor, Siok Moi
building USM Institutional Repository
collection Online Access
description The objectives of this study are to develop rice husk-based adsorbents activated with different activating agents, namely potassium hydroxide (KRH), nitric acid and methanol (ARH), and ethylenediamine (MRH), and compare their adsorption capacities and bioregeneration efficiencies to remove 4-chlorophenol (4- CP) and 2,4-dichlorophenol (2,4-DCP) from the aqueous solutions with the commercially available powdered activated carbon (PAC). From the adsorption equilibrium studies of 4-CP and 2,4-DCP, the trend of maximum adsorption capacity, qm, among the adsorbents followed KRH > PAC > ARH > MRH and in agreement with the trend of BET surface areas. The equilibrium adsorption data of KRH and PAC were best described by the Langmuir model (R2 > 0.98) while the Freundlich model was suitable to describe the equilibrium adsorption data for MRH and ARH (R2 > 0.99). These observations were confirmed by the values of heterogeneity constant, μ, obtained from the Redlich-Peterson model. It could be concluded that the adsorbent surfaces of MRH and ARH were heterogeneous, while those of the KRH and PAC were homogenous. For the temperature-dependent Temkin and Dubinin-Radushkevich isotherm models, the Dubinin-Radushkevich model was better fitted to the experimental data than the Temkin model.
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spelling usm-435342019-04-12T05:26:16Z http://eprints.usm.my/43534/ Activated Rice Husk-Based Adsorbents For Chlorophenol Removal And Their Bioregeneration Khor, Siok Moi QD1-999 Chemistry The objectives of this study are to develop rice husk-based adsorbents activated with different activating agents, namely potassium hydroxide (KRH), nitric acid and methanol (ARH), and ethylenediamine (MRH), and compare their adsorption capacities and bioregeneration efficiencies to remove 4-chlorophenol (4- CP) and 2,4-dichlorophenol (2,4-DCP) from the aqueous solutions with the commercially available powdered activated carbon (PAC). From the adsorption equilibrium studies of 4-CP and 2,4-DCP, the trend of maximum adsorption capacity, qm, among the adsorbents followed KRH > PAC > ARH > MRH and in agreement with the trend of BET surface areas. The equilibrium adsorption data of KRH and PAC were best described by the Langmuir model (R2 > 0.98) while the Freundlich model was suitable to describe the equilibrium adsorption data for MRH and ARH (R2 > 0.99). These observations were confirmed by the values of heterogeneity constant, μ, obtained from the Redlich-Peterson model. It could be concluded that the adsorbent surfaces of MRH and ARH were heterogeneous, while those of the KRH and PAC were homogenous. For the temperature-dependent Temkin and Dubinin-Radushkevich isotherm models, the Dubinin-Radushkevich model was better fitted to the experimental data than the Temkin model. 2013-05 Thesis NonPeerReviewed application/pdf en http://eprints.usm.my/43534/1/Khor%20Siok%20Moi24.pdf Khor, Siok Moi (2013) Activated Rice Husk-Based Adsorbents For Chlorophenol Removal And Their Bioregeneration. PhD thesis, Universiti Sains Malaysia.
spellingShingle QD1-999 Chemistry
Khor, Siok Moi
Activated Rice Husk-Based Adsorbents For Chlorophenol Removal And Their Bioregeneration
title Activated Rice Husk-Based Adsorbents For Chlorophenol Removal And Their Bioregeneration
title_full Activated Rice Husk-Based Adsorbents For Chlorophenol Removal And Their Bioregeneration
title_fullStr Activated Rice Husk-Based Adsorbents For Chlorophenol Removal And Their Bioregeneration
title_full_unstemmed Activated Rice Husk-Based Adsorbents For Chlorophenol Removal And Their Bioregeneration
title_short Activated Rice Husk-Based Adsorbents For Chlorophenol Removal And Their Bioregeneration
title_sort activated rice husk-based adsorbents for chlorophenol removal and their bioregeneration
topic QD1-999 Chemistry
url http://eprints.usm.my/43534/
http://eprints.usm.my/43534/1/Khor%20Siok%20Moi24.pdf