Synthesis of nano-magnetite from industrial mill chips for the application of boron removal: characterization and adsorption efficacy

The present study synthesized nano-magnetite (Fe3O4) from milled steel chips using the high energy ball milling (HEBM) method, characterized it, and then utilized it as a sorbent to remediate boron concentration at various pH (4–9), dosages (0.1–0.5 g), contact times (20–240 min), and initial concen...

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Main Authors: Abba, Mohammed Umar, Che Man, Hasfalina, Azis, Raba’ah Syahidah, Idris, Aida Isma
Format: Article
Published: MDPI AG 2021
Online Access:http://psasir.upm.edu.my/id/eprint/95270/
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author Abba, Mohammed Umar
Che Man, Hasfalina
Azis, Raba’ah Syahidah
Idris, Aida Isma
author_facet Abba, Mohammed Umar
Che Man, Hasfalina
Azis, Raba’ah Syahidah
Idris, Aida Isma
author_sort Abba, Mohammed Umar
building UPM Institutional Repository
collection Online Access
description The present study synthesized nano-magnetite (Fe3O4) from milled steel chips using the high energy ball milling (HEBM) method, characterized it, and then utilized it as a sorbent to remediate boron concentration at various pH (4–9), dosages (0.1–0.5 g), contact times (20–240 min), and initial concentrations (10–100 mg/L). The nano-sorbents were characterized based on SEM structure, elemental composition (EDX), surface area analysis (BET), crystallinity (XRD), and functional group analysis (FTIR). The highest adsorption capacity of 8.44 mg/g with removal efficiency of 84% was attained at pH 8, 0.5 g dosage, contact time of 180 min, and 50 mg/L initial concentration. The experimental data fit best with the pseudo-second-order kinetic model with R2 of 0.998, while the Freundlich adsorption isotherm describes the adsorption process with an R2 value of 0.9464. A regeneration efficiency of 47% was attained even after five cycles of reusability studies. This efficiency implies that the nano-magnetite has the potential for sustainable industrial application.
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institution Universiti Putra Malaysia
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publishDate 2021
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spelling upm-952702023-01-31T04:14:29Z http://psasir.upm.edu.my/id/eprint/95270/ Synthesis of nano-magnetite from industrial mill chips for the application of boron removal: characterization and adsorption efficacy Abba, Mohammed Umar Che Man, Hasfalina Azis, Raba’ah Syahidah Idris, Aida Isma The present study synthesized nano-magnetite (Fe3O4) from milled steel chips using the high energy ball milling (HEBM) method, characterized it, and then utilized it as a sorbent to remediate boron concentration at various pH (4–9), dosages (0.1–0.5 g), contact times (20–240 min), and initial concentrations (10–100 mg/L). The nano-sorbents were characterized based on SEM structure, elemental composition (EDX), surface area analysis (BET), crystallinity (XRD), and functional group analysis (FTIR). The highest adsorption capacity of 8.44 mg/g with removal efficiency of 84% was attained at pH 8, 0.5 g dosage, contact time of 180 min, and 50 mg/L initial concentration. The experimental data fit best with the pseudo-second-order kinetic model with R2 of 0.998, while the Freundlich adsorption isotherm describes the adsorption process with an R2 value of 0.9464. A regeneration efficiency of 47% was attained even after five cycles of reusability studies. This efficiency implies that the nano-magnetite has the potential for sustainable industrial application. MDPI AG 2021-02-03 Article PeerReviewed Abba, Mohammed Umar and Che Man, Hasfalina and Azis, Raba’ah Syahidah and Idris, Aida Isma (2021) Synthesis of nano-magnetite from industrial mill chips for the application of boron removal: characterization and adsorption efficacy. International Journal of Environmental Research and Public Health, 18 (4). art. no. 1400. pp. 1-18. ISSN 1660-4601 https://www.mdpi.com/1660-4601/18/4/1400 10.3390/ijerph18041400
spellingShingle Abba, Mohammed Umar
Che Man, Hasfalina
Azis, Raba’ah Syahidah
Idris, Aida Isma
Synthesis of nano-magnetite from industrial mill chips for the application of boron removal: characterization and adsorption efficacy
title Synthesis of nano-magnetite from industrial mill chips for the application of boron removal: characterization and adsorption efficacy
title_full Synthesis of nano-magnetite from industrial mill chips for the application of boron removal: characterization and adsorption efficacy
title_fullStr Synthesis of nano-magnetite from industrial mill chips for the application of boron removal: characterization and adsorption efficacy
title_full_unstemmed Synthesis of nano-magnetite from industrial mill chips for the application of boron removal: characterization and adsorption efficacy
title_short Synthesis of nano-magnetite from industrial mill chips for the application of boron removal: characterization and adsorption efficacy
title_sort synthesis of nano-magnetite from industrial mill chips for the application of boron removal: characterization and adsorption efficacy
url http://psasir.upm.edu.my/id/eprint/95270/
http://psasir.upm.edu.my/id/eprint/95270/
http://psasir.upm.edu.my/id/eprint/95270/