Synthesis and characterization of bifunctional magnetic nano-catalyst from rice husk for production of biodiesel

In this work, bifunctional magnetic nano-catalyst was successfully derived from rice husk char doped with potassium oxide and nickel oxide by impregnation techniques, and their catalytic ability was tested via transesterification of used cooking oil (UCO). The catalyst was characterized by thermogra...

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Main Authors: Hazmi, Balkis, Rashid, Umer, Ibrahim, Mohd Lokman, Nehdi, Imededdine Arbi, Azam, Mohammad, Al-Resayes, Saud Ibrahim
Format: Article
Published: Elsevier BV 2021
Online Access:http://psasir.upm.edu.my/id/eprint/95250/
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author Hazmi, Balkis
Rashid, Umer
Ibrahim, Mohd Lokman
Nehdi, Imededdine Arbi
Azam, Mohammad
Al-Resayes, Saud Ibrahim
author_facet Hazmi, Balkis
Rashid, Umer
Ibrahim, Mohd Lokman
Nehdi, Imededdine Arbi
Azam, Mohammad
Al-Resayes, Saud Ibrahim
author_sort Hazmi, Balkis
building UPM Institutional Repository
collection Online Access
description In this work, bifunctional magnetic nano-catalyst was successfully derived from rice husk char doped with potassium oxide and nickel oxide by impregnation techniques, and their catalytic ability was tested via transesterification of used cooking oil (UCO). The catalyst was characterized by thermogravimetric analyzer (TGA), X-ray diffraction spectroscopy (XRD), Fourier-transform infrared spectroscopy (FTIR), Temperature programmed desorption (TPD), Brunauer–Emmett–Teller (BET), Scanning electron microscopy equipped with energy dispersive x-ray analyzer (FESEM-EDX), and Vibrating sampling magnetometer (VSM) for magnetic properties. The optimized nanomagnetic bifunctional catalyst (RHC/K2O-20%/Ni-5%) had 3.014 mmol g-1 & 4.485 mmol g-1 of acidity and basicity, respectively, with the magnetic strength was recorded at 2.312 emu g−1. For the catalytic evaluation, a maximum biodiesel yield of 98.2% was accomplished with 4 wt% of catalyst loading, 12:1 methanol to UCO molar ratio at 65 °C within 2 h of reaction time. The catalyst was reused for up to 5 reaction cycles and producing 70% of biodiesel at the last cycles. The fuel properties of optimized biodiesel were measured using Biodiesel - American Standard Testing Method (ASTM) D6751. Due to the magnetic properties of the catalyst, it was easily recovered by an external magnetic device and has the potential to improve the separation and purification processes.
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institution Universiti Putra Malaysia
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spelling upm-952502023-02-20T01:41:23Z http://psasir.upm.edu.my/id/eprint/95250/ Synthesis and characterization of bifunctional magnetic nano-catalyst from rice husk for production of biodiesel Hazmi, Balkis Rashid, Umer Ibrahim, Mohd Lokman Nehdi, Imededdine Arbi Azam, Mohammad Al-Resayes, Saud Ibrahim In this work, bifunctional magnetic nano-catalyst was successfully derived from rice husk char doped with potassium oxide and nickel oxide by impregnation techniques, and their catalytic ability was tested via transesterification of used cooking oil (UCO). The catalyst was characterized by thermogravimetric analyzer (TGA), X-ray diffraction spectroscopy (XRD), Fourier-transform infrared spectroscopy (FTIR), Temperature programmed desorption (TPD), Brunauer–Emmett–Teller (BET), Scanning electron microscopy equipped with energy dispersive x-ray analyzer (FESEM-EDX), and Vibrating sampling magnetometer (VSM) for magnetic properties. The optimized nanomagnetic bifunctional catalyst (RHC/K2O-20%/Ni-5%) had 3.014 mmol g-1 & 4.485 mmol g-1 of acidity and basicity, respectively, with the magnetic strength was recorded at 2.312 emu g−1. For the catalytic evaluation, a maximum biodiesel yield of 98.2% was accomplished with 4 wt% of catalyst loading, 12:1 methanol to UCO molar ratio at 65 °C within 2 h of reaction time. The catalyst was reused for up to 5 reaction cycles and producing 70% of biodiesel at the last cycles. The fuel properties of optimized biodiesel were measured using Biodiesel - American Standard Testing Method (ASTM) D6751. Due to the magnetic properties of the catalyst, it was easily recovered by an external magnetic device and has the potential to improve the separation and purification processes. Elsevier BV 2021 Article PeerReviewed Hazmi, Balkis and Rashid, Umer and Ibrahim, Mohd Lokman and Nehdi, Imededdine Arbi and Azam, Mohammad and Al-Resayes, Saud Ibrahim (2021) Synthesis and characterization of bifunctional magnetic nano-catalyst from rice husk for production of biodiesel. Environmental Technology & Innovation, 21. pp. 1-15. ISSN 2352-1864 https://www.sciencedirect.com/science/article/pii/S2352186420315960 10.1016/j.eti.2020.101296
spellingShingle Hazmi, Balkis
Rashid, Umer
Ibrahim, Mohd Lokman
Nehdi, Imededdine Arbi
Azam, Mohammad
Al-Resayes, Saud Ibrahim
Synthesis and characterization of bifunctional magnetic nano-catalyst from rice husk for production of biodiesel
title Synthesis and characterization of bifunctional magnetic nano-catalyst from rice husk for production of biodiesel
title_full Synthesis and characterization of bifunctional magnetic nano-catalyst from rice husk for production of biodiesel
title_fullStr Synthesis and characterization of bifunctional magnetic nano-catalyst from rice husk for production of biodiesel
title_full_unstemmed Synthesis and characterization of bifunctional magnetic nano-catalyst from rice husk for production of biodiesel
title_short Synthesis and characterization of bifunctional magnetic nano-catalyst from rice husk for production of biodiesel
title_sort synthesis and characterization of bifunctional magnetic nano-catalyst from rice husk for production of biodiesel
url http://psasir.upm.edu.my/id/eprint/95250/
http://psasir.upm.edu.my/id/eprint/95250/
http://psasir.upm.edu.my/id/eprint/95250/