Nanocrystalline cellulose from microcrystalline cellulose of date palm fibers as a promising candidate for bio-nanocomposites: isolation and characterization

Date palm fiber (Phoenix dactylifera L.) is a natural biopolymer rich in lignocellulosic components. Its high cellulose content lends them to the extraction of tiny particles like microcrystalline cellulose (MCC) and nanocrystalline cellulose (NCC). These cellulose-derived small size particles can b...

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Main Authors: Hachaichi, Amina, Kouini, Benalia, Lau, Kia Kian, Asim, Mohammad, Fouad, Hassan, Jawaid, Mohammad, Sain, Mohini
Format: Article
Published: MDPI 2021
Online Access:http://psasir.upm.edu.my/id/eprint/94318/
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author Hachaichi, Amina
Kouini, Benalia
Lau, Kia Kian
Asim, Mohammad
Fouad, Hassan
Jawaid, Mohammad
Sain, Mohini
author_facet Hachaichi, Amina
Kouini, Benalia
Lau, Kia Kian
Asim, Mohammad
Fouad, Hassan
Jawaid, Mohammad
Sain, Mohini
author_sort Hachaichi, Amina
building UPM Institutional Repository
collection Online Access
description Date palm fiber (Phoenix dactylifera L.) is a natural biopolymer rich in lignocellulosic components. Its high cellulose content lends them to the extraction of tiny particles like microcrystalline cellulose (MCC) and nanocrystalline cellulose (NCC). These cellulose-derived small size particles can be used as an alternative biomaterial in wide fields of application due to their renewability and sustainability. In the present work, NCC (A) and NCC (B) were isolated from date palm MCC at 60 min and 90 min hydrolysis times, respectively. The isolated NCC product was subjected to characterization to study their properties differences. With the hydrolysis treatment, the yields of produced NCC could be attained at between 22% and 25%. The infrared-ray functional analysis also revealed the isolated NCC possessed a highly exposed cellulose compartment with minimized lignoresidues of lignin and hemicellulose. From morphology evaluation, the nanoparticles’ size was decreased gradually from NCC (A) (7.51 nm width, 139.91 nm length) to NCC (B) (4.34 nm width, 111.51 nm length) as a result of fragmentation into cellulose fibrils. The crystallinity index was found increasing from NCC (A) to NCC (B). With 90 min hydrolysis time, NCC (B) showed the highest crystallinity index of 71% due to its great cellulose rigidity. For thermal analysis, NCC (B) also exhibited stable heat resistance, in associating with its highly crystalline cellulose structure. In conclusion, the NCC isolated from date palm MCC would be a promising biomaterial for various applications such as biomedical and food packaging applications.
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spelling upm-943182023-05-08T03:57:56Z http://psasir.upm.edu.my/id/eprint/94318/ Nanocrystalline cellulose from microcrystalline cellulose of date palm fibers as a promising candidate for bio-nanocomposites: isolation and characterization Hachaichi, Amina Kouini, Benalia Lau, Kia Kian Asim, Mohammad Fouad, Hassan Jawaid, Mohammad Sain, Mohini Date palm fiber (Phoenix dactylifera L.) is a natural biopolymer rich in lignocellulosic components. Its high cellulose content lends them to the extraction of tiny particles like microcrystalline cellulose (MCC) and nanocrystalline cellulose (NCC). These cellulose-derived small size particles can be used as an alternative biomaterial in wide fields of application due to their renewability and sustainability. In the present work, NCC (A) and NCC (B) were isolated from date palm MCC at 60 min and 90 min hydrolysis times, respectively. The isolated NCC product was subjected to characterization to study their properties differences. With the hydrolysis treatment, the yields of produced NCC could be attained at between 22% and 25%. The infrared-ray functional analysis also revealed the isolated NCC possessed a highly exposed cellulose compartment with minimized lignoresidues of lignin and hemicellulose. From morphology evaluation, the nanoparticles’ size was decreased gradually from NCC (A) (7.51 nm width, 139.91 nm length) to NCC (B) (4.34 nm width, 111.51 nm length) as a result of fragmentation into cellulose fibrils. The crystallinity index was found increasing from NCC (A) to NCC (B). With 90 min hydrolysis time, NCC (B) showed the highest crystallinity index of 71% due to its great cellulose rigidity. For thermal analysis, NCC (B) also exhibited stable heat resistance, in associating with its highly crystalline cellulose structure. In conclusion, the NCC isolated from date palm MCC would be a promising biomaterial for various applications such as biomedical and food packaging applications. MDPI 2021-09-15 Article PeerReviewed Hachaichi, Amina and Kouini, Benalia and Lau, Kia Kian and Asim, Mohammad and Fouad, Hassan and Jawaid, Mohammad and Sain, Mohini (2021) Nanocrystalline cellulose from microcrystalline cellulose of date palm fibers as a promising candidate for bio-nanocomposites: isolation and characterization. Materials, 14 (18). art. no. 5313. pp. 1-13. ISSN 1996-1944 https://www.mdpi.com/1996-1944/14/18/5313 10.3390/ma14185313
spellingShingle Hachaichi, Amina
Kouini, Benalia
Lau, Kia Kian
Asim, Mohammad
Fouad, Hassan
Jawaid, Mohammad
Sain, Mohini
Nanocrystalline cellulose from microcrystalline cellulose of date palm fibers as a promising candidate for bio-nanocomposites: isolation and characterization
title Nanocrystalline cellulose from microcrystalline cellulose of date palm fibers as a promising candidate for bio-nanocomposites: isolation and characterization
title_full Nanocrystalline cellulose from microcrystalline cellulose of date palm fibers as a promising candidate for bio-nanocomposites: isolation and characterization
title_fullStr Nanocrystalline cellulose from microcrystalline cellulose of date palm fibers as a promising candidate for bio-nanocomposites: isolation and characterization
title_full_unstemmed Nanocrystalline cellulose from microcrystalline cellulose of date palm fibers as a promising candidate for bio-nanocomposites: isolation and characterization
title_short Nanocrystalline cellulose from microcrystalline cellulose of date palm fibers as a promising candidate for bio-nanocomposites: isolation and characterization
title_sort nanocrystalline cellulose from microcrystalline cellulose of date palm fibers as a promising candidate for bio-nanocomposites: isolation and characterization
url http://psasir.upm.edu.my/id/eprint/94318/
http://psasir.upm.edu.my/id/eprint/94318/
http://psasir.upm.edu.my/id/eprint/94318/