Effect of cobalt on nickel oxide toward reduction behaviour in hydrogen and carbon monoxide atmosphere

The reduction behaviour of cobalt doped with nickel oxide and undoped nickel oxide (NiO) by hydrogen (H2) in nitrogen (20%, v/v) and carbon monoxide (CO) in nitrogen (40%, v/v) atmospheres have been investigated by temperature programmed reduction (TPR). The phases formed of partially and completely...

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Main Authors: Dzakaria, Norliza, Abu Tahari, Maratun Najiha, Samidin, Salma, Tengku Saharuddin, Tengku Shafazila, Salleh, Fairous, Lahuri, Azizul Hakim, Yarmo, Mohd Ambar
Format: Article
Language:English
Published: Trans Tech Publications 2020
Online Access:http://psasir.upm.edu.my/id/eprint/88578/
http://psasir.upm.edu.my/id/eprint/88578/1/ABSTRACT.pdf
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author Dzakaria, Norliza
Abu Tahari, Maratun Najiha
Samidin, Salma
Tengku Saharuddin, Tengku Shafazila
Salleh, Fairous
Lahuri, Azizul Hakim
Yarmo, Mohd Ambar
author_facet Dzakaria, Norliza
Abu Tahari, Maratun Najiha
Samidin, Salma
Tengku Saharuddin, Tengku Shafazila
Salleh, Fairous
Lahuri, Azizul Hakim
Yarmo, Mohd Ambar
author_sort Dzakaria, Norliza
building UPM Institutional Repository
collection Online Access
description The reduction behaviour of cobalt doped with nickel oxide and undoped nickel oxide (NiO) by hydrogen (H2) in nitrogen (20%, v/v) and carbon monoxide (CO) in nitrogen (40%, v/v) atmospheres have been investigated by temperature programmed reduction (TPR). The phases formed of partially and completely reduced samples were characterized by X-ray diffraction spectroscopy (XRD). TPR results indicate that the reduction of Co doped and undoped nickel oxide in both reductants proceed in one step reduction (NiO → Ni) without intermediate. TPR results also suggested that by adding Co metal into NiO, the reduction to metallic Ni by both reductant gaseous give different intensity of the peak. The reduction process of Co and undoped NiO become faster when H2 was used as a reductant. Furthermore, in H2 atmosphere, Co-NiO give complete reduction to metallic Ni at 700 °C. Meanwhile, XRD analysis indicated that NiO without Co composed better crystallite phases of NiO with higher intensity.
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institution Universiti Putra Malaysia
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publisher Trans Tech Publications
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spelling upm-885782021-12-21T08:56:06Z http://psasir.upm.edu.my/id/eprint/88578/ Effect of cobalt on nickel oxide toward reduction behaviour in hydrogen and carbon monoxide atmosphere Dzakaria, Norliza Abu Tahari, Maratun Najiha Samidin, Salma Tengku Saharuddin, Tengku Shafazila Salleh, Fairous Lahuri, Azizul Hakim Yarmo, Mohd Ambar The reduction behaviour of cobalt doped with nickel oxide and undoped nickel oxide (NiO) by hydrogen (H2) in nitrogen (20%, v/v) and carbon monoxide (CO) in nitrogen (40%, v/v) atmospheres have been investigated by temperature programmed reduction (TPR). The phases formed of partially and completely reduced samples were characterized by X-ray diffraction spectroscopy (XRD). TPR results indicate that the reduction of Co doped and undoped nickel oxide in both reductants proceed in one step reduction (NiO → Ni) without intermediate. TPR results also suggested that by adding Co metal into NiO, the reduction to metallic Ni by both reductant gaseous give different intensity of the peak. The reduction process of Co and undoped NiO become faster when H2 was used as a reductant. Furthermore, in H2 atmosphere, Co-NiO give complete reduction to metallic Ni at 700 °C. Meanwhile, XRD analysis indicated that NiO without Co composed better crystallite phases of NiO with higher intensity. Trans Tech Publications 2020 Article PeerReviewed text en http://psasir.upm.edu.my/id/eprint/88578/1/ABSTRACT.pdf Dzakaria, Norliza and Abu Tahari, Maratun Najiha and Samidin, Salma and Tengku Saharuddin, Tengku Shafazila and Salleh, Fairous and Lahuri, Azizul Hakim and Yarmo, Mohd Ambar (2020) Effect of cobalt on nickel oxide toward reduction behaviour in hydrogen and carbon monoxide atmosphere. Materials Science Forum, 1010. 373 - 378. ISSN 1662-9752 https://www.scientific.net/MSF.1010.373 10.4028/www.scientific.net/MSF.1010.373
spellingShingle Dzakaria, Norliza
Abu Tahari, Maratun Najiha
Samidin, Salma
Tengku Saharuddin, Tengku Shafazila
Salleh, Fairous
Lahuri, Azizul Hakim
Yarmo, Mohd Ambar
Effect of cobalt on nickel oxide toward reduction behaviour in hydrogen and carbon monoxide atmosphere
title Effect of cobalt on nickel oxide toward reduction behaviour in hydrogen and carbon monoxide atmosphere
title_full Effect of cobalt on nickel oxide toward reduction behaviour in hydrogen and carbon monoxide atmosphere
title_fullStr Effect of cobalt on nickel oxide toward reduction behaviour in hydrogen and carbon monoxide atmosphere
title_full_unstemmed Effect of cobalt on nickel oxide toward reduction behaviour in hydrogen and carbon monoxide atmosphere
title_short Effect of cobalt on nickel oxide toward reduction behaviour in hydrogen and carbon monoxide atmosphere
title_sort effect of cobalt on nickel oxide toward reduction behaviour in hydrogen and carbon monoxide atmosphere
url http://psasir.upm.edu.my/id/eprint/88578/
http://psasir.upm.edu.my/id/eprint/88578/
http://psasir.upm.edu.my/id/eprint/88578/
http://psasir.upm.edu.my/id/eprint/88578/1/ABSTRACT.pdf