Voltammetric determination of iodide in iodized table salt using cetyltrimethylammonium bromide as ion-pairing

In this work, voltammetric study based on cetyltrimethylammonium bromide (CTAB) as an ion-pairing agent for the determination of iodine level in iodized table salt has been explored. CTAB was used as an intermediate compound between iodide (I−) and the electrode due to its ability to dissociate to p...

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Main Authors: Jamilan, M. A., Abdullah, J., Alang Ahmad, S. A., Md Noh, M. F.
Format: Article
Language:English
Published: Springer 2019
Online Access:http://psasir.upm.edu.my/id/eprint/82738/
http://psasir.upm.edu.my/id/eprint/82738/1/Voltammetric%20determination.pdf
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author Jamilan, M. A.
Abdullah, J.
Alang Ahmad, S. A.
Md Noh, M. F.
author_facet Jamilan, M. A.
Abdullah, J.
Alang Ahmad, S. A.
Md Noh, M. F.
author_sort Jamilan, M. A.
building UPM Institutional Repository
collection Online Access
description In this work, voltammetric study based on cetyltrimethylammonium bromide (CTAB) as an ion-pairing agent for the determination of iodine level in iodized table salt has been explored. CTAB was used as an intermediate compound between iodide (I−) and the electrode due to its ability to dissociate to produce cetyltrimethylammonium ions ([CTA]+). The [CTA]+ with a long hydrophobic alkyl chain can be directly adsorbed onto the surface of the working electrode, and this in turns coated the electrode with cationic charge and enhance the electrode ability to bind to iodide (I−) and other molecular iodine ions. A mixture of iodide and CTAB ([CTA]+I−) was prepared and potential of 1.0 V for 60.0 s was applied to pre-concentrate the solution on the working electrode causing the [CTA]+I− to oxidize to iodine (I2). The produced I2 immediately react with chloride ion (Cl−) from the electrolyte of hydrochloric acid (HCl) to produce I2Cl− and form ion-pair with CTA+ as [CTA]+I2Cl−. The linear calibration curve of the developed method towards iodide was in the concentration range of 0.5–4.0 mg/L with sensitivity of − 1.383 µA mg/L−1 cm−2 (R2 = 0.9950), limit of detection (LOD) of 0.3 mg/L and limit of quantification (LOQ) of 1.0 mg/L, respectively. The proposed method indicates good agreement with the standard method for iodine determination with recovery range from 95.0 to 104.3%. The developed method provided potential application as a portable on-site iodine detector.
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spelling upm-827382020-10-16T20:16:01Z http://psasir.upm.edu.my/id/eprint/82738/ Voltammetric determination of iodide in iodized table salt using cetyltrimethylammonium bromide as ion-pairing Jamilan, M. A. Abdullah, J. Alang Ahmad, S. A. Md Noh, M. F. In this work, voltammetric study based on cetyltrimethylammonium bromide (CTAB) as an ion-pairing agent for the determination of iodine level in iodized table salt has been explored. CTAB was used as an intermediate compound between iodide (I−) and the electrode due to its ability to dissociate to produce cetyltrimethylammonium ions ([CTA]+). The [CTA]+ with a long hydrophobic alkyl chain can be directly adsorbed onto the surface of the working electrode, and this in turns coated the electrode with cationic charge and enhance the electrode ability to bind to iodide (I−) and other molecular iodine ions. A mixture of iodide and CTAB ([CTA]+I−) was prepared and potential of 1.0 V for 60.0 s was applied to pre-concentrate the solution on the working electrode causing the [CTA]+I− to oxidize to iodine (I2). The produced I2 immediately react with chloride ion (Cl−) from the electrolyte of hydrochloric acid (HCl) to produce I2Cl− and form ion-pair with CTA+ as [CTA]+I2Cl−. The linear calibration curve of the developed method towards iodide was in the concentration range of 0.5–4.0 mg/L with sensitivity of − 1.383 µA mg/L−1 cm−2 (R2 = 0.9950), limit of detection (LOD) of 0.3 mg/L and limit of quantification (LOQ) of 1.0 mg/L, respectively. The proposed method indicates good agreement with the standard method for iodine determination with recovery range from 95.0 to 104.3%. The developed method provided potential application as a portable on-site iodine detector. Springer 2019 Article PeerReviewed text en http://psasir.upm.edu.my/id/eprint/82738/1/Voltammetric%20determination.pdf Jamilan, M. A. and Abdullah, J. and Alang Ahmad, S. A. and Md Noh, M. F. (2019) Voltammetric determination of iodide in iodized table salt using cetyltrimethylammonium bromide as ion-pairing. Journal of Food Science and Technology, 56 (8). pp. 3846-3853. ISSN 0022-1155; ESSN: 0975-8402 10.1007/s13197-019-03855-x
spellingShingle Jamilan, M. A.
Abdullah, J.
Alang Ahmad, S. A.
Md Noh, M. F.
Voltammetric determination of iodide in iodized table salt using cetyltrimethylammonium bromide as ion-pairing
title Voltammetric determination of iodide in iodized table salt using cetyltrimethylammonium bromide as ion-pairing
title_full Voltammetric determination of iodide in iodized table salt using cetyltrimethylammonium bromide as ion-pairing
title_fullStr Voltammetric determination of iodide in iodized table salt using cetyltrimethylammonium bromide as ion-pairing
title_full_unstemmed Voltammetric determination of iodide in iodized table salt using cetyltrimethylammonium bromide as ion-pairing
title_short Voltammetric determination of iodide in iodized table salt using cetyltrimethylammonium bromide as ion-pairing
title_sort voltammetric determination of iodide in iodized table salt using cetyltrimethylammonium bromide as ion-pairing
url http://psasir.upm.edu.my/id/eprint/82738/
http://psasir.upm.edu.my/id/eprint/82738/
http://psasir.upm.edu.my/id/eprint/82738/1/Voltammetric%20determination.pdf