Lipase-catalysed production and chemical composition of diacylglycerols from soybean oil deodoriser distillate

Diacylglycerols (DAG) were enzymatically produced by lipase-catalysed esterification of glycerol with fatty acids from soybean oil deodoriser distillate (SODD). Effects of reaction parameters such as reaction time, temperature, enzyme type, enzyme load, substrate molar ratio and water content, as we...

Full description

Bibliographic Details
Main Authors: Lo, Seong Koon, Baharin, Badlishah Sham, Tan, Chin Ping, Lai, Oi Ming
Format: Article
Language:English
English
Published: Wiley-Blackwell 2004
Online Access:http://psasir.upm.edu.my/id/eprint/7289/
http://psasir.upm.edu.my/id/eprint/7289/1/Lipase-catalysed%20production%20and%20chemical%20composition%20of%20diacylglycerols%20from%20soybean%20oil%20deodoriser%20distillate.pdf
_version_ 1848840553763962880
author Lo, Seong Koon
Baharin, Badlishah Sham
Tan, Chin Ping
Lai, Oi Ming
author_facet Lo, Seong Koon
Baharin, Badlishah Sham
Tan, Chin Ping
Lai, Oi Ming
author_sort Lo, Seong Koon
building UPM Institutional Repository
collection Online Access
description Diacylglycerols (DAG) were enzymatically produced by lipase-catalysed esterification of glycerol with fatty acids from soybean oil deodoriser distillate (SODD). Effects of reaction parameters such as reaction time, temperature, enzyme type, enzyme load, substrate molar ratio and water content, as well as the effect of molecular sieves as water adsorbent were studied. Lipozyme RM IM was determined to be the most effective among the lipases screened. The following conditions yielded 69.9% DAG (all percentages are wt/wt): 4 h reaction time, 65 °C reaction temperature, 10% Lipozyme RM IM, 2.5:1 fatty acid to glycerol molar ratio, and 30% molecular sieves. DAG synthesis of 11.9% was still observed at 10% water content. After purification, the product oil contained 86.3% DAG. This oil consisted predominantly of 1,3-diolein (19.1%), 1-oleoyl-3-linoleoyl-glycerol (18.2%) and 1-oleoyl-2-linoleoyl-glycerol (16.6%). The fatty acid profile of the oil was similar to that of refined, bleached and deodorised (RBD) soybean oil. The % ratio of 1,3- to 1,2-positional isomers of DAG was at 56:44.
first_indexed 2025-11-15T07:29:11Z
format Article
id upm-7289
institution Universiti Putra Malaysia
institution_category Local University
language English
English
last_indexed 2025-11-15T07:29:11Z
publishDate 2004
publisher Wiley-Blackwell
recordtype eprints
repository_type Digital Repository
spelling upm-72892015-10-06T00:47:47Z http://psasir.upm.edu.my/id/eprint/7289/ Lipase-catalysed production and chemical composition of diacylglycerols from soybean oil deodoriser distillate Lo, Seong Koon Baharin, Badlishah Sham Tan, Chin Ping Lai, Oi Ming Diacylglycerols (DAG) were enzymatically produced by lipase-catalysed esterification of glycerol with fatty acids from soybean oil deodoriser distillate (SODD). Effects of reaction parameters such as reaction time, temperature, enzyme type, enzyme load, substrate molar ratio and water content, as well as the effect of molecular sieves as water adsorbent were studied. Lipozyme RM IM was determined to be the most effective among the lipases screened. The following conditions yielded 69.9% DAG (all percentages are wt/wt): 4 h reaction time, 65 °C reaction temperature, 10% Lipozyme RM IM, 2.5:1 fatty acid to glycerol molar ratio, and 30% molecular sieves. DAG synthesis of 11.9% was still observed at 10% water content. After purification, the product oil contained 86.3% DAG. This oil consisted predominantly of 1,3-diolein (19.1%), 1-oleoyl-3-linoleoyl-glycerol (18.2%) and 1-oleoyl-2-linoleoyl-glycerol (16.6%). The fatty acid profile of the oil was similar to that of refined, bleached and deodorised (RBD) soybean oil. The % ratio of 1,3- to 1,2-positional isomers of DAG was at 56:44. Wiley-Blackwell 2004-04-21 Article PeerReviewed application/pdf en http://psasir.upm.edu.my/id/eprint/7289/1/Lipase-catalysed%20production%20and%20chemical%20composition%20of%20diacylglycerols%20from%20soybean%20oil%20deodoriser%20distillate.pdf Lo, Seong Koon and Baharin, Badlishah Sham and Tan, Chin Ping and Lai, Oi Ming (2004) Lipase-catalysed production and chemical composition of diacylglycerols from soybean oil deodoriser distillate. European Journal of Lipid Science and Technology, 106 (4). pp. 218-224. ISSN 1438-7697 http://dx.doi.org/10.1002/ejlt.200300888 10.1002/ejlt.200300888 English
spellingShingle Lo, Seong Koon
Baharin, Badlishah Sham
Tan, Chin Ping
Lai, Oi Ming
Lipase-catalysed production and chemical composition of diacylglycerols from soybean oil deodoriser distillate
title Lipase-catalysed production and chemical composition of diacylglycerols from soybean oil deodoriser distillate
title_full Lipase-catalysed production and chemical composition of diacylglycerols from soybean oil deodoriser distillate
title_fullStr Lipase-catalysed production and chemical composition of diacylglycerols from soybean oil deodoriser distillate
title_full_unstemmed Lipase-catalysed production and chemical composition of diacylglycerols from soybean oil deodoriser distillate
title_short Lipase-catalysed production and chemical composition of diacylglycerols from soybean oil deodoriser distillate
title_sort lipase-catalysed production and chemical composition of diacylglycerols from soybean oil deodoriser distillate
url http://psasir.upm.edu.my/id/eprint/7289/
http://psasir.upm.edu.my/id/eprint/7289/
http://psasir.upm.edu.my/id/eprint/7289/
http://psasir.upm.edu.my/id/eprint/7289/1/Lipase-catalysed%20production%20and%20chemical%20composition%20of%20diacylglycerols%20from%20soybean%20oil%20deodoriser%20distillate.pdf