Evaluation of porogen factors for the preparation of ion imprinted polymer monoliths used in mercury removal

In the present study, ion imprinted polymer monoliths (IIPMs) were developed to overcome the limitations of ion imprinted polymer particles (IIPPs) used for the removal of Hg(II) ions from waste water samples. The adsorbents preparation, characterization and Hg(II) removal were very well reported. T...

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Main Authors: Ab. Rahman, Siti Khadijah, Yusof, Nor Azah, Abdullah, Abdul Halim, Mohammad, Faruq, Idris, Azni, Al-Lohedan, Hamad A.
Format: Article
Language:English
Published: Public Library of Science 2018
Online Access:http://psasir.upm.edu.my/id/eprint/72641/
http://psasir.upm.edu.my/id/eprint/72641/1/Evaluation%20of%20porogen%20factors.pdf
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author Ab. Rahman, Siti Khadijah
Yusof, Nor Azah
Abdullah, Abdul Halim
Mohammad, Faruq
Idris, Azni
Al-Lohedan, Hamad A.
author_facet Ab. Rahman, Siti Khadijah
Yusof, Nor Azah
Abdullah, Abdul Halim
Mohammad, Faruq
Idris, Azni
Al-Lohedan, Hamad A.
author_sort Ab. Rahman, Siti Khadijah
building UPM Institutional Repository
collection Online Access
description In the present study, ion imprinted polymer monoliths (IIPMs) were developed to overcome the limitations of ion imprinted polymer particles (IIPPs) used for the removal of Hg(II) ions from waste water samples. The adsorbents preparation, characterization and Hg(II) removal were very well reported. The IIPMs on porogen optimization was prepared using the molding technique with Hg(II) as a template ion, [2-(methacryloyloxy)ethyl]trimethylammonium cysteine (MAETC) as ligand, methacrylic acid (MAA) as functional monomer, ethylene glycol dimethacrylamide (EGDMA) as cross-linker, benzoyl peroxide as an initiator and methanol and acetonitrile as porogen in the polypropylene tube (drinking straw) as mold. The IIPMs prepared with higher volumes of porogen were indicated to have a good adsorption rate for the Hg(II) removal along with good water permeability and larger porosity as compared to a lower volume of porogen. The IIPMs prepared using the binary porogen were able to improve the porosity and surface area of the monolithic polymers as compared to the single porogen added IIPMs. Finally, we indicate from our analysis that the IIPM having the efficient capacity for the Hg(II) ions is easy to prepare, and has higher water permeability along with high porosity and high adsorption capacity and all these factors making it one of the suitable adsorbent for the successful removal of Hg(II) ions.
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spelling upm-726412020-11-19T01:39:54Z http://psasir.upm.edu.my/id/eprint/72641/ Evaluation of porogen factors for the preparation of ion imprinted polymer monoliths used in mercury removal Ab. Rahman, Siti Khadijah Yusof, Nor Azah Abdullah, Abdul Halim Mohammad, Faruq Idris, Azni Al-Lohedan, Hamad A. In the present study, ion imprinted polymer monoliths (IIPMs) were developed to overcome the limitations of ion imprinted polymer particles (IIPPs) used for the removal of Hg(II) ions from waste water samples. The adsorbents preparation, characterization and Hg(II) removal were very well reported. The IIPMs on porogen optimization was prepared using the molding technique with Hg(II) as a template ion, [2-(methacryloyloxy)ethyl]trimethylammonium cysteine (MAETC) as ligand, methacrylic acid (MAA) as functional monomer, ethylene glycol dimethacrylamide (EGDMA) as cross-linker, benzoyl peroxide as an initiator and methanol and acetonitrile as porogen in the polypropylene tube (drinking straw) as mold. The IIPMs prepared with higher volumes of porogen were indicated to have a good adsorption rate for the Hg(II) removal along with good water permeability and larger porosity as compared to a lower volume of porogen. The IIPMs prepared using the binary porogen were able to improve the porosity and surface area of the monolithic polymers as compared to the single porogen added IIPMs. Finally, we indicate from our analysis that the IIPM having the efficient capacity for the Hg(II) ions is easy to prepare, and has higher water permeability along with high porosity and high adsorption capacity and all these factors making it one of the suitable adsorbent for the successful removal of Hg(II) ions. Public Library of Science 2018-04 Article PeerReviewed text en http://psasir.upm.edu.my/id/eprint/72641/1/Evaluation%20of%20porogen%20factors.pdf Ab. Rahman, Siti Khadijah and Yusof, Nor Azah and Abdullah, Abdul Halim and Mohammad, Faruq and Idris, Azni and Al-Lohedan, Hamad A. (2018) Evaluation of porogen factors for the preparation of ion imprinted polymer monoliths used in mercury removal. PLoS One, 13 (4). pp. 1-14. ISSN 1932-6203 https://journals.plos.org/plosone/article?id=10.1371/journal.pone.0195546 10.1371/journal.pone.0195546
spellingShingle Ab. Rahman, Siti Khadijah
Yusof, Nor Azah
Abdullah, Abdul Halim
Mohammad, Faruq
Idris, Azni
Al-Lohedan, Hamad A.
Evaluation of porogen factors for the preparation of ion imprinted polymer monoliths used in mercury removal
title Evaluation of porogen factors for the preparation of ion imprinted polymer monoliths used in mercury removal
title_full Evaluation of porogen factors for the preparation of ion imprinted polymer monoliths used in mercury removal
title_fullStr Evaluation of porogen factors for the preparation of ion imprinted polymer monoliths used in mercury removal
title_full_unstemmed Evaluation of porogen factors for the preparation of ion imprinted polymer monoliths used in mercury removal
title_short Evaluation of porogen factors for the preparation of ion imprinted polymer monoliths used in mercury removal
title_sort evaluation of porogen factors for the preparation of ion imprinted polymer monoliths used in mercury removal
url http://psasir.upm.edu.my/id/eprint/72641/
http://psasir.upm.edu.my/id/eprint/72641/
http://psasir.upm.edu.my/id/eprint/72641/
http://psasir.upm.edu.my/id/eprint/72641/1/Evaluation%20of%20porogen%20factors.pdf