Effects of aging time on microstructure, hydrophobic and optical properties of BiFeO3 thin films synthesized via sol-gel method

BiFeO3 (BFO) films were synthesized with the sol-gel method followed by the spin coating technique using 2-methoxyethanol as solvent and acetylacetone as chelating agent. The effects of aging time (t = 0, 1, 3, 6 days) of the BFO sol on the microstructure, wettability and optical properties of BFO f...

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Main Authors: Baqiah, Hussein Abdullah Hussein, Talib, Zainal Abidin, Shaari, Abdul Halim, Awang Kechik, Mohd Mustafa, Liew, Josephine Ying Chyi, Ibrahim, Noor Baa'yah
Format: Article
Language:English
Published: Goeller Verlag GmbH 2018
Online Access:http://psasir.upm.edu.my/id/eprint/72477/
http://psasir.upm.edu.my/id/eprint/72477/1/Effects%20of%20aging%20time%20on%20microstructure.pdf
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author Baqiah, Hussein Abdullah Hussein
Talib, Zainal Abidin
Shaari, Abdul Halim
Awang Kechik, Mohd Mustafa
Liew, Josephine Ying Chyi
Ibrahim, Noor Baa'yah
author_facet Baqiah, Hussein Abdullah Hussein
Talib, Zainal Abidin
Shaari, Abdul Halim
Awang Kechik, Mohd Mustafa
Liew, Josephine Ying Chyi
Ibrahim, Noor Baa'yah
author_sort Baqiah, Hussein Abdullah Hussein
building UPM Institutional Repository
collection Online Access
description BiFeO3 (BFO) films were synthesized with the sol-gel method followed by the spin coating technique using 2-methoxyethanol as solvent and acetylacetone as chelating agent. The effects of aging time (t = 0, 1, 3, 6 days) of the BFO sol on the microstructure, wettability and optical properties of BFO films were investigated by means of X-ray diffraction (XRD), atomic force microscopy (AFM), contact angle (CA) measurement, Uv-vis and photoluminescence. The crystallinity of films was affected by t. Crystallite size of the films changed slightly in the range of 14.2 – 15.2 nm while the lattice parameters clearly varied with t. The average particle size of BFO films ranged between 45.9 and 52.7 nm while the mean square roughness (Rq) varied between 1.0 and 4.2 nm. The films showed maximum optical transmittance (81 – 90 %) in the range 600 – 800 nm. The band gap of the films was also affected with t, and it has a value of 2.85 to 2.76 eV. The films showed a hydrophobic property with CA ranging between 95.3 to 104.7 °. The best crystallinity, lowest Rq and highest Eg = 2.85 eV were obtained for the film with t = 1 day. The results demonstrate possible development of a superhydrophobic coating using BiFeO3 coating.
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spelling upm-724772020-06-17T02:22:04Z http://psasir.upm.edu.my/id/eprint/72477/ Effects of aging time on microstructure, hydrophobic and optical properties of BiFeO3 thin films synthesized via sol-gel method Baqiah, Hussein Abdullah Hussein Talib, Zainal Abidin Shaari, Abdul Halim Awang Kechik, Mohd Mustafa Liew, Josephine Ying Chyi Ibrahim, Noor Baa'yah BiFeO3 (BFO) films were synthesized with the sol-gel method followed by the spin coating technique using 2-methoxyethanol as solvent and acetylacetone as chelating agent. The effects of aging time (t = 0, 1, 3, 6 days) of the BFO sol on the microstructure, wettability and optical properties of BFO films were investigated by means of X-ray diffraction (XRD), atomic force microscopy (AFM), contact angle (CA) measurement, Uv-vis and photoluminescence. The crystallinity of films was affected by t. Crystallite size of the films changed slightly in the range of 14.2 – 15.2 nm while the lattice parameters clearly varied with t. The average particle size of BFO films ranged between 45.9 and 52.7 nm while the mean square roughness (Rq) varied between 1.0 and 4.2 nm. The films showed maximum optical transmittance (81 – 90 %) in the range 600 – 800 nm. The band gap of the films was also affected with t, and it has a value of 2.85 to 2.76 eV. The films showed a hydrophobic property with CA ranging between 95.3 to 104.7 °. The best crystallinity, lowest Rq and highest Eg = 2.85 eV were obtained for the film with t = 1 day. The results demonstrate possible development of a superhydrophobic coating using BiFeO3 coating. Goeller Verlag GmbH 2018 Article NonPeerReviewed text en http://psasir.upm.edu.my/id/eprint/72477/1/Effects%20of%20aging%20time%20on%20microstructure.pdf Baqiah, Hussein Abdullah Hussein and Talib, Zainal Abidin and Shaari, Abdul Halim and Awang Kechik, Mohd Mustafa and Liew, Josephine Ying Chyi and Ibrahim, Noor Baa'yah (2018) Effects of aging time on microstructure, hydrophobic and optical properties of BiFeO3 thin films synthesized via sol-gel method. Journal of Ceramic Science and Technology, 9 (4). 419 - 426. ISSN 2190-9385 https://www.ceramic-science.com/articles/all-articles.html?article_id=100686 10.4416/JCST2018-00039
spellingShingle Baqiah, Hussein Abdullah Hussein
Talib, Zainal Abidin
Shaari, Abdul Halim
Awang Kechik, Mohd Mustafa
Liew, Josephine Ying Chyi
Ibrahim, Noor Baa'yah
Effects of aging time on microstructure, hydrophobic and optical properties of BiFeO3 thin films synthesized via sol-gel method
title Effects of aging time on microstructure, hydrophobic and optical properties of BiFeO3 thin films synthesized via sol-gel method
title_full Effects of aging time on microstructure, hydrophobic and optical properties of BiFeO3 thin films synthesized via sol-gel method
title_fullStr Effects of aging time on microstructure, hydrophobic and optical properties of BiFeO3 thin films synthesized via sol-gel method
title_full_unstemmed Effects of aging time on microstructure, hydrophobic and optical properties of BiFeO3 thin films synthesized via sol-gel method
title_short Effects of aging time on microstructure, hydrophobic and optical properties of BiFeO3 thin films synthesized via sol-gel method
title_sort effects of aging time on microstructure, hydrophobic and optical properties of bifeo3 thin films synthesized via sol-gel method
url http://psasir.upm.edu.my/id/eprint/72477/
http://psasir.upm.edu.my/id/eprint/72477/
http://psasir.upm.edu.my/id/eprint/72477/
http://psasir.upm.edu.my/id/eprint/72477/1/Effects%20of%20aging%20time%20on%20microstructure.pdf