Sol-gel synthesis of Fe₂O₃-doped TiO₂ for optimized photocatalytic degradation of 2,4- dichlorophenoxyacetic acid

Fe₂O₃-doped and undoped TiO₂ catalysts were synthesized by sol-gel method and used to optimize the photocatalytic degradation of 2,4-Dichlorophenoxyacetic acid (2,4-D). The catalysts produced were dominated by the tetragonal, crystalline anatase TiO₂ cell structure. The 0.05wt% Fe₂O₃-doped TiO₂ cata...

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Main Authors: Razani, Afini, Abdullah, Abdul Halim, Fitrianto, Anwar, Yusof, Nor Azah, Gaya, Umar Ibrahim
Format: Article
Language:English
Published: Oriental Scientific Publishing 2017
Online Access:http://psasir.upm.edu.my/id/eprint/63252/
http://psasir.upm.edu.my/id/eprint/63252/1/Sol-gel%20synthesis%20of%20Fe%E2%82%82O%E2%82%83-doped%20TiO%E2%82%82%20for%20optimized%20photocatalytic%20degradation%20of%202%2C%204-%20dichlorophenoxyacetic%20acid.pdf
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author Razani, Afini
Abdullah, Abdul Halim
Fitrianto, Anwar
Yusof, Nor Azah
Gaya, Umar Ibrahim
author_facet Razani, Afini
Abdullah, Abdul Halim
Fitrianto, Anwar
Yusof, Nor Azah
Gaya, Umar Ibrahim
author_sort Razani, Afini
building UPM Institutional Repository
collection Online Access
description Fe₂O₃-doped and undoped TiO₂ catalysts were synthesized by sol-gel method and used to optimize the photocatalytic degradation of 2,4-Dichlorophenoxyacetic acid (2,4-D). The catalysts produced were dominated by the tetragonal, crystalline anatase TiO₂ cell structure. The 0.05wt% Fe₂O₃-doped TiO₂ catalyst exhibited higher photocatalytic activity than that of undoped TiO₂ but its performance decline with increase Fe₂O₃ content due to possible increase of recombination centers. Photocatalytic degradation of 2,4-DA was optimized by response surface methodology. The highest 2,4-DA degradation (48%) was obtained when 1.0 g of 0.05wt% Fe₂O₃-doped TiO₂ is used to degrade 10 ppm of 2,4-DA at pH 4.
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language English
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publishDate 2017
publisher Oriental Scientific Publishing
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spelling upm-632522018-09-26T01:31:20Z http://psasir.upm.edu.my/id/eprint/63252/ Sol-gel synthesis of Fe₂O₃-doped TiO₂ for optimized photocatalytic degradation of 2,4- dichlorophenoxyacetic acid Razani, Afini Abdullah, Abdul Halim Fitrianto, Anwar Yusof, Nor Azah Gaya, Umar Ibrahim Fe₂O₃-doped and undoped TiO₂ catalysts were synthesized by sol-gel method and used to optimize the photocatalytic degradation of 2,4-Dichlorophenoxyacetic acid (2,4-D). The catalysts produced were dominated by the tetragonal, crystalline anatase TiO₂ cell structure. The 0.05wt% Fe₂O₃-doped TiO₂ catalyst exhibited higher photocatalytic activity than that of undoped TiO₂ but its performance decline with increase Fe₂O₃ content due to possible increase of recombination centers. Photocatalytic degradation of 2,4-DA was optimized by response surface methodology. The highest 2,4-DA degradation (48%) was obtained when 1.0 g of 0.05wt% Fe₂O₃-doped TiO₂ is used to degrade 10 ppm of 2,4-DA at pH 4. Oriental Scientific Publishing 2017 Article PeerReviewed text en http://psasir.upm.edu.my/id/eprint/63252/1/Sol-gel%20synthesis%20of%20Fe%E2%82%82O%E2%82%83-doped%20TiO%E2%82%82%20for%20optimized%20photocatalytic%20degradation%20of%202%2C%204-%20dichlorophenoxyacetic%20acid.pdf Razani, Afini and Abdullah, Abdul Halim and Fitrianto, Anwar and Yusof, Nor Azah and Gaya, Umar Ibrahim (2017) Sol-gel synthesis of Fe₂O₃-doped TiO₂ for optimized photocatalytic degradation of 2,4- dichlorophenoxyacetic acid. Oriental Journal of Chemistry, 33 (4). 1959 - 1968. ISSN 0970-020X http://www.orientjchem.org/vol33no4/sol-gel-synthesis-of-fe2o3-doped-tio2-photocatalyst-for-optimized-photocatalytic-degradation-of-24-dichlorophenoxyacetic-acid/ 10.13005/ojc/330442
spellingShingle Razani, Afini
Abdullah, Abdul Halim
Fitrianto, Anwar
Yusof, Nor Azah
Gaya, Umar Ibrahim
Sol-gel synthesis of Fe₂O₃-doped TiO₂ for optimized photocatalytic degradation of 2,4- dichlorophenoxyacetic acid
title Sol-gel synthesis of Fe₂O₃-doped TiO₂ for optimized photocatalytic degradation of 2,4- dichlorophenoxyacetic acid
title_full Sol-gel synthesis of Fe₂O₃-doped TiO₂ for optimized photocatalytic degradation of 2,4- dichlorophenoxyacetic acid
title_fullStr Sol-gel synthesis of Fe₂O₃-doped TiO₂ for optimized photocatalytic degradation of 2,4- dichlorophenoxyacetic acid
title_full_unstemmed Sol-gel synthesis of Fe₂O₃-doped TiO₂ for optimized photocatalytic degradation of 2,4- dichlorophenoxyacetic acid
title_short Sol-gel synthesis of Fe₂O₃-doped TiO₂ for optimized photocatalytic degradation of 2,4- dichlorophenoxyacetic acid
title_sort sol-gel synthesis of fe₂o₃-doped tio₂ for optimized photocatalytic degradation of 2,4- dichlorophenoxyacetic acid
url http://psasir.upm.edu.my/id/eprint/63252/
http://psasir.upm.edu.my/id/eprint/63252/
http://psasir.upm.edu.my/id/eprint/63252/
http://psasir.upm.edu.my/id/eprint/63252/1/Sol-gel%20synthesis%20of%20Fe%E2%82%82O%E2%82%83-doped%20TiO%E2%82%82%20for%20optimized%20photocatalytic%20degradation%20of%202%2C%204-%20dichlorophenoxyacetic%20acid.pdf