Down-top nanofabrication of binary (CdO)x (ZnO)1–x nanoparticles and their antibacterial activity

In the present study, binary oxide (cadmium oxide [CdO])x (zinc oxide [ZnO])1–x nanoparticles (NPs) at different concentrations of precursor in calcination temperature were prepared using thermal treatment technique. Cadmium and zinc nitrates (source of cadmium and zinc) with polyvinylpyrrolidone (c...

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Main Authors: Al-Hada, Naif Mohammed, Mohamed Kamari, Halimah, Che Abdullah, Che Azurahanim, Saion, Elias, Shaari, Abdul Halim, Talib, Zainal Abidin, Matori, Khamirul Amin
Format: Article
Language:English
Published: Dove Medical Press 2017
Online Access:http://psasir.upm.edu.my/id/eprint/61519/
http://psasir.upm.edu.my/id/eprint/61519/1/Down-top%20nanofabrication%20of%20binary%20%28CdO%29x%20%28ZnO%291%E2%80%93x%20nanoparticles%20and%20their%20antibacterial%20activity.pdf
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author Al-Hada, Naif Mohammed
Mohamed Kamari, Halimah
Che Abdullah, Che Azurahanim
Saion, Elias
Shaari, Abdul Halim
Talib, Zainal Abidin
Matori, Khamirul Amin
author_facet Al-Hada, Naif Mohammed
Mohamed Kamari, Halimah
Che Abdullah, Che Azurahanim
Saion, Elias
Shaari, Abdul Halim
Talib, Zainal Abidin
Matori, Khamirul Amin
author_sort Al-Hada, Naif Mohammed
building UPM Institutional Repository
collection Online Access
description In the present study, binary oxide (cadmium oxide [CdO])x (zinc oxide [ZnO])1–x nanoparticles (NPs) at different concentrations of precursor in calcination temperature were prepared using thermal treatment technique. Cadmium and zinc nitrates (source of cadmium and zinc) with polyvinylpyrrolidone (capping agent) have been used to prepare (CdO)x (ZnO)1–x NPs samples. The sample was characterized by X-ray diffraction (XRD), scanning electron microscopy, energy-dispersive X-ray (EDX), transmission electron microscopy (TEM), and Fourier transform infrared (FTIR) spectroscopy. XRD patterns analysis revealed that NPs were formed after calcination, which showed a cubic and hexagonal crystalline structure of (CdO)x (ZnO)1–x NPs. The phase analysis using EDX spectroscopy and FTIR spectroscopy confirmed the presence of Cd and Zn as the original compounds of prepared (CdO)x (ZnO)1–x NP samples. The average particle size of the samples increased from 14 to 33 nm as the concentration of precursor increased from x=0.20 to x=0.80, as observed by TEM results. The surface composition and valance state of the prepared product NPs were determined by X-ray photoelectron spectroscopy (XPS) analyses. Diffuse UV–visible reflectance spectra were used to determine the optical band gap through the Kubelka–Munk equation; the energy band gap was found to decrease for CdO from 2.92 to 2.82 eV and for ZnO from 3.22 to 3.11 eV with increasing x value. Additionally, photoluminescence (PL) spectra revealed that the intensity in PL increased with an increase in particle size. In addition, the antibacterial activity of binary oxide NP was carried out in vitro against Escherichia coli ATCC 25922 Gram (-ve), Salmonella choleraesuis ATCC 10708, and Bacillus subtilis UPMC 1175 Gram (+ve). This study indicated that the zone of inhibition of 21 mm has good antibacterial activity toward the Gram-positive B. subtilis UPMC 1175.
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spelling upm-615192022-04-05T02:09:56Z http://psasir.upm.edu.my/id/eprint/61519/ Down-top nanofabrication of binary (CdO)x (ZnO)1–x nanoparticles and their antibacterial activity Al-Hada, Naif Mohammed Mohamed Kamari, Halimah Che Abdullah, Che Azurahanim Saion, Elias Shaari, Abdul Halim Talib, Zainal Abidin Matori, Khamirul Amin In the present study, binary oxide (cadmium oxide [CdO])x (zinc oxide [ZnO])1–x nanoparticles (NPs) at different concentrations of precursor in calcination temperature were prepared using thermal treatment technique. Cadmium and zinc nitrates (source of cadmium and zinc) with polyvinylpyrrolidone (capping agent) have been used to prepare (CdO)x (ZnO)1–x NPs samples. The sample was characterized by X-ray diffraction (XRD), scanning electron microscopy, energy-dispersive X-ray (EDX), transmission electron microscopy (TEM), and Fourier transform infrared (FTIR) spectroscopy. XRD patterns analysis revealed that NPs were formed after calcination, which showed a cubic and hexagonal crystalline structure of (CdO)x (ZnO)1–x NPs. The phase analysis using EDX spectroscopy and FTIR spectroscopy confirmed the presence of Cd and Zn as the original compounds of prepared (CdO)x (ZnO)1–x NP samples. The average particle size of the samples increased from 14 to 33 nm as the concentration of precursor increased from x=0.20 to x=0.80, as observed by TEM results. The surface composition and valance state of the prepared product NPs were determined by X-ray photoelectron spectroscopy (XPS) analyses. Diffuse UV–visible reflectance spectra were used to determine the optical band gap through the Kubelka–Munk equation; the energy band gap was found to decrease for CdO from 2.92 to 2.82 eV and for ZnO from 3.22 to 3.11 eV with increasing x value. Additionally, photoluminescence (PL) spectra revealed that the intensity in PL increased with an increase in particle size. In addition, the antibacterial activity of binary oxide NP was carried out in vitro against Escherichia coli ATCC 25922 Gram (-ve), Salmonella choleraesuis ATCC 10708, and Bacillus subtilis UPMC 1175 Gram (+ve). This study indicated that the zone of inhibition of 21 mm has good antibacterial activity toward the Gram-positive B. subtilis UPMC 1175. Dove Medical Press 2017 Article PeerReviewed text en http://psasir.upm.edu.my/id/eprint/61519/1/Down-top%20nanofabrication%20of%20binary%20%28CdO%29x%20%28ZnO%291%E2%80%93x%20nanoparticles%20and%20their%20antibacterial%20activity.pdf Al-Hada, Naif Mohammed and Mohamed Kamari, Halimah and Che Abdullah, Che Azurahanim and Saion, Elias and Shaari, Abdul Halim and Talib, Zainal Abidin and Matori, Khamirul Amin (2017) Down-top nanofabrication of binary (CdO)x (ZnO)1–x nanoparticles and their antibacterial activity. International Journal of Nanomedicine, 2017 (12). 8309 - 8323. ISSN 1176-9114; ESSN: 1178-2013 https://www.dovepress.com/down-top-nanofabrication-of-binary-cdox-zno1-x-nanoparticles-and-their-peer-reviewed-fulltext-article-IJN 10.2147/IJN.S150405
spellingShingle Al-Hada, Naif Mohammed
Mohamed Kamari, Halimah
Che Abdullah, Che Azurahanim
Saion, Elias
Shaari, Abdul Halim
Talib, Zainal Abidin
Matori, Khamirul Amin
Down-top nanofabrication of binary (CdO)x (ZnO)1–x nanoparticles and their antibacterial activity
title Down-top nanofabrication of binary (CdO)x (ZnO)1–x nanoparticles and their antibacterial activity
title_full Down-top nanofabrication of binary (CdO)x (ZnO)1–x nanoparticles and their antibacterial activity
title_fullStr Down-top nanofabrication of binary (CdO)x (ZnO)1–x nanoparticles and their antibacterial activity
title_full_unstemmed Down-top nanofabrication of binary (CdO)x (ZnO)1–x nanoparticles and their antibacterial activity
title_short Down-top nanofabrication of binary (CdO)x (ZnO)1–x nanoparticles and their antibacterial activity
title_sort down-top nanofabrication of binary (cdo)x (zno)1–x nanoparticles and their antibacterial activity
url http://psasir.upm.edu.my/id/eprint/61519/
http://psasir.upm.edu.my/id/eprint/61519/
http://psasir.upm.edu.my/id/eprint/61519/
http://psasir.upm.edu.my/id/eprint/61519/1/Down-top%20nanofabrication%20of%20binary%20%28CdO%29x%20%28ZnO%291%E2%80%93x%20nanoparticles%20and%20their%20antibacterial%20activity.pdf