Synthesis, characterization and biological studies of S- benzyl-b-N-(benzoyl)dithiocarbazate and its metal complexes

S-Benzyl-b-N-(benzoyl) dithiocarbazate (SBNBODTC) a new disubstituted dithio-carbazate oxygen–sulfur (OS) donor ligand derived from reaction of S-benzyl dithiocarbazate with benzoyl chloride, formed bischelated complexes of general formula [M(OS)2] where M is Cu2+, Ni2+, Cd2+, Co2+ or Pb2+ and OS is...

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Main Authors: How, Fiona Ni Foong, Crouse, Karen Anne, Mohamed Tahir, Mohamed Ibrahim, Tarafder, Md. Tofassa Hossain, Cowley, Andrew R.
Format: Article
Language:English
English
Published: Elsevier 2008
Online Access:http://psasir.upm.edu.my/id/eprint/5690/
http://psasir.upm.edu.my/id/eprint/5690/1/Synthesis.pdf
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author How, Fiona Ni Foong
Crouse, Karen Anne
Mohamed Tahir, Mohamed Ibrahim
Tarafder, Md. Tofassa Hossain
Cowley, Andrew R.
author_facet How, Fiona Ni Foong
Crouse, Karen Anne
Mohamed Tahir, Mohamed Ibrahim
Tarafder, Md. Tofassa Hossain
Cowley, Andrew R.
author_sort How, Fiona Ni Foong
building UPM Institutional Repository
collection Online Access
description S-Benzyl-b-N-(benzoyl) dithiocarbazate (SBNBODTC) a new disubstituted dithio-carbazate oxygen–sulfur (OS) donor ligand derived from reaction of S-benzyl dithiocarbazate with benzoyl chloride, formed bischelated complexes of general formula [M(OS)2] where M is Cu2+, Ni2+, Cd2+, Co2+ or Pb2+ and OS is a uninegative bidentate ligand. The ligand and its metal complexes have been characterized by a variety of physico-chemical techniques. S-benzyl-b-N-(benzoyl) dithiocarbazate crystallized with Z0 = 2 in its thione form in cis–cis conformation, with the N–N bond adopting a cis geometry with respect to C@S, while the S-benzyl group adopts a cis geometry with respect to the thione sulfur atom across the C–S bond.SBNBODTC, Cu(OS)2, Ni(OS)2 and Pb(OS)2 display marked cytotoxicity against HL-60 (human myeloid leukemia)while Cd(OS)2 and Co(OS)2 are moderately cytotoxic. The compounds showed moderate but selective activity towards targeted pathogens.
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spelling upm-56902015-09-17T01:33:10Z http://psasir.upm.edu.my/id/eprint/5690/ Synthesis, characterization and biological studies of S- benzyl-b-N-(benzoyl)dithiocarbazate and its metal complexes How, Fiona Ni Foong Crouse, Karen Anne Mohamed Tahir, Mohamed Ibrahim Tarafder, Md. Tofassa Hossain Cowley, Andrew R. S-Benzyl-b-N-(benzoyl) dithiocarbazate (SBNBODTC) a new disubstituted dithio-carbazate oxygen–sulfur (OS) donor ligand derived from reaction of S-benzyl dithiocarbazate with benzoyl chloride, formed bischelated complexes of general formula [M(OS)2] where M is Cu2+, Ni2+, Cd2+, Co2+ or Pb2+ and OS is a uninegative bidentate ligand. The ligand and its metal complexes have been characterized by a variety of physico-chemical techniques. S-benzyl-b-N-(benzoyl) dithiocarbazate crystallized with Z0 = 2 in its thione form in cis–cis conformation, with the N–N bond adopting a cis geometry with respect to C@S, while the S-benzyl group adopts a cis geometry with respect to the thione sulfur atom across the C–S bond.SBNBODTC, Cu(OS)2, Ni(OS)2 and Pb(OS)2 display marked cytotoxicity against HL-60 (human myeloid leukemia)while Cd(OS)2 and Co(OS)2 are moderately cytotoxic. The compounds showed moderate but selective activity towards targeted pathogens. Elsevier 2008 Article PeerReviewed application/pdf en http://psasir.upm.edu.my/id/eprint/5690/1/Synthesis.pdf How, Fiona Ni Foong and Crouse, Karen Anne and Mohamed Tahir, Mohamed Ibrahim and Tarafder, Md. Tofassa Hossain and Cowley, Andrew R. (2008) Synthesis, characterization and biological studies of S- benzyl-b-N-(benzoyl)dithiocarbazate and its metal complexes. Polyhedron, 27 (15). pp. 3325-3329. ISSN 0277-5387 http://dx.doi.org/10.1016/j.poly.2008.07.022 10.1016/j.poly.2008.07.022 English
spellingShingle How, Fiona Ni Foong
Crouse, Karen Anne
Mohamed Tahir, Mohamed Ibrahim
Tarafder, Md. Tofassa Hossain
Cowley, Andrew R.
Synthesis, characterization and biological studies of S- benzyl-b-N-(benzoyl)dithiocarbazate and its metal complexes
title Synthesis, characterization and biological studies of S- benzyl-b-N-(benzoyl)dithiocarbazate and its metal complexes
title_full Synthesis, characterization and biological studies of S- benzyl-b-N-(benzoyl)dithiocarbazate and its metal complexes
title_fullStr Synthesis, characterization and biological studies of S- benzyl-b-N-(benzoyl)dithiocarbazate and its metal complexes
title_full_unstemmed Synthesis, characterization and biological studies of S- benzyl-b-N-(benzoyl)dithiocarbazate and its metal complexes
title_short Synthesis, characterization and biological studies of S- benzyl-b-N-(benzoyl)dithiocarbazate and its metal complexes
title_sort synthesis, characterization and biological studies of s- benzyl-b-n-(benzoyl)dithiocarbazate and its metal complexes
url http://psasir.upm.edu.my/id/eprint/5690/
http://psasir.upm.edu.my/id/eprint/5690/
http://psasir.upm.edu.my/id/eprint/5690/
http://psasir.upm.edu.my/id/eprint/5690/1/Synthesis.pdf