Thermogravimetric study of Chlorella vulgaris for syngas production

The present study investigates the thermal degradation behavior of Chlorella vulgaris using a thermogravimetric analyzer (TGA) to explore application as feedstock for syngas production. The biomass was heated continuously from room temperature to 1000 °C at different heating rates (5, 10 and 20 °C m...

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Main Authors: Abdul Raheem, S., Sivasangar, Wan Ab. Karim Ghani, Wan Azlina, Yap, Taufiq Yun Hin, Danquah, Michael K., Harun, Mohd Razif
Format: Article
Language:English
Published: Elsevier 2015
Online Access:http://psasir.upm.edu.my/id/eprint/46728/
http://psasir.upm.edu.my/id/eprint/46728/1/Thermogravimetric%20study%20of%20Chlorella%20vulgaris%20for%20syngas%20production.pdf
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author Abdul Raheem
S., Sivasangar
Wan Ab. Karim Ghani, Wan Azlina
Yap, Taufiq Yun Hin
Danquah, Michael K.
Harun, Mohd Razif
author_facet Abdul Raheem
S., Sivasangar
Wan Ab. Karim Ghani, Wan Azlina
Yap, Taufiq Yun Hin
Danquah, Michael K.
Harun, Mohd Razif
author_sort Abdul Raheem
building UPM Institutional Repository
collection Online Access
description The present study investigates the thermal degradation behavior of Chlorella vulgaris using a thermogravimetric analyzer (TGA) to explore application as feedstock for syngas production. The biomass was heated continuously from room temperature to 1000 °C at different heating rates (5, 10 and 20 °C min− 1) under N2/air conditions at a constant flow rate of 25 mL min− 1. Experimental results showed that the combustion process of C. vulgaris can be divided into three major phases; (1) moisture removal, (2) devolatilization of carbohydrates, protein and lipids and (3) degradation of carbonaceous material. A degradation rate of 80% was obtained at the second phase of the combustion process in the presence of air whilst a degradation rate of 60% was obtained under N2 atmosphere at the same phase. The biomass was further gasified for syngas production using a Temperature Programmed Gasifier (TPG). The effect of three different process variables, temperature, microalgal loading, and heating rate was investigated. The maximum H2 production was found at 800 °C temperature with a biomass loading of 0.5 g. No significant effect of heating rate was observed on H2 production. The activation energy values, based on the Kissinger method, were evaluated to be 45.38 ± 0.5 kJ mol− 1 (1st stage), 61.20 ± 0.5 kJ mol− 1 (2nd stage) and 97.22 ± 0.5 kJ mol− 1 (3rd stage). The results demonstrate a significant potential for the utilization of the microalgae biomass as feedstock for large-scale production of syngas via gasification.
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spelling upm-467282018-04-23T02:08:43Z http://psasir.upm.edu.my/id/eprint/46728/ Thermogravimetric study of Chlorella vulgaris for syngas production Abdul Raheem S., Sivasangar Wan Ab. Karim Ghani, Wan Azlina Yap, Taufiq Yun Hin Danquah, Michael K. Harun, Mohd Razif The present study investigates the thermal degradation behavior of Chlorella vulgaris using a thermogravimetric analyzer (TGA) to explore application as feedstock for syngas production. The biomass was heated continuously from room temperature to 1000 °C at different heating rates (5, 10 and 20 °C min− 1) under N2/air conditions at a constant flow rate of 25 mL min− 1. Experimental results showed that the combustion process of C. vulgaris can be divided into three major phases; (1) moisture removal, (2) devolatilization of carbohydrates, protein and lipids and (3) degradation of carbonaceous material. A degradation rate of 80% was obtained at the second phase of the combustion process in the presence of air whilst a degradation rate of 60% was obtained under N2 atmosphere at the same phase. The biomass was further gasified for syngas production using a Temperature Programmed Gasifier (TPG). The effect of three different process variables, temperature, microalgal loading, and heating rate was investigated. The maximum H2 production was found at 800 °C temperature with a biomass loading of 0.5 g. No significant effect of heating rate was observed on H2 production. The activation energy values, based on the Kissinger method, were evaluated to be 45.38 ± 0.5 kJ mol− 1 (1st stage), 61.20 ± 0.5 kJ mol− 1 (2nd stage) and 97.22 ± 0.5 kJ mol− 1 (3rd stage). The results demonstrate a significant potential for the utilization of the microalgae biomass as feedstock for large-scale production of syngas via gasification. Elsevier 2015-11 Article PeerReviewed text en http://psasir.upm.edu.my/id/eprint/46728/1/Thermogravimetric%20study%20of%20Chlorella%20vulgaris%20for%20syngas%20production.pdf Abdul Raheem and S., Sivasangar and Wan Ab. Karim Ghani, Wan Azlina and Yap, Taufiq Yun Hin and Danquah, Michael K. and Harun, Mohd Razif (2015) Thermogravimetric study of Chlorella vulgaris for syngas production. Algal Research, 12. pp. 52-59. ISSN 2211-9264 http://www.journals.elsevier.com/algal-research/ 10.1016/j.algal.2015.08.003
spellingShingle Abdul Raheem
S., Sivasangar
Wan Ab. Karim Ghani, Wan Azlina
Yap, Taufiq Yun Hin
Danquah, Michael K.
Harun, Mohd Razif
Thermogravimetric study of Chlorella vulgaris for syngas production
title Thermogravimetric study of Chlorella vulgaris for syngas production
title_full Thermogravimetric study of Chlorella vulgaris for syngas production
title_fullStr Thermogravimetric study of Chlorella vulgaris for syngas production
title_full_unstemmed Thermogravimetric study of Chlorella vulgaris for syngas production
title_short Thermogravimetric study of Chlorella vulgaris for syngas production
title_sort thermogravimetric study of chlorella vulgaris for syngas production
url http://psasir.upm.edu.my/id/eprint/46728/
http://psasir.upm.edu.my/id/eprint/46728/
http://psasir.upm.edu.my/id/eprint/46728/
http://psasir.upm.edu.my/id/eprint/46728/1/Thermogravimetric%20study%20of%20Chlorella%20vulgaris%20for%20syngas%20production.pdf