Beta-hydroxy-beta-methylglutaryl coenzyme a hydrolase of rat liver

Beta-Hydroxy-beta-methylglutaryl coenzyme A hydrolase, or deacylase, (EC 3.1.2.5) is important, at least potentially, in the regulation of mammalian cholesterol synthesis. This is so for two reasons, both related to the enzyme generally regarded as rate-limiting for cholesterogenesis, namely beta-hy...

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Main Authors: Sipat, Abdullah, Sabine, John R.
Format: Article
Language:English
Published: Elsevier 1981
Online Access:http://psasir.upm.edu.my/id/eprint/38811/
http://psasir.upm.edu.my/id/eprint/38811/1/a84%20-%20hydroxy%20methyglutar.pdf
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author Sipat, Abdullah
Sabine, John R.
author_facet Sipat, Abdullah
Sabine, John R.
author_sort Sipat, Abdullah
building UPM Institutional Repository
collection Online Access
description Beta-Hydroxy-beta-methylglutaryl coenzyme A hydrolase, or deacylase, (EC 3.1.2.5) is important, at least potentially, in the regulation of mammalian cholesterol synthesis. This is so for two reasons, both related to the enzyme generally regarded as rate-limiting for cholesterogenesis, namely beta-hydroxy-beta-methylglutaryl CoA reductase: (i) the hydrolase competes for the same substrate as the reductase and (ii) its end product, hydroxymethylglutamic acid, is a known inhibitor of the reductase. Consequently we have examined some of the properties of the hydrolase, as found in rat liver, after first developing a simple isotopic technique for its assay. Beta-Hydroxy-beta-methylglutaryl CoA hydrolase is both soluble and microsomal. The microsomal enzyme is inactivated by pre-incubation at 37 degree C, but not a 4 degree C, has an apparent pH optimum of approximately 7.6, and has Km and V values of 270 (microM) and 33.3 (nmol HMG/10 per mg protein), respectively, at 37 degree C. For the cytosolic enzyme the corresponding Km and V values are 830 and 111.1. From our observations it seems unlikely that beta-hydroxy-beta-methylglutaryl CoA hydrolase plays a significant role in the regulation of hepatic cholesterol synthesis since, in contrast to microsomal beta-hydroxy-beta-methylglutaryl coenzyme A reductase, we could find for the microsomal hydrolase no evidence of a diurnal rhythm of activity, no inhibition of activity by short-term cholesterol feeding and no evidence from Arrhenius-plot data for any membrane-mediated control of enzyme activity. Thus, the significance of the enzyme in mammalian systems remains unknown.
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spelling upm-388112015-06-10T00:26:27Z http://psasir.upm.edu.my/id/eprint/38811/ Beta-hydroxy-beta-methylglutaryl coenzyme a hydrolase of rat liver Sipat, Abdullah Sabine, John R. Beta-Hydroxy-beta-methylglutaryl coenzyme A hydrolase, or deacylase, (EC 3.1.2.5) is important, at least potentially, in the regulation of mammalian cholesterol synthesis. This is so for two reasons, both related to the enzyme generally regarded as rate-limiting for cholesterogenesis, namely beta-hydroxy-beta-methylglutaryl CoA reductase: (i) the hydrolase competes for the same substrate as the reductase and (ii) its end product, hydroxymethylglutamic acid, is a known inhibitor of the reductase. Consequently we have examined some of the properties of the hydrolase, as found in rat liver, after first developing a simple isotopic technique for its assay. Beta-Hydroxy-beta-methylglutaryl CoA hydrolase is both soluble and microsomal. The microsomal enzyme is inactivated by pre-incubation at 37 degree C, but not a 4 degree C, has an apparent pH optimum of approximately 7.6, and has Km and V values of 270 (microM) and 33.3 (nmol HMG/10 per mg protein), respectively, at 37 degree C. For the cytosolic enzyme the corresponding Km and V values are 830 and 111.1. From our observations it seems unlikely that beta-hydroxy-beta-methylglutaryl CoA hydrolase plays a significant role in the regulation of hepatic cholesterol synthesis since, in contrast to microsomal beta-hydroxy-beta-methylglutaryl coenzyme A reductase, we could find for the microsomal hydrolase no evidence of a diurnal rhythm of activity, no inhibition of activity by short-term cholesterol feeding and no evidence from Arrhenius-plot data for any membrane-mediated control of enzyme activity. Thus, the significance of the enzyme in mammalian systems remains unknown. Elsevier 1981-10-23 Article PeerReviewed application/pdf en http://psasir.upm.edu.my/id/eprint/38811/1/a84%20-%20hydroxy%20methyglutar.pdf Sipat, Abdullah and Sabine, John R. (1981) Beta-hydroxy-beta-methylglutaryl coenzyme a hydrolase of rat liver. Biochimica et Biophysica Acta, 666 (1). pp. 181-190. ISSN 0304-4165; ESSN: 1872-8006
spellingShingle Sipat, Abdullah
Sabine, John R.
Beta-hydroxy-beta-methylglutaryl coenzyme a hydrolase of rat liver
title Beta-hydroxy-beta-methylglutaryl coenzyme a hydrolase of rat liver
title_full Beta-hydroxy-beta-methylglutaryl coenzyme a hydrolase of rat liver
title_fullStr Beta-hydroxy-beta-methylglutaryl coenzyme a hydrolase of rat liver
title_full_unstemmed Beta-hydroxy-beta-methylglutaryl coenzyme a hydrolase of rat liver
title_short Beta-hydroxy-beta-methylglutaryl coenzyme a hydrolase of rat liver
title_sort beta-hydroxy-beta-methylglutaryl coenzyme a hydrolase of rat liver
url http://psasir.upm.edu.my/id/eprint/38811/
http://psasir.upm.edu.my/id/eprint/38811/1/a84%20-%20hydroxy%20methyglutar.pdf