Synthesis and reactivities of triphenyl acetamide analogs for potential nonlinear optical material uses

We have synthesized aniline based amides (3a–h) via palladium catalyzed Suzuki cross coupling of N-(2,5-dibromophenyl) acetamide with different arylboronic acids in moderate to good yields. A variety of functional groups were well tolerated in reaction conditions. For exploring the possible applicat...

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Main Authors: Israr, Hira, Rasool, Nasir, Rizwan, Komal, Hashmi, Muhammad Ali, Mahmood, Tariq, Rashid, Umer, Hussein, Mohd Zobir, Akhtar, Muhammad Nadeem
Format: Article
Language:English
Published: MDPI 2019
Online Access:http://psasir.upm.edu.my/id/eprint/38377/
http://psasir.upm.edu.my/id/eprint/38377/1/38377.pdf
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author Israr, Hira
Rasool, Nasir
Rizwan, Komal
Hashmi, Muhammad Ali
Mahmood, Tariq
Rashid, Umer
Hussein, Mohd Zobir
Akhtar, Muhammad Nadeem
author_facet Israr, Hira
Rasool, Nasir
Rizwan, Komal
Hashmi, Muhammad Ali
Mahmood, Tariq
Rashid, Umer
Hussein, Mohd Zobir
Akhtar, Muhammad Nadeem
author_sort Israr, Hira
building UPM Institutional Repository
collection Online Access
description We have synthesized aniline based amides (3a–h) via palladium catalyzed Suzuki cross coupling of N-(2,5-dibromophenyl) acetamide with different arylboronic acids in moderate to good yields. A variety of functional groups were well tolerated in reaction conditions. For exploring the possible applications as optoelectronic devices, the nonlinear optical (NLO) properties of all synthesized derivatives (3a–h) were investigated with the help of density functional theory (DFT) methods. The frontier molecular orbitals analysis and reactivity descriptors were investigated for exploring the reactivities.
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institution Universiti Putra Malaysia
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language English
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publishDate 2019
publisher MDPI
recordtype eprints
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spelling upm-383772020-05-04T16:25:29Z http://psasir.upm.edu.my/id/eprint/38377/ Synthesis and reactivities of triphenyl acetamide analogs for potential nonlinear optical material uses Israr, Hira Rasool, Nasir Rizwan, Komal Hashmi, Muhammad Ali Mahmood, Tariq Rashid, Umer Hussein, Mohd Zobir Akhtar, Muhammad Nadeem We have synthesized aniline based amides (3a–h) via palladium catalyzed Suzuki cross coupling of N-(2,5-dibromophenyl) acetamide with different arylboronic acids in moderate to good yields. A variety of functional groups were well tolerated in reaction conditions. For exploring the possible applications as optoelectronic devices, the nonlinear optical (NLO) properties of all synthesized derivatives (3a–h) were investigated with the help of density functional theory (DFT) methods. The frontier molecular orbitals analysis and reactivity descriptors were investigated for exploring the reactivities. MDPI 2019 Article PeerReviewed text en http://psasir.upm.edu.my/id/eprint/38377/1/38377.pdf Israr, Hira and Rasool, Nasir and Rizwan, Komal and Hashmi, Muhammad Ali and Mahmood, Tariq and Rashid, Umer and Hussein, Mohd Zobir and Akhtar, Muhammad Nadeem (2019) Synthesis and reactivities of triphenyl acetamide analogs for potential nonlinear optical material uses. Symmetry, 11 (5). art. no. 622. pp. 1-11. ISSN 2073-8994 https://www.mdpi.com/2073-8994/11/5/622 10.3390/sym11050622
spellingShingle Israr, Hira
Rasool, Nasir
Rizwan, Komal
Hashmi, Muhammad Ali
Mahmood, Tariq
Rashid, Umer
Hussein, Mohd Zobir
Akhtar, Muhammad Nadeem
Synthesis and reactivities of triphenyl acetamide analogs for potential nonlinear optical material uses
title Synthesis and reactivities of triphenyl acetamide analogs for potential nonlinear optical material uses
title_full Synthesis and reactivities of triphenyl acetamide analogs for potential nonlinear optical material uses
title_fullStr Synthesis and reactivities of triphenyl acetamide analogs for potential nonlinear optical material uses
title_full_unstemmed Synthesis and reactivities of triphenyl acetamide analogs for potential nonlinear optical material uses
title_short Synthesis and reactivities of triphenyl acetamide analogs for potential nonlinear optical material uses
title_sort synthesis and reactivities of triphenyl acetamide analogs for potential nonlinear optical material uses
url http://psasir.upm.edu.my/id/eprint/38377/
http://psasir.upm.edu.my/id/eprint/38377/
http://psasir.upm.edu.my/id/eprint/38377/
http://psasir.upm.edu.my/id/eprint/38377/1/38377.pdf