Bis{(Z)-[(E)-2-(pyridin-2-ylmethylidene)hydrazin-1-ylidene][(pyridin-2-yl) methylsulfanyl]methanethiolato}nickel(II)

The title compound, [Ni(C13H11N4S 2)2], was obtained by the reaction of S-2- picolyldithiocarbazate and pyridine-2-carbaldehyde with nickel(II) acetate. The NiII atom is located on a twofold rotation axis and is bonded to four N atoms at distances of 2.037 (8) and 2.109 (9) Å, and to two S atoms at...

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Main Authors: Khoo, Teng Jin, Break, Mohammed Khaled, Mohamed Tahir, Mohamed Ibrahim, Crouse, Karen Anne, Cowley, Andrew R., Watkin, David J.
Format: Article
Language:English
English
Published: International Union of Crystallography 2013
Online Access:http://psasir.upm.edu.my/id/eprint/30096/
http://psasir.upm.edu.my/id/eprint/30096/1/Bis.pdf
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author Khoo, Teng Jin
Break, Mohammed Khaled
Mohamed Tahir, Mohamed Ibrahim
Crouse, Karen Anne
Cowley, Andrew R.
Watkin, David J.
author_facet Khoo, Teng Jin
Break, Mohammed Khaled
Mohamed Tahir, Mohamed Ibrahim
Crouse, Karen Anne
Cowley, Andrew R.
Watkin, David J.
author_sort Khoo, Teng Jin
building UPM Institutional Repository
collection Online Access
description The title compound, [Ni(C13H11N4S 2)2], was obtained by the reaction of S-2- picolyldithiocarbazate and pyridine-2-carbaldehyde with nickel(II) acetate. The NiII atom is located on a twofold rotation axis and is bonded to four N atoms at distances of 2.037 (8) and 2.109 (9) Å, and to two S atoms at a distance of 2.406 (3) Å, leading to a distorted octahedral coordination. The angle between the mean planes of the coordinating moieties of the two symmetry-related tridentate ligands is 83.3 (2)°. In the crystal, complex molecules are linked by weak C - H⋯S hydrogen bonds, π-π interactions between the pyridine rings [centroid-centroid distance = 3.775 (9) Å] and C - H⋯π interactions. The hydrogen-bonding interactions lead to the formation of layers parallel to (010); π-π interactions link these layers into a three-dimensional network.
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language English
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publishDate 2013
publisher International Union of Crystallography
recordtype eprints
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spelling upm-300962015-09-18T02:13:31Z http://psasir.upm.edu.my/id/eprint/30096/ Bis{(Z)-[(E)-2-(pyridin-2-ylmethylidene)hydrazin-1-ylidene][(pyridin-2-yl) methylsulfanyl]methanethiolato}nickel(II) Khoo, Teng Jin Break, Mohammed Khaled Mohamed Tahir, Mohamed Ibrahim Crouse, Karen Anne Cowley, Andrew R. Watkin, David J. The title compound, [Ni(C13H11N4S 2)2], was obtained by the reaction of S-2- picolyldithiocarbazate and pyridine-2-carbaldehyde with nickel(II) acetate. The NiII atom is located on a twofold rotation axis and is bonded to four N atoms at distances of 2.037 (8) and 2.109 (9) Å, and to two S atoms at a distance of 2.406 (3) Å, leading to a distorted octahedral coordination. The angle between the mean planes of the coordinating moieties of the two symmetry-related tridentate ligands is 83.3 (2)°. In the crystal, complex molecules are linked by weak C - H⋯S hydrogen bonds, π-π interactions between the pyridine rings [centroid-centroid distance = 3.775 (9) Å] and C - H⋯π interactions. The hydrogen-bonding interactions lead to the formation of layers parallel to (010); π-π interactions link these layers into a three-dimensional network. International Union of Crystallography 2013 Article PeerReviewed application/pdf en http://psasir.upm.edu.my/id/eprint/30096/1/Bis.pdf Khoo, Teng Jin and Break, Mohammed Khaled and Mohamed Tahir, Mohamed Ibrahim and Crouse, Karen Anne and Cowley, Andrew R. and Watkin, David J. (2013) Bis{(Z)-[(E)-2-(pyridin-2-ylmethylidene)hydrazin-1-ylidene][(pyridin-2-yl) methylsulfanyl]methanethiolato}nickel(II). Acta Crystallographica Section E: Structure Reports Online, 69 (pt.6). m323-m324. ISSN 1600-5368 10.1107/S1600536813013032 English
spellingShingle Khoo, Teng Jin
Break, Mohammed Khaled
Mohamed Tahir, Mohamed Ibrahim
Crouse, Karen Anne
Cowley, Andrew R.
Watkin, David J.
Bis{(Z)-[(E)-2-(pyridin-2-ylmethylidene)hydrazin-1-ylidene][(pyridin-2-yl) methylsulfanyl]methanethiolato}nickel(II)
title Bis{(Z)-[(E)-2-(pyridin-2-ylmethylidene)hydrazin-1-ylidene][(pyridin-2-yl) methylsulfanyl]methanethiolato}nickel(II)
title_full Bis{(Z)-[(E)-2-(pyridin-2-ylmethylidene)hydrazin-1-ylidene][(pyridin-2-yl) methylsulfanyl]methanethiolato}nickel(II)
title_fullStr Bis{(Z)-[(E)-2-(pyridin-2-ylmethylidene)hydrazin-1-ylidene][(pyridin-2-yl) methylsulfanyl]methanethiolato}nickel(II)
title_full_unstemmed Bis{(Z)-[(E)-2-(pyridin-2-ylmethylidene)hydrazin-1-ylidene][(pyridin-2-yl) methylsulfanyl]methanethiolato}nickel(II)
title_short Bis{(Z)-[(E)-2-(pyridin-2-ylmethylidene)hydrazin-1-ylidene][(pyridin-2-yl) methylsulfanyl]methanethiolato}nickel(II)
title_sort bis{(z)-[(e)-2-(pyridin-2-ylmethylidene)hydrazin-1-ylidene][(pyridin-2-yl) methylsulfanyl]methanethiolato}nickel(ii)
url http://psasir.upm.edu.my/id/eprint/30096/
http://psasir.upm.edu.my/id/eprint/30096/
http://psasir.upm.edu.my/id/eprint/30096/1/Bis.pdf