Optimization of lipase catalyzed synthesis of Ethyl Valerate, a green apple flavor using Response Surface Methodology (RSM).

Ethyl valerate, a green apple flavor is short-chain ester with fruity notes is widely used in food, cosmetic and pharmaceutical industries. Traditionally, flavor esters are produced by chemical method or extracted by natural sources. However, with the steadily growing demand for natural flavor compo...

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Main Authors: Mat Radzi, Salina, Kamar Muhammad, Syamsul, Othman, Siti Salhah, Abdul Rahman, Mohd Basyaruddin, Mohd. Noor, Hanina
Format: Article
Language:English
English
Published: David Publishing Company 2011
Online Access:http://psasir.upm.edu.my/id/eprint/25064/
http://psasir.upm.edu.my/id/eprint/25064/1/Optimization%20of%20lipase%20catalyzed%20synthesis%20of%20Ethyl%20Valerate.pdf
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author Mat Radzi, Salina
Kamar Muhammad, Syamsul
Othman, Siti Salhah
Abdul Rahman, Mohd Basyaruddin
Mohd. Noor, Hanina
author_facet Mat Radzi, Salina
Kamar Muhammad, Syamsul
Othman, Siti Salhah
Abdul Rahman, Mohd Basyaruddin
Mohd. Noor, Hanina
author_sort Mat Radzi, Salina
building UPM Institutional Repository
collection Online Access
description Ethyl valerate, a green apple flavor is short-chain ester with fruity notes is widely used in food, cosmetic and pharmaceutical industries. Traditionally, flavor esters are produced by chemical method or extracted by natural sources. However, with the steadily growing demand for natural flavor compounds, the biosynthesis of such esters by lipase under mild conditions has been receiving much attention for producing these valuable products. In this study, enzymatic synthesis of ethyl valerate in solvent free system, was successfully optimized via response surface method (RSM) based on 5-level, 4-variable of central composite rotatable design (CCRD). The parameters were reaction time (30-60 min), reaction temperature (30-60 ℃), amount of enzyme (10-25%, w/w) and shaking speed (50-150 rpm). The optimum condition derived via RSM for the reaction was reaction time of 48 min, reaction temperature of 30 ℃, enzyme amount of 25%, (w/w) and shaking speed of 51 rpm. The actual experimental yield was 84.28 % under the optimum condition, which compared well with the maximum predicted value of 84.61%. Comparison of predicted and experimental values reveals good correspondence between them, implying that empirical models derived from RSM can be used to adequately describe the relationship between the factors and response in the synthesis of ethyl valerate.
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language English
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spelling upm-250642015-10-20T00:56:59Z http://psasir.upm.edu.my/id/eprint/25064/ Optimization of lipase catalyzed synthesis of Ethyl Valerate, a green apple flavor using Response Surface Methodology (RSM). Mat Radzi, Salina Kamar Muhammad, Syamsul Othman, Siti Salhah Abdul Rahman, Mohd Basyaruddin Mohd. Noor, Hanina Ethyl valerate, a green apple flavor is short-chain ester with fruity notes is widely used in food, cosmetic and pharmaceutical industries. Traditionally, flavor esters are produced by chemical method or extracted by natural sources. However, with the steadily growing demand for natural flavor compounds, the biosynthesis of such esters by lipase under mild conditions has been receiving much attention for producing these valuable products. In this study, enzymatic synthesis of ethyl valerate in solvent free system, was successfully optimized via response surface method (RSM) based on 5-level, 4-variable of central composite rotatable design (CCRD). The parameters were reaction time (30-60 min), reaction temperature (30-60 ℃), amount of enzyme (10-25%, w/w) and shaking speed (50-150 rpm). The optimum condition derived via RSM for the reaction was reaction time of 48 min, reaction temperature of 30 ℃, enzyme amount of 25%, (w/w) and shaking speed of 51 rpm. The actual experimental yield was 84.28 % under the optimum condition, which compared well with the maximum predicted value of 84.61%. Comparison of predicted and experimental values reveals good correspondence between them, implying that empirical models derived from RSM can be used to adequately describe the relationship between the factors and response in the synthesis of ethyl valerate. David Publishing Company 2011 Article PeerReviewed application/pdf en http://psasir.upm.edu.my/id/eprint/25064/1/Optimization%20of%20lipase%20catalyzed%20synthesis%20of%20Ethyl%20Valerate.pdf Mat Radzi, Salina and Kamar Muhammad, Syamsul and Othman, Siti Salhah and Abdul Rahman, Mohd Basyaruddin and Mohd. Noor, Hanina (2011) Optimization of lipase catalyzed synthesis of Ethyl Valerate, a green apple flavor using Response Surface Methodology (RSM). Journal of Environmental Science and Engineering, 5 (-). pp. 146-153. ISSN 1934-8932 http://www.davidpublishing.org/ English
spellingShingle Mat Radzi, Salina
Kamar Muhammad, Syamsul
Othman, Siti Salhah
Abdul Rahman, Mohd Basyaruddin
Mohd. Noor, Hanina
Optimization of lipase catalyzed synthesis of Ethyl Valerate, a green apple flavor using Response Surface Methodology (RSM).
title Optimization of lipase catalyzed synthesis of Ethyl Valerate, a green apple flavor using Response Surface Methodology (RSM).
title_full Optimization of lipase catalyzed synthesis of Ethyl Valerate, a green apple flavor using Response Surface Methodology (RSM).
title_fullStr Optimization of lipase catalyzed synthesis of Ethyl Valerate, a green apple flavor using Response Surface Methodology (RSM).
title_full_unstemmed Optimization of lipase catalyzed synthesis of Ethyl Valerate, a green apple flavor using Response Surface Methodology (RSM).
title_short Optimization of lipase catalyzed synthesis of Ethyl Valerate, a green apple flavor using Response Surface Methodology (RSM).
title_sort optimization of lipase catalyzed synthesis of ethyl valerate, a green apple flavor using response surface methodology (rsm).
url http://psasir.upm.edu.my/id/eprint/25064/
http://psasir.upm.edu.my/id/eprint/25064/
http://psasir.upm.edu.my/id/eprint/25064/1/Optimization%20of%20lipase%20catalyzed%20synthesis%20of%20Ethyl%20Valerate.pdf