Synthesis and characterization of a molecularly imprinted polymer for 2,4-Dinitrophenol uptake using 4-Vinylbenzoic acid as the complexing monomer.

A new technique for analysis of 2,4-dinitrophenol in water at low concentration is proposed based on a molecular imprinted polymer. Molecular imprinted polymer (MIP) is cross linked polymeric materials that exhibit high binding capacity and selectivity towards target molecules (template) purposely p...

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Main Authors: Zakaria, Nor Dyana, Yusof, Nor Azah, Haron, Jelas, Abdullah, Abdul Halim
Format: Article
Language:English
English
Published: Chemical Publishing Co. 2011
Online Access:http://psasir.upm.edu.my/id/eprint/24881/
http://psasir.upm.edu.my/id/eprint/24881/1/Synthesis%20and%20characterization%20of%20a%20molecularly%20imprinted%20polymer%20for%202.pdf
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author Zakaria, Nor Dyana
Yusof, Nor Azah
Haron, Jelas
Abdullah, Abdul Halim
author_facet Zakaria, Nor Dyana
Yusof, Nor Azah
Haron, Jelas
Abdullah, Abdul Halim
author_sort Zakaria, Nor Dyana
building UPM Institutional Repository
collection Online Access
description A new technique for analysis of 2,4-dinitrophenol in water at low concentration is proposed based on a molecular imprinted polymer. Molecular imprinted polymer (MIP) is cross linked polymeric materials that exhibit high binding capacity and selectivity towards target molecules (template) purposely present during the synthesis process. The molecular imprinted polymer was prepared in bulk, radical polymerization method using 2,4-dinitrophenol, 4-vinylbenzoic acid, ethylene glycol dimethacrylate and benzoyl peroxide as template, functional monomer, cross-linker and initiator, respectively. Adsorption process for removal of nitrophenol by molecular imprinted polymer was evaluated under various conditions to determine the effect of pH, adsorption kinetics, the isotherm and its selectivity. The maximum adsorption of 2,4- dinitrophenol was 2.50 mg/g. The adsorption of 2,4-dinitrophenol by 4-vinylbenzoic acid was found most effective at pH 5.0. Kinetics study showed that 2,4-dinitrophenol adsorption was modeled by second order kinetic. Adsorption isotherm data could be interpreted using the Langmuir equation.
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institution Universiti Putra Malaysia
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language English
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publishDate 2011
publisher Chemical Publishing Co.
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spelling upm-248812015-11-23T02:21:49Z http://psasir.upm.edu.my/id/eprint/24881/ Synthesis and characterization of a molecularly imprinted polymer for 2,4-Dinitrophenol uptake using 4-Vinylbenzoic acid as the complexing monomer. Zakaria, Nor Dyana Yusof, Nor Azah Haron, Jelas Abdullah, Abdul Halim A new technique for analysis of 2,4-dinitrophenol in water at low concentration is proposed based on a molecular imprinted polymer. Molecular imprinted polymer (MIP) is cross linked polymeric materials that exhibit high binding capacity and selectivity towards target molecules (template) purposely present during the synthesis process. The molecular imprinted polymer was prepared in bulk, radical polymerization method using 2,4-dinitrophenol, 4-vinylbenzoic acid, ethylene glycol dimethacrylate and benzoyl peroxide as template, functional monomer, cross-linker and initiator, respectively. Adsorption process for removal of nitrophenol by molecular imprinted polymer was evaluated under various conditions to determine the effect of pH, adsorption kinetics, the isotherm and its selectivity. The maximum adsorption of 2,4- dinitrophenol was 2.50 mg/g. The adsorption of 2,4-dinitrophenol by 4-vinylbenzoic acid was found most effective at pH 5.0. Kinetics study showed that 2,4-dinitrophenol adsorption was modeled by second order kinetic. Adsorption isotherm data could be interpreted using the Langmuir equation. Chemical Publishing Co. 2011 Article PeerReviewed application/pdf en http://psasir.upm.edu.my/id/eprint/24881/1/Synthesis%20and%20characterization%20of%20a%20molecularly%20imprinted%20polymer%20for%202.pdf Zakaria, Nor Dyana and Yusof, Nor Azah and Haron, Jelas and Abdullah, Abdul Halim (2011) Synthesis and characterization of a molecularly imprinted polymer for 2,4-Dinitrophenol uptake using 4-Vinylbenzoic acid as the complexing monomer. Asian Journal of Chemistry, 23 (6). pp. 2456-2460. ISSN 0970-7077 http://www.chemical-publishing.com/ English
spellingShingle Zakaria, Nor Dyana
Yusof, Nor Azah
Haron, Jelas
Abdullah, Abdul Halim
Synthesis and characterization of a molecularly imprinted polymer for 2,4-Dinitrophenol uptake using 4-Vinylbenzoic acid as the complexing monomer.
title Synthesis and characterization of a molecularly imprinted polymer for 2,4-Dinitrophenol uptake using 4-Vinylbenzoic acid as the complexing monomer.
title_full Synthesis and characterization of a molecularly imprinted polymer for 2,4-Dinitrophenol uptake using 4-Vinylbenzoic acid as the complexing monomer.
title_fullStr Synthesis and characterization of a molecularly imprinted polymer for 2,4-Dinitrophenol uptake using 4-Vinylbenzoic acid as the complexing monomer.
title_full_unstemmed Synthesis and characterization of a molecularly imprinted polymer for 2,4-Dinitrophenol uptake using 4-Vinylbenzoic acid as the complexing monomer.
title_short Synthesis and characterization of a molecularly imprinted polymer for 2,4-Dinitrophenol uptake using 4-Vinylbenzoic acid as the complexing monomer.
title_sort synthesis and characterization of a molecularly imprinted polymer for 2,4-dinitrophenol uptake using 4-vinylbenzoic acid as the complexing monomer.
url http://psasir.upm.edu.my/id/eprint/24881/
http://psasir.upm.edu.my/id/eprint/24881/
http://psasir.upm.edu.my/id/eprint/24881/1/Synthesis%20and%20characterization%20of%20a%20molecularly%20imprinted%20polymer%20for%202.pdf