Biocatalytic production of lactose ester catalysed by mica-based immobilised lipase

Enzyme immobilisation technology is an effective means to improve sugar ester production through the employment of biocatalysts. In the present study, immobilisation of Candida rugosa (CRL) lipase onto amino-activated mica is performed via covalent bonding (namely Amino-CRL) and the cross-linking of...

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Main Authors: Zaidan, Uswatun Hasanah, Abdul Rahman, Mohd Basyaruddin, Othman, Siti Salhah, Basri, Mahiran, Abd. Malek, Emilia, Raja Abdul Rahman, Raja Noor Zaliha, Salleh, Abu Bakar
Format: Article
Language:English
Published: Elsevier 2012
Online Access:http://psasir.upm.edu.my/id/eprint/22360/
http://psasir.upm.edu.my/id/eprint/22360/1/Biocatalytic%20production%20of%20lactose%20ester%20catalysed%20by%20mica.pdf
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author Zaidan, Uswatun Hasanah
Abdul Rahman, Mohd Basyaruddin
Othman, Siti Salhah
Basri, Mahiran
Abd. Malek, Emilia
Raja Abdul Rahman, Raja Noor Zaliha
Salleh, Abu Bakar
author_facet Zaidan, Uswatun Hasanah
Abdul Rahman, Mohd Basyaruddin
Othman, Siti Salhah
Basri, Mahiran
Abd. Malek, Emilia
Raja Abdul Rahman, Raja Noor Zaliha
Salleh, Abu Bakar
author_sort Zaidan, Uswatun Hasanah
building UPM Institutional Repository
collection Online Access
description Enzyme immobilisation technology is an effective means to improve sugar ester production through the employment of biocatalysts. In the present study, immobilisation of Candida rugosa (CRL) lipase onto amino-activated mica is performed via covalent bonding (namely Amino-CRL) and the cross-linking of lipases into nano-reactors through physical adsorption (namely NER-CRL). Free and immobilised lipases were tested for their esterification activities. Specific activities for Amino-CRL and NER-CRL increased by 2.4 and 2.6-fold, respectively, upon immobilisation. Extending this work, immobilised lipases have novel capabilities in the synthesis of sugar esters. The optimised conditions for sugar fatty acid ester syntheses are 48 h at 2:1 of molar ratio of lactose sugar to capric acid at 55 °C. Furthermore, a high operational stability with half-lives of over 13 and 10 runs was achieved for NER-CRL and Amino-CRL, respectively, indicating the efficiency of the immobilisation process.
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spelling upm-223602016-09-26T07:01:53Z http://psasir.upm.edu.my/id/eprint/22360/ Biocatalytic production of lactose ester catalysed by mica-based immobilised lipase Zaidan, Uswatun Hasanah Abdul Rahman, Mohd Basyaruddin Othman, Siti Salhah Basri, Mahiran Abd. Malek, Emilia Raja Abdul Rahman, Raja Noor Zaliha Salleh, Abu Bakar Enzyme immobilisation technology is an effective means to improve sugar ester production through the employment of biocatalysts. In the present study, immobilisation of Candida rugosa (CRL) lipase onto amino-activated mica is performed via covalent bonding (namely Amino-CRL) and the cross-linking of lipases into nano-reactors through physical adsorption (namely NER-CRL). Free and immobilised lipases were tested for their esterification activities. Specific activities for Amino-CRL and NER-CRL increased by 2.4 and 2.6-fold, respectively, upon immobilisation. Extending this work, immobilised lipases have novel capabilities in the synthesis of sugar esters. The optimised conditions for sugar fatty acid ester syntheses are 48 h at 2:1 of molar ratio of lactose sugar to capric acid at 55 °C. Furthermore, a high operational stability with half-lives of over 13 and 10 runs was achieved for NER-CRL and Amino-CRL, respectively, indicating the efficiency of the immobilisation process. Elsevier 2012-03-01 Article PeerReviewed application/pdf en http://psasir.upm.edu.my/id/eprint/22360/1/Biocatalytic%20production%20of%20lactose%20ester%20catalysed%20by%20mica.pdf Zaidan, Uswatun Hasanah and Abdul Rahman, Mohd Basyaruddin and Othman, Siti Salhah and Basri, Mahiran and Abd. Malek, Emilia and Raja Abdul Rahman, Raja Noor Zaliha and Salleh, Abu Bakar (2012) Biocatalytic production of lactose ester catalysed by mica-based immobilised lipase. Food Chemistry, 131 (1). pp. 199-205. ISSN 0308-8146; ESSN: 1873-7072 10.1016/j.foodchem.2011.08.060
spellingShingle Zaidan, Uswatun Hasanah
Abdul Rahman, Mohd Basyaruddin
Othman, Siti Salhah
Basri, Mahiran
Abd. Malek, Emilia
Raja Abdul Rahman, Raja Noor Zaliha
Salleh, Abu Bakar
Biocatalytic production of lactose ester catalysed by mica-based immobilised lipase
title Biocatalytic production of lactose ester catalysed by mica-based immobilised lipase
title_full Biocatalytic production of lactose ester catalysed by mica-based immobilised lipase
title_fullStr Biocatalytic production of lactose ester catalysed by mica-based immobilised lipase
title_full_unstemmed Biocatalytic production of lactose ester catalysed by mica-based immobilised lipase
title_short Biocatalytic production of lactose ester catalysed by mica-based immobilised lipase
title_sort biocatalytic production of lactose ester catalysed by mica-based immobilised lipase
url http://psasir.upm.edu.my/id/eprint/22360/
http://psasir.upm.edu.my/id/eprint/22360/
http://psasir.upm.edu.my/id/eprint/22360/1/Biocatalytic%20production%20of%20lactose%20ester%20catalysed%20by%20mica.pdf