Synthesis and characterization of Manganese doped ZnO nanoparticles

Various levels of manganese (Mn)-doped ZnO were synthesized by precipitation method. Characterization was carried out by XRD, TEM, SEM, EDX, BET and the band gap measured by UV-visible reflectance. In the XRD pattern of samples, there is no signature of impurity peaks, which could indicate Mn-...

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Main Authors: Abdollahi, Yadollahi, Abdullah, Abdul Halim, Zainal, Zulkarnain, Yusof, Nor Azah
Format: Article
Language:English
English
Published: 2011
Online Access:http://psasir.upm.edu.my/id/eprint/18784/
http://psasir.upm.edu.my/id/eprint/18784/1/Synthesis%20and%20characterization%20of%20Manganese%20doped%20ZnO%20nanoparticles.pdf
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author Abdollahi, Yadollahi
Abdullah, Abdul Halim
Zainal, Zulkarnain
Yusof, Nor Azah
author_facet Abdollahi, Yadollahi
Abdullah, Abdul Halim
Zainal, Zulkarnain
Yusof, Nor Azah
author_sort Abdollahi, Yadollahi
building UPM Institutional Repository
collection Online Access
description Various levels of manganese (Mn)-doped ZnO were synthesized by precipitation method. Characterization was carried out by XRD, TEM, SEM, EDX, BET and the band gap measured by UV-visible reflectance. In the XRD pattern of samples, there is no signature of impurity peaks, which could indicate Mn-related secondary phases. The EDX show the amount of Mn doped on ZnO is slightly lower than the theoretical value. The SEM of 1% Mn-doped ZnO illustrated that morphology is well ordered, has low aggregation, and homogeneous distribution of particle size. High aggregation is observed, however, in other percentages of Mn-doped ZnO. Results of TEM show that more than 50% of the particles for undoped and Mn-doped ZnO use between 15 and 35 nm, with 1% Mn doped ZnO having the highest percentage (77%). The BET shows that the surface area of synthesized catalyst increases when the weight ratio of manganese increases up to 1% Mn, but decreases thereafter. The band gap of 1% Mn-doped ZnO is 2.2 eV which is smaller than the undoped ZnO band gap. The results of characterization show 1% Mn-doped ZnO has the highest surface area, the lowest particles size and the lowest agglomerate. Moreover the calculated band gap of 1% Mn-doped ZnO is lower than others except 0.5%Mn. Additionally, photodegradation of cresols under visible light showed that 1% Mn-doped ZnO had maximum adsorption and rate of photodegradation. In conclusion 1% Mn doped ZnO is suitable as the best photocatalyst to degrade cresols under visible light irradiation.
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spelling upm-187842015-10-21T03:43:08Z http://psasir.upm.edu.my/id/eprint/18784/ Synthesis and characterization of Manganese doped ZnO nanoparticles Abdollahi, Yadollahi Abdullah, Abdul Halim Zainal, Zulkarnain Yusof, Nor Azah Various levels of manganese (Mn)-doped ZnO were synthesized by precipitation method. Characterization was carried out by XRD, TEM, SEM, EDX, BET and the band gap measured by UV-visible reflectance. In the XRD pattern of samples, there is no signature of impurity peaks, which could indicate Mn-related secondary phases. The EDX show the amount of Mn doped on ZnO is slightly lower than the theoretical value. The SEM of 1% Mn-doped ZnO illustrated that morphology is well ordered, has low aggregation, and homogeneous distribution of particle size. High aggregation is observed, however, in other percentages of Mn-doped ZnO. Results of TEM show that more than 50% of the particles for undoped and Mn-doped ZnO use between 15 and 35 nm, with 1% Mn doped ZnO having the highest percentage (77%). The BET shows that the surface area of synthesized catalyst increases when the weight ratio of manganese increases up to 1% Mn, but decreases thereafter. The band gap of 1% Mn-doped ZnO is 2.2 eV which is smaller than the undoped ZnO band gap. The results of characterization show 1% Mn-doped ZnO has the highest surface area, the lowest particles size and the lowest agglomerate. Moreover the calculated band gap of 1% Mn-doped ZnO is lower than others except 0.5%Mn. Additionally, photodegradation of cresols under visible light showed that 1% Mn-doped ZnO had maximum adsorption and rate of photodegradation. In conclusion 1% Mn doped ZnO is suitable as the best photocatalyst to degrade cresols under visible light irradiation. 2011 Article PeerReviewed application/pdf en http://psasir.upm.edu.my/id/eprint/18784/1/Synthesis%20and%20characterization%20of%20Manganese%20doped%20ZnO%20nanoparticles.pdf Abdollahi, Yadollahi and Abdullah, Abdul Halim and Zainal, Zulkarnain and Yusof, Nor Azah (2011) Synthesis and characterization of Manganese doped ZnO nanoparticles. International Journal of Basic and Applied Sciences, 11 (4). pp. 62-69. http://ijens.org/Vol_11_I_04/118104-7373-IJBAS-IJENS.pdf English
spellingShingle Abdollahi, Yadollahi
Abdullah, Abdul Halim
Zainal, Zulkarnain
Yusof, Nor Azah
Synthesis and characterization of Manganese doped ZnO nanoparticles
title Synthesis and characterization of Manganese doped ZnO nanoparticles
title_full Synthesis and characterization of Manganese doped ZnO nanoparticles
title_fullStr Synthesis and characterization of Manganese doped ZnO nanoparticles
title_full_unstemmed Synthesis and characterization of Manganese doped ZnO nanoparticles
title_short Synthesis and characterization of Manganese doped ZnO nanoparticles
title_sort synthesis and characterization of manganese doped zno nanoparticles
url http://psasir.upm.edu.my/id/eprint/18784/
http://psasir.upm.edu.my/id/eprint/18784/
http://psasir.upm.edu.my/id/eprint/18784/1/Synthesis%20and%20characterization%20of%20Manganese%20doped%20ZnO%20nanoparticles.pdf