Comparative performance of single and binary metal selenides in dye‑sensitized solar cells

Iron selenide (FeSe2), cobalt selenide (Co3Se4), and iron cobalt selenide (FeCo2Se4) have been synthesized via a two-step hydrothermal process. The formation of FeSe2, Co3Se4, and FeCo2Se4 has been proven by sample characterization to support their catalytic activity as the counter electrodes for dy...

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Main Authors: Mohd Noor, Ikhwan Syafiq, Winie, Tan, Najihah, M. Z., Saaid, Farish Irfal, Woo, H. J., Hisam, R.
Format: Article
Language:English
Published: Springer Verlag 2024
Online Access:http://psasir.upm.edu.my/id/eprint/118507/
http://psasir.upm.edu.my/id/eprint/118507/1/118507.pdf
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author Mohd Noor, Ikhwan Syafiq
Winie, Tan
Najihah, M. Z.
Saaid, Farish Irfal
Woo, H. J.
Hisam, R.
author_facet Mohd Noor, Ikhwan Syafiq
Winie, Tan
Najihah, M. Z.
Saaid, Farish Irfal
Woo, H. J.
Hisam, R.
author_sort Mohd Noor, Ikhwan Syafiq
building UPM Institutional Repository
collection Online Access
description Iron selenide (FeSe2), cobalt selenide (Co3Se4), and iron cobalt selenide (FeCo2Se4) have been synthesized via a two-step hydrothermal process. The formation of FeSe2, Co3Se4, and FeCo2Se4 has been proven by sample characterization to support their catalytic activity as the counter electrodes for dye-sensitized solar cells (DSSCs). The poly(vinylidene fuoride-ohexafuoropropylene) (PVdF-HFP)/propylene carbonate (PC)/1,2-dimethoxyethane (DME)/1-methyl-3-propyl imidazolium iodide (MPII)/sodium iodide (NaI)/iodine (I2) gel electrolytes were assembled into DSSCs with FeCo2Se4, FeSe2, Co3Se4, or platinum (Pt) as the counter electrode. The DSSC with FeCo2Se4 counter electrode shows an efciency of 8.55%, whereas Pt counter electrode shows an efciency of 7.06%. The highest performance of DSSC achieved with FeCo2Se4 can be attributed to its highest surface area and pore volume. Hence, FeCo2Se4 can be used as a Pt-free counter electrode for highperformance DSSCs.
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spelling upm-1185072025-08-05T04:35:13Z http://psasir.upm.edu.my/id/eprint/118507/ Comparative performance of single and binary metal selenides in dye‑sensitized solar cells Mohd Noor, Ikhwan Syafiq Winie, Tan Najihah, M. Z. Saaid, Farish Irfal Woo, H. J. Hisam, R. Iron selenide (FeSe2), cobalt selenide (Co3Se4), and iron cobalt selenide (FeCo2Se4) have been synthesized via a two-step hydrothermal process. The formation of FeSe2, Co3Se4, and FeCo2Se4 has been proven by sample characterization to support their catalytic activity as the counter electrodes for dye-sensitized solar cells (DSSCs). The poly(vinylidene fuoride-ohexafuoropropylene) (PVdF-HFP)/propylene carbonate (PC)/1,2-dimethoxyethane (DME)/1-methyl-3-propyl imidazolium iodide (MPII)/sodium iodide (NaI)/iodine (I2) gel electrolytes were assembled into DSSCs with FeCo2Se4, FeSe2, Co3Se4, or platinum (Pt) as the counter electrode. The DSSC with FeCo2Se4 counter electrode shows an efciency of 8.55%, whereas Pt counter electrode shows an efciency of 7.06%. The highest performance of DSSC achieved with FeCo2Se4 can be attributed to its highest surface area and pore volume. Hence, FeCo2Se4 can be used as a Pt-free counter electrode for highperformance DSSCs. Springer Verlag 2024-02-14 Article PeerReviewed text en http://psasir.upm.edu.my/id/eprint/118507/1/118507.pdf Mohd Noor, Ikhwan Syafiq and Winie, Tan and Najihah, M. Z. and Saaid, Farish Irfal and Woo, H. J. and Hisam, R. (2024) Comparative performance of single and binary metal selenides in dye‑sensitized solar cells. Journal of Solid State Electrochemistry, 28 (8). pp. 2703-2713. ISSN 1432-8488; eISSN: 1433-0768 https://link.springer.com/article/10.1007/s10008-024-05835-4 10.1007/s10008-024-05835-4
spellingShingle Mohd Noor, Ikhwan Syafiq
Winie, Tan
Najihah, M. Z.
Saaid, Farish Irfal
Woo, H. J.
Hisam, R.
Comparative performance of single and binary metal selenides in dye‑sensitized solar cells
title Comparative performance of single and binary metal selenides in dye‑sensitized solar cells
title_full Comparative performance of single and binary metal selenides in dye‑sensitized solar cells
title_fullStr Comparative performance of single and binary metal selenides in dye‑sensitized solar cells
title_full_unstemmed Comparative performance of single and binary metal selenides in dye‑sensitized solar cells
title_short Comparative performance of single and binary metal selenides in dye‑sensitized solar cells
title_sort comparative performance of single and binary metal selenides in dye‑sensitized solar cells
url http://psasir.upm.edu.my/id/eprint/118507/
http://psasir.upm.edu.my/id/eprint/118507/
http://psasir.upm.edu.my/id/eprint/118507/
http://psasir.upm.edu.my/id/eprint/118507/1/118507.pdf