Microwave-assisted aging of organic-inorganic hybrid nanocomposite of α-naphthaleneacetate in the lamella of Zn-Al-layered double hydroxide

Microwave-assisted aging Zn-Al-layered double hydroxide with nitrate as the interlayer anion (ZANOL) and its nanohybrid with an organic moiety, α-naphthaleneacetate (ZANAN), was done and the resulting properties of the materials compared. The results showed that intercalation of the α-naphthaleneace...

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Main Authors: Hussein, Mohd Zobir, Zainal, Zulkarnain, Yahaya, Asmah, Vui Foo, Dickens Wong
Format: Article
Published: 2002
Online Access:http://psasir.upm.edu.my/id/eprint/116187/
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author Hussein, Mohd Zobir
Zainal, Zulkarnain
Yahaya, Asmah
Vui Foo, Dickens Wong
author_facet Hussein, Mohd Zobir
Zainal, Zulkarnain
Yahaya, Asmah
Vui Foo, Dickens Wong
author_sort Hussein, Mohd Zobir
building UPM Institutional Repository
collection Online Access
description Microwave-assisted aging Zn-Al-layered double hydroxide with nitrate as the interlayer anion (ZANOL) and its nanohybrid with an organic moiety, α-naphthaleneacetate (ZANAN), was done and the resulting properties of the materials compared. The results showed that intercalation of the α-naphthaleneacetate (NAA) anion into the Zn-Al layered double hydroxide lamella is readily accomplished, resulting in the expansion of the interlayer spacing from 9.0 Å in the layered double hydroxide to 20.0 Å in the nanohybrid. This expansion accommodates the NAA anion of larger size than nitrate, as indicated by its molecular structure. For both methods, the resulting materials afforded a well-ordered organic-inorganic nanolayered structure. The Zn to Al ratio of the resulting nanocomposite is lower than the ratio present in the mother liquor at the beginning of the reaction, which implied less incorporation of aluminum ions from the mother liquor into the inorganic metal hydroxide layers. By using the microwave-assisted method, however, slightly more Al3+ ions were incorporated into the inorganic metal double hydroxide layers. In general, there is not much difference in the physicochemical properties of ZANANs aged by either the microwave or the conventional oil bath method. For both methods, longer aging time slightly enriched the organic content of the resulting nanohybrid and the inorganic Zn to Al ratio remained the same, independent of the aging time.
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spelling upm-1161872025-03-20T03:24:07Z http://psasir.upm.edu.my/id/eprint/116187/ Microwave-assisted aging of organic-inorganic hybrid nanocomposite of α-naphthaleneacetate in the lamella of Zn-Al-layered double hydroxide Hussein, Mohd Zobir Zainal, Zulkarnain Yahaya, Asmah Vui Foo, Dickens Wong Microwave-assisted aging Zn-Al-layered double hydroxide with nitrate as the interlayer anion (ZANOL) and its nanohybrid with an organic moiety, α-naphthaleneacetate (ZANAN), was done and the resulting properties of the materials compared. The results showed that intercalation of the α-naphthaleneacetate (NAA) anion into the Zn-Al layered double hydroxide lamella is readily accomplished, resulting in the expansion of the interlayer spacing from 9.0 Å in the layered double hydroxide to 20.0 Å in the nanohybrid. This expansion accommodates the NAA anion of larger size than nitrate, as indicated by its molecular structure. For both methods, the resulting materials afforded a well-ordered organic-inorganic nanolayered structure. The Zn to Al ratio of the resulting nanocomposite is lower than the ratio present in the mother liquor at the beginning of the reaction, which implied less incorporation of aluminum ions from the mother liquor into the inorganic metal hydroxide layers. By using the microwave-assisted method, however, slightly more Al3+ ions were incorporated into the inorganic metal double hydroxide layers. In general, there is not much difference in the physicochemical properties of ZANANs aged by either the microwave or the conventional oil bath method. For both methods, longer aging time slightly enriched the organic content of the resulting nanohybrid and the inorganic Zn to Al ratio remained the same, independent of the aging time. 2002 Article PeerReviewed Hussein, Mohd Zobir and Zainal, Zulkarnain and Yahaya, Asmah and Vui Foo, Dickens Wong (2002) Microwave-assisted aging of organic-inorganic hybrid nanocomposite of α-naphthaleneacetate in the lamella of Zn-Al-layered double hydroxide. Journal of Materials Synthesis and Processing, 10 (2). pp. 89-95. ISSN 1064-7562; eISSN: 1064-7562 https://link.springer.com/article/10.1023/A:1021283511165?error=cookies_not_supported&code=d873429b-52eb-4157-8ee6-db5a714b5a86 10.1023/A:1021283511165
spellingShingle Hussein, Mohd Zobir
Zainal, Zulkarnain
Yahaya, Asmah
Vui Foo, Dickens Wong
Microwave-assisted aging of organic-inorganic hybrid nanocomposite of α-naphthaleneacetate in the lamella of Zn-Al-layered double hydroxide
title Microwave-assisted aging of organic-inorganic hybrid nanocomposite of α-naphthaleneacetate in the lamella of Zn-Al-layered double hydroxide
title_full Microwave-assisted aging of organic-inorganic hybrid nanocomposite of α-naphthaleneacetate in the lamella of Zn-Al-layered double hydroxide
title_fullStr Microwave-assisted aging of organic-inorganic hybrid nanocomposite of α-naphthaleneacetate in the lamella of Zn-Al-layered double hydroxide
title_full_unstemmed Microwave-assisted aging of organic-inorganic hybrid nanocomposite of α-naphthaleneacetate in the lamella of Zn-Al-layered double hydroxide
title_short Microwave-assisted aging of organic-inorganic hybrid nanocomposite of α-naphthaleneacetate in the lamella of Zn-Al-layered double hydroxide
title_sort microwave-assisted aging of organic-inorganic hybrid nanocomposite of α-naphthaleneacetate in the lamella of zn-al-layered double hydroxide
url http://psasir.upm.edu.my/id/eprint/116187/
http://psasir.upm.edu.my/id/eprint/116187/
http://psasir.upm.edu.my/id/eprint/116187/