Experimental and multiscale analysis of volume fraction effects in tensile properties of recycled PLA-PDA/kenaf fiber 3D printing filament composites

Polylactic acid, a biodegradable thermoplastic derived from renewable sources, has notable environmental advantages and versatile properties. However, recycled PLA often experiences reduced mechanical strength and altered chemical composition due to the recycling process, limiting its suitability fo...

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Main Authors: Hamat, Sanusi, Ishak, M.R., Salit @ Sinon, Mohd Sapuan, Yidris, N., Hussin, M.S., Showkat Ali, S.A., Ibrahim, M.
Format: Article
Language:English
Published: Taylor and Francis 2024
Online Access:http://psasir.upm.edu.my/id/eprint/114649/
http://psasir.upm.edu.my/id/eprint/114649/1/114649.pdf
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author Hamat, Sanusi
Ishak, M.R.
Salit @ Sinon, Mohd Sapuan
Yidris, N.
Hussin, M.S.
Showkat Ali, S.A.
Ibrahim, M.
author_facet Hamat, Sanusi
Ishak, M.R.
Salit @ Sinon, Mohd Sapuan
Yidris, N.
Hussin, M.S.
Showkat Ali, S.A.
Ibrahim, M.
author_sort Hamat, Sanusi
building UPM Institutional Repository
collection Online Access
description Polylactic acid, a biodegradable thermoplastic derived from renewable sources, has notable environmental advantages and versatile properties. However, recycled PLA often experiences reduced mechanical strength and altered chemical composition due to the recycling process, limiting its suitability for 3D printing filament applications. Recognizing the inherent limitations of recycled PLA (rPLA), this research employs a unique method of coating rPLA with dopamine (DA) and reinforcing it with kenaf fibers (KF) at various weight fractions, introducing a novel multiscale modeling approach to address the challenges of interfacial bonding and tensile performance in recycled polymers. The methodology integrates experimental single filament tensile testing with multiscale finite element modeling to accurately predict the composite’s mechanical behavior across different scales. The findings reveal that a 5% kenaf fiber weight/volume fraction provides the optimal balance between tensile strength, stiffness, and toughness, achieving a significant 49.3% improvement over the unreinforced rPLA. However, increasing the kenaf fiber content beyond 5% leads to a decline in mechanical properties, attributed to higher fiber agglomeration and suboptimal fiber-matrix interactions. The novelty of this research lies in its combined use of PDA coating, natural kenaf fiber reinforcement, and advanced multiscale modeling to enhance and predict the performance of rPLA-PDA/kenaf composites, paving the way for sustainable, high-performance materials in 3D printing applications.
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institution Universiti Putra Malaysia
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language English
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publisher Taylor and Francis
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spelling upm-1146492025-01-22T09:07:47Z http://psasir.upm.edu.my/id/eprint/114649/ Experimental and multiscale analysis of volume fraction effects in tensile properties of recycled PLA-PDA/kenaf fiber 3D printing filament composites Hamat, Sanusi Ishak, M.R. Salit @ Sinon, Mohd Sapuan Yidris, N. Hussin, M.S. Showkat Ali, S.A. Ibrahim, M. Polylactic acid, a biodegradable thermoplastic derived from renewable sources, has notable environmental advantages and versatile properties. However, recycled PLA often experiences reduced mechanical strength and altered chemical composition due to the recycling process, limiting its suitability for 3D printing filament applications. Recognizing the inherent limitations of recycled PLA (rPLA), this research employs a unique method of coating rPLA with dopamine (DA) and reinforcing it with kenaf fibers (KF) at various weight fractions, introducing a novel multiscale modeling approach to address the challenges of interfacial bonding and tensile performance in recycled polymers. The methodology integrates experimental single filament tensile testing with multiscale finite element modeling to accurately predict the composite’s mechanical behavior across different scales. The findings reveal that a 5% kenaf fiber weight/volume fraction provides the optimal balance between tensile strength, stiffness, and toughness, achieving a significant 49.3% improvement over the unreinforced rPLA. However, increasing the kenaf fiber content beyond 5% leads to a decline in mechanical properties, attributed to higher fiber agglomeration and suboptimal fiber-matrix interactions. The novelty of this research lies in its combined use of PDA coating, natural kenaf fiber reinforcement, and advanced multiscale modeling to enhance and predict the performance of rPLA-PDA/kenaf composites, paving the way for sustainable, high-performance materials in 3D printing applications. Taylor and Francis 2024 Article PeerReviewed text en http://psasir.upm.edu.my/id/eprint/114649/1/114649.pdf Hamat, Sanusi and Ishak, M.R. and Salit @ Sinon, Mohd Sapuan and Yidris, N. and Hussin, M.S. and Showkat Ali, S.A. and Ibrahim, M. (2024) Experimental and multiscale analysis of volume fraction effects in tensile properties of recycled PLA-PDA/kenaf fiber 3D printing filament composites. Advanced Composite Materials. pp. 1-18. ISSN 0924-3046; eISSN: 1568-5519 (In Press) https://www.tandfonline.com/doi/full/10.1080/09243046.2024.2425468 10.1080/09243046.2024.2425468
spellingShingle Hamat, Sanusi
Ishak, M.R.
Salit @ Sinon, Mohd Sapuan
Yidris, N.
Hussin, M.S.
Showkat Ali, S.A.
Ibrahim, M.
Experimental and multiscale analysis of volume fraction effects in tensile properties of recycled PLA-PDA/kenaf fiber 3D printing filament composites
title Experimental and multiscale analysis of volume fraction effects in tensile properties of recycled PLA-PDA/kenaf fiber 3D printing filament composites
title_full Experimental and multiscale analysis of volume fraction effects in tensile properties of recycled PLA-PDA/kenaf fiber 3D printing filament composites
title_fullStr Experimental and multiscale analysis of volume fraction effects in tensile properties of recycled PLA-PDA/kenaf fiber 3D printing filament composites
title_full_unstemmed Experimental and multiscale analysis of volume fraction effects in tensile properties of recycled PLA-PDA/kenaf fiber 3D printing filament composites
title_short Experimental and multiscale analysis of volume fraction effects in tensile properties of recycled PLA-PDA/kenaf fiber 3D printing filament composites
title_sort experimental and multiscale analysis of volume fraction effects in tensile properties of recycled pla-pda/kenaf fiber 3d printing filament composites
url http://psasir.upm.edu.my/id/eprint/114649/
http://psasir.upm.edu.my/id/eprint/114649/
http://psasir.upm.edu.my/id/eprint/114649/
http://psasir.upm.edu.my/id/eprint/114649/1/114649.pdf