Enhanced properties of TEMPO-oxidized bacterial cellulose films via eco-friendly non-pressurized hot water vapor treatment for sustainable and smart food packaging

Developing a simple and environmentally friendly method to vary the physical, mechanical, and thermal properties of cellulose films is of great importance. This study aimed to characterize 2,2,6,6-tetramethylpiperidinyl-1-oxyl (TEMPO)-oxidized bacterial cellulose (BC) films prepared using non-pressu...

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Main Authors: Rahmadiawan, Dieter, Abral, Hairul, Azka, Muhammad Adlan, Sapuan, S.M., Admi, Ratna Isnanita, Shi, Shih-Chen, Zainul, Rahadian, Azril, None, Zikri, Ahmad, Mahardika, Melbi
Format: Article
Language:English
Published: Royal Society of Chemistry 2024
Online Access:http://psasir.upm.edu.my/id/eprint/114493/
http://psasir.upm.edu.my/id/eprint/114493/1/114493.pdf
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author Rahmadiawan, Dieter
Abral, Hairul
Azka, Muhammad Adlan
Sapuan, S.M.
Admi, Ratna Isnanita
Shi, Shih-Chen
Zainul, Rahadian
Azril, None
Zikri, Ahmad
Mahardika, Melbi
author_facet Rahmadiawan, Dieter
Abral, Hairul
Azka, Muhammad Adlan
Sapuan, S.M.
Admi, Ratna Isnanita
Shi, Shih-Chen
Zainul, Rahadian
Azril, None
Zikri, Ahmad
Mahardika, Melbi
author_sort Rahmadiawan, Dieter
building UPM Institutional Repository
collection Online Access
description Developing a simple and environmentally friendly method to vary the physical, mechanical, and thermal properties of cellulose films is of great importance. This study aimed to characterize 2,2,6,6-tetramethylpiperidinyl-1-oxyl (TEMPO)-oxidized bacterial cellulose (BC) films prepared using non-pressurized hot water vapor (NPHWV) method. A wet BC-pellicle that had been oxidized with TEMPO was treated with NPHWV for 60, 120, and 240 minutes, respectively. As a control, a TEMPO-oxidized BC (TOBC) film without NPHWV was prepared. The results show that the longer NPHWV duration of the TOBC film increased the tensile and thermal properties. This film became more hydrophobic and showed lower moisture absorption, thermal conductivity and organic solvent uptake, more crystalline structure, and higher fiber density after NPHWV treatment. The acquired results provide a simple, inexpensive, and ecologically friendly method for varying TOBC film properties.
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institution Universiti Putra Malaysia
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language English
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publisher Royal Society of Chemistry
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spelling upm-1144932025-01-16T03:41:09Z http://psasir.upm.edu.my/id/eprint/114493/ Enhanced properties of TEMPO-oxidized bacterial cellulose films via eco-friendly non-pressurized hot water vapor treatment for sustainable and smart food packaging Rahmadiawan, Dieter Abral, Hairul Azka, Muhammad Adlan Sapuan, S.M. Admi, Ratna Isnanita Shi, Shih-Chen Zainul, Rahadian Azril, None Zikri, Ahmad Mahardika, Melbi Developing a simple and environmentally friendly method to vary the physical, mechanical, and thermal properties of cellulose films is of great importance. This study aimed to characterize 2,2,6,6-tetramethylpiperidinyl-1-oxyl (TEMPO)-oxidized bacterial cellulose (BC) films prepared using non-pressurized hot water vapor (NPHWV) method. A wet BC-pellicle that had been oxidized with TEMPO was treated with NPHWV for 60, 120, and 240 minutes, respectively. As a control, a TEMPO-oxidized BC (TOBC) film without NPHWV was prepared. The results show that the longer NPHWV duration of the TOBC film increased the tensile and thermal properties. This film became more hydrophobic and showed lower moisture absorption, thermal conductivity and organic solvent uptake, more crystalline structure, and higher fiber density after NPHWV treatment. The acquired results provide a simple, inexpensive, and ecologically friendly method for varying TOBC film properties. Royal Society of Chemistry 2024 Article PeerReviewed text en cc_by_nc_4 http://psasir.upm.edu.my/id/eprint/114493/1/114493.pdf Rahmadiawan, Dieter and Abral, Hairul and Azka, Muhammad Adlan and Sapuan, S.M. and Admi, Ratna Isnanita and Shi, Shih-Chen and Zainul, Rahadian and Azril, None and Zikri, Ahmad and Mahardika, Melbi (2024) Enhanced properties of TEMPO-oxidized bacterial cellulose films via eco-friendly non-pressurized hot water vapor treatment for sustainable and smart food packaging. RSC Advances, 14 (40). pp. 29624-29635. ISSN 2046-2069; eISSN: 2046-2069 https://pubs.rsc.org/en/content/articlelanding/2024/ra/d4ra06099g 10.1039/d4ra06099g
spellingShingle Rahmadiawan, Dieter
Abral, Hairul
Azka, Muhammad Adlan
Sapuan, S.M.
Admi, Ratna Isnanita
Shi, Shih-Chen
Zainul, Rahadian
Azril, None
Zikri, Ahmad
Mahardika, Melbi
Enhanced properties of TEMPO-oxidized bacterial cellulose films via eco-friendly non-pressurized hot water vapor treatment for sustainable and smart food packaging
title Enhanced properties of TEMPO-oxidized bacterial cellulose films via eco-friendly non-pressurized hot water vapor treatment for sustainable and smart food packaging
title_full Enhanced properties of TEMPO-oxidized bacterial cellulose films via eco-friendly non-pressurized hot water vapor treatment for sustainable and smart food packaging
title_fullStr Enhanced properties of TEMPO-oxidized bacterial cellulose films via eco-friendly non-pressurized hot water vapor treatment for sustainable and smart food packaging
title_full_unstemmed Enhanced properties of TEMPO-oxidized bacterial cellulose films via eco-friendly non-pressurized hot water vapor treatment for sustainable and smart food packaging
title_short Enhanced properties of TEMPO-oxidized bacterial cellulose films via eco-friendly non-pressurized hot water vapor treatment for sustainable and smart food packaging
title_sort enhanced properties of tempo-oxidized bacterial cellulose films via eco-friendly non-pressurized hot water vapor treatment for sustainable and smart food packaging
url http://psasir.upm.edu.my/id/eprint/114493/
http://psasir.upm.edu.my/id/eprint/114493/
http://psasir.upm.edu.my/id/eprint/114493/
http://psasir.upm.edu.my/id/eprint/114493/1/114493.pdf