Adsorption isotherm analysis for CO2 capture using barium oxide impregnated iron (iii) oxide by ultrasonic-assisted synthesis

The barium oxide impregnated iron(III) oxide (BaO/Fe2O3) adsorbent was synthesized by an ultrasonic-assisted method. The adsorbent was calcined at 200-500 °C and its adsorption capacity was measured. The ultrasonic-assisted synthesis generated well-dispersed of BaO on Fe2O3 by giving none of the BaO...

Full description

Bibliographic Details
Main Authors: Lahuri, Azizul Hakim, Yarmo, Mohd Ambar, Abu Tahari, Maratun Najiha, Dzakaria, Norliza
Format: Article
Published: Trans Tech Publications 2022
Online Access:http://psasir.upm.edu.my/id/eprint/100132/
_version_ 1848863242052435968
author Lahuri, Azizul Hakim
Yarmo, Mohd Ambar
Abu Tahari, Maratun Najiha
Dzakaria, Norliza
author_facet Lahuri, Azizul Hakim
Yarmo, Mohd Ambar
Abu Tahari, Maratun Najiha
Dzakaria, Norliza
author_sort Lahuri, Azizul Hakim
building UPM Institutional Repository
collection Online Access
description The barium oxide impregnated iron(III) oxide (BaO/Fe2O3) adsorbent was synthesized by an ultrasonic-assisted method. The adsorbent was calcined at 200-500 °C and its adsorption capacity was measured. The ultrasonic-assisted synthesis generated well-dispersed of BaO on Fe2O3 by giving none of the BaO peaks were observed through the XRD pattern. The most efficient adsorbent of BaO/Fe2O3200 was calcined at 200 °C with adsorption capacity for physisorption and chemisorption of 5.01 and 88.81 mg/g respectively. Besides other carbonate species, it was believed the presence of the hydroxyl group could enhance the sorption by forming bicarbonate upon CO2 chemisorption. It is also possessed a lower desorption range compared to BaO and Fe2O3 alone. The experimental CO2 adsorption isotherm at 25 °C fit better with the Freundlich isotherm model. It implies a favorable adsorption process with multilayer adsorption occurs onto the heterogeneous surface.
first_indexed 2025-11-15T13:29:48Z
format Article
id upm-100132
institution Universiti Putra Malaysia
institution_category Local University
last_indexed 2025-11-15T13:29:48Z
publishDate 2022
publisher Trans Tech Publications
recordtype eprints
repository_type Digital Repository
spelling upm-1001322024-07-15T06:43:40Z http://psasir.upm.edu.my/id/eprint/100132/ Adsorption isotherm analysis for CO2 capture using barium oxide impregnated iron (iii) oxide by ultrasonic-assisted synthesis Lahuri, Azizul Hakim Yarmo, Mohd Ambar Abu Tahari, Maratun Najiha Dzakaria, Norliza The barium oxide impregnated iron(III) oxide (BaO/Fe2O3) adsorbent was synthesized by an ultrasonic-assisted method. The adsorbent was calcined at 200-500 °C and its adsorption capacity was measured. The ultrasonic-assisted synthesis generated well-dispersed of BaO on Fe2O3 by giving none of the BaO peaks were observed through the XRD pattern. The most efficient adsorbent of BaO/Fe2O3200 was calcined at 200 °C with adsorption capacity for physisorption and chemisorption of 5.01 and 88.81 mg/g respectively. Besides other carbonate species, it was believed the presence of the hydroxyl group could enhance the sorption by forming bicarbonate upon CO2 chemisorption. It is also possessed a lower desorption range compared to BaO and Fe2O3 alone. The experimental CO2 adsorption isotherm at 25 °C fit better with the Freundlich isotherm model. It implies a favorable adsorption process with multilayer adsorption occurs onto the heterogeneous surface. Trans Tech Publications 2022-01 Article PeerReviewed Lahuri, Azizul Hakim and Yarmo, Mohd Ambar and Abu Tahari, Maratun Najiha and Dzakaria, Norliza (2022) Adsorption isotherm analysis for CO2 capture using barium oxide impregnated iron (iii) oxide by ultrasonic-assisted synthesis. Key Engineering Materials, 908. pp. 379-384. ISSN 1662-9795 https://www.scientific.net/KEM.908.379 10.4028/p-lm9fmx
spellingShingle Lahuri, Azizul Hakim
Yarmo, Mohd Ambar
Abu Tahari, Maratun Najiha
Dzakaria, Norliza
Adsorption isotherm analysis for CO2 capture using barium oxide impregnated iron (iii) oxide by ultrasonic-assisted synthesis
title Adsorption isotherm analysis for CO2 capture using barium oxide impregnated iron (iii) oxide by ultrasonic-assisted synthesis
title_full Adsorption isotherm analysis for CO2 capture using barium oxide impregnated iron (iii) oxide by ultrasonic-assisted synthesis
title_fullStr Adsorption isotherm analysis for CO2 capture using barium oxide impregnated iron (iii) oxide by ultrasonic-assisted synthesis
title_full_unstemmed Adsorption isotherm analysis for CO2 capture using barium oxide impregnated iron (iii) oxide by ultrasonic-assisted synthesis
title_short Adsorption isotherm analysis for CO2 capture using barium oxide impregnated iron (iii) oxide by ultrasonic-assisted synthesis
title_sort adsorption isotherm analysis for co2 capture using barium oxide impregnated iron (iii) oxide by ultrasonic-assisted synthesis
url http://psasir.upm.edu.my/id/eprint/100132/
http://psasir.upm.edu.my/id/eprint/100132/
http://psasir.upm.edu.my/id/eprint/100132/