Sulphated mesoporous silica synthesized from rice husk ash for chalcone production

Chalcone is an aromatic ketone that have important biological properties. It can be prepared by an aldol condensation between a benzaldehyde and an acetophenone in the presence of catalyst. A series of S-MCM-48 (SO 42 / MCM-48) was synthesized in this study. Rice husk ash (RHA), an agriculture waste...

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Main Author: Nor Illiana , Mohd Nor
Format: Undergraduates Project Papers
Language:English
Published: 2012
Subjects:
Online Access:http://umpir.ump.edu.my/id/eprint/7820/
http://umpir.ump.edu.my/id/eprint/7820/1/NOR_ILLIANA_BINTI_MOHD_NOOR.PDF
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author Nor Illiana , Mohd Nor
author_facet Nor Illiana , Mohd Nor
author_sort Nor Illiana , Mohd Nor
building UMP Institutional Repository
collection Online Access
description Chalcone is an aromatic ketone that have important biological properties. It can be prepared by an aldol condensation between a benzaldehyde and an acetophenone in the presence of catalyst. A series of S-MCM-48 (SO 42 / MCM-48) was synthesized in this study. Rice husk ash (RHA), an agriculture waste was used as a silica (Si0 2 ) source to synthesis the MCM-48 mesoporous molecular sieves by mean of hydrothermal method and suiphation medification using sulfuric acid (H2SO4) as the sulphate sources. The pore packing order of the SO4 2-doped material dependend strongly on the synthesis conditions such as aging temperature, pH of reaction mixture and dopant concentration. The physicochemical properties of mesoporous material was characterized by X-Ray diffraction (XRD), surface area analysis (BET), Fourier- Transform Infrared Spectroscopy (FTIR) and Thermogravimetric Analyzer (TGA). A simple preparation method was used to generate strong acidity catalyst by introducing sulphate groups onto the surface of MCM-48. The prepared sulphated MCM-48 has been used to catalyzed benzaldehyde and acetophenone and was analyzed by using GC. The conversion of acetophenone was calculated and the best conversion was 85.5% by using S-MCM48(60) catalysts. Keyword:SO42-doped MCM-48; Heterogeneous catalyst; chalcone; mesoporous materials.
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format Undergraduates Project Papers
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institution Universiti Malaysia Pahang
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language English
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publishDate 2012
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spelling ump-78202021-06-10T04:04:03Z http://umpir.ump.edu.my/id/eprint/7820/ Sulphated mesoporous silica synthesized from rice husk ash for chalcone production Nor Illiana , Mohd Nor QD Chemistry Chalcone is an aromatic ketone that have important biological properties. It can be prepared by an aldol condensation between a benzaldehyde and an acetophenone in the presence of catalyst. A series of S-MCM-48 (SO 42 / MCM-48) was synthesized in this study. Rice husk ash (RHA), an agriculture waste was used as a silica (Si0 2 ) source to synthesis the MCM-48 mesoporous molecular sieves by mean of hydrothermal method and suiphation medification using sulfuric acid (H2SO4) as the sulphate sources. The pore packing order of the SO4 2-doped material dependend strongly on the synthesis conditions such as aging temperature, pH of reaction mixture and dopant concentration. The physicochemical properties of mesoporous material was characterized by X-Ray diffraction (XRD), surface area analysis (BET), Fourier- Transform Infrared Spectroscopy (FTIR) and Thermogravimetric Analyzer (TGA). A simple preparation method was used to generate strong acidity catalyst by introducing sulphate groups onto the surface of MCM-48. The prepared sulphated MCM-48 has been used to catalyzed benzaldehyde and acetophenone and was analyzed by using GC. The conversion of acetophenone was calculated and the best conversion was 85.5% by using S-MCM48(60) catalysts. Keyword:SO42-doped MCM-48; Heterogeneous catalyst; chalcone; mesoporous materials. 2012 Undergraduates Project Papers NonPeerReviewed application/pdf en http://umpir.ump.edu.my/id/eprint/7820/1/NOR_ILLIANA_BINTI_MOHD_NOOR.PDF Nor Illiana , Mohd Nor (2012) Sulphated mesoporous silica synthesized from rice husk ash for chalcone production. Faculty of Industrial Sciences & Technology, Universiti Malaysia Pahang.
spellingShingle QD Chemistry
Nor Illiana , Mohd Nor
Sulphated mesoporous silica synthesized from rice husk ash for chalcone production
title Sulphated mesoporous silica synthesized from rice husk ash for chalcone production
title_full Sulphated mesoporous silica synthesized from rice husk ash for chalcone production
title_fullStr Sulphated mesoporous silica synthesized from rice husk ash for chalcone production
title_full_unstemmed Sulphated mesoporous silica synthesized from rice husk ash for chalcone production
title_short Sulphated mesoporous silica synthesized from rice husk ash for chalcone production
title_sort sulphated mesoporous silica synthesized from rice husk ash for chalcone production
topic QD Chemistry
url http://umpir.ump.edu.my/id/eprint/7820/
http://umpir.ump.edu.my/id/eprint/7820/1/NOR_ILLIANA_BINTI_MOHD_NOOR.PDF