Modeling and Characterization of Ion-Imprinted Polymer for Arsenic Species Removal From Aqueous Solution

Arsenic (As) contamination is a global issue, especially in As-rich geological formations. In this study, an ion-imprinted polymer (As(III)-IIP) is synthesized and characterized in terms of kinetic modeling and application via solid phase extraction (SPE). As is detected by using the inductively cou...

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Main Author: Nurlin, Abu Samah
Format: Article
Language:English
Published: John Wiley & Sons, Inc. 2025
Subjects:
Online Access:https://umpir.ump.edu.my/id/eprint/45333/
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author Nurlin, Abu Samah
author_facet Nurlin, Abu Samah
author_sort Nurlin, Abu Samah
building UMP Institutional Repository
collection Online Access
description Arsenic (As) contamination is a global issue, especially in As-rich geological formations. In this study, an ion-imprinted polymer (As(III)-IIP) is synthesized and characterized in terms of kinetic modeling and application via solid phase extraction (SPE). As is detected by using the inductively coupled plasma-mass spectrometer (ICP-MS). The surface study is also included in this study, in which the differences between non-imprinted polymer (NIP) and As(III)-IIP before and after sorption are observed via field electron scanning electron microscope (FESEM). As a result, As(III)-IIP follows the pseudo-second-order of reaction in kinetics and reaches 95% within 5 min of removal. In FESEM micrographs, As(III)-IIP shows the particles on the surface are likely homogenous compared to NIP. Whereas As(III)-IIP after sorption is much more likely bigger than the original As(III)-IIP due to the expansion of particles during agitation in an aqueous solution. In the first cycle, 99.53% ± 0.45% of removal in real wastewater analysis is obtained via SPE. However, for the second cycle onwards, the removal is not removed totally, which shows that a new combination of eluent is required. In conclusion, As(III)-IIP shows good potential as a sorbent to be used for the removal of As from wastewater.
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spelling ump-453332025-08-12T03:57:12Z https://umpir.ump.edu.my/id/eprint/45333/ Modeling and Characterization of Ion-Imprinted Polymer for Arsenic Species Removal From Aqueous Solution Nurlin, Abu Samah QD Chemistry TP Chemical technology Arsenic (As) contamination is a global issue, especially in As-rich geological formations. In this study, an ion-imprinted polymer (As(III)-IIP) is synthesized and characterized in terms of kinetic modeling and application via solid phase extraction (SPE). As is detected by using the inductively coupled plasma-mass spectrometer (ICP-MS). The surface study is also included in this study, in which the differences between non-imprinted polymer (NIP) and As(III)-IIP before and after sorption are observed via field electron scanning electron microscope (FESEM). As a result, As(III)-IIP follows the pseudo-second-order of reaction in kinetics and reaches 95% within 5 min of removal. In FESEM micrographs, As(III)-IIP shows the particles on the surface are likely homogenous compared to NIP. Whereas As(III)-IIP after sorption is much more likely bigger than the original As(III)-IIP due to the expansion of particles during agitation in an aqueous solution. In the first cycle, 99.53% ± 0.45% of removal in real wastewater analysis is obtained via SPE. However, for the second cycle onwards, the removal is not removed totally, which shows that a new combination of eluent is required. In conclusion, As(III)-IIP shows good potential as a sorbent to be used for the removal of As from wastewater. John Wiley & Sons, Inc. 2025-02-17 Article PeerReviewed pdf en https://umpir.ump.edu.my/id/eprint/45333/1/100105409.pdf Nurlin, Abu Samah (2025) Modeling and Characterization of Ion-Imprinted Polymer for Arsenic Species Removal From Aqueous Solution. Macromolecular Symposia, 414 (2300222). pp. 1-6. ISSN 1521-3900. (Published) https://doi.org/10.1002/masy.202300222 https://doi.org/10.1002/masy.202300222 https://doi.org/10.1002/masy.202300222
spellingShingle QD Chemistry
TP Chemical technology
Nurlin, Abu Samah
Modeling and Characterization of Ion-Imprinted Polymer for Arsenic Species Removal From Aqueous Solution
title Modeling and Characterization of Ion-Imprinted Polymer for Arsenic Species Removal From Aqueous Solution
title_full Modeling and Characterization of Ion-Imprinted Polymer for Arsenic Species Removal From Aqueous Solution
title_fullStr Modeling and Characterization of Ion-Imprinted Polymer for Arsenic Species Removal From Aqueous Solution
title_full_unstemmed Modeling and Characterization of Ion-Imprinted Polymer for Arsenic Species Removal From Aqueous Solution
title_short Modeling and Characterization of Ion-Imprinted Polymer for Arsenic Species Removal From Aqueous Solution
title_sort modeling and characterization of ion-imprinted polymer for arsenic species removal from aqueous solution
topic QD Chemistry
TP Chemical technology
url https://umpir.ump.edu.my/id/eprint/45333/
https://umpir.ump.edu.my/id/eprint/45333/
https://umpir.ump.edu.my/id/eprint/45333/