Systematic study of Co-free LiNi0.9Mn0.07Al0.03O2 Ni-rich cathode materials to realize high-energy density Li-ion batteries

The growing use of EVs and society's energy needs require safe, affordable, durable, and eco-friendly high-energy lithium-ion batteries (LIBs). To this end, we synthesized and investigated the removal of Co from Al-doped Ni-rich cathode materials, specifically LiNi0.9Co0.1Al0.0O2 (NCA-0), LiNi0...

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Main Authors: Seenivasan, Manojkumar, Yang, Chunchen, Wu, She–Huang, Chang, Jeng Kuei, Jose, Rajan
Format: Article
Language:English
Published: Elsevier Ltd
Subjects:
Online Access:http://umpir.ump.edu.my/id/eprint/45047/
http://umpir.ump.edu.my/id/eprint/45047/1/Systematic%20study%20of%20Co-free%20LiNi0.9Mn0.07Al0.03O2%20Ni-rich%20cathode.pdf
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author Seenivasan, Manojkumar
Yang, Chunchen
Wu, She–Huang
Chang, Jeng Kuei
Jose, Rajan
author_facet Seenivasan, Manojkumar
Yang, Chunchen
Wu, She–Huang
Chang, Jeng Kuei
Jose, Rajan
author_sort Seenivasan, Manojkumar
building UMP Institutional Repository
collection Online Access
description The growing use of EVs and society's energy needs require safe, affordable, durable, and eco-friendly high-energy lithium-ion batteries (LIBs). To this end, we synthesized and investigated the removal of Co from Al-doped Ni-rich cathode materials, specifically LiNi0.9Co0.1Al0.0O2 (NCA-0), LiNi0.9Mn0.1Al0.0O2 (NMA-0), LiNi0.9Mn0.07Al0.03O2 (NMA-3), intending to enhance LIB performance and reduce the reliance on cobalt, a costly and scarce resource. Our study primarily focuses on how the removal of Co affects the material characteristics of Ni-rich cathode material and further introduces aluminum into the cathode composition to study its impacts on electrochemical properties and overall performance. Among the synthesized samples, we discovered that the NMA-3 sample, modified with 3 mol% of Al, exhibited superior battery performance, demonstrating the effectiveness of aluminum in promoting cathode stability. Furthermore, the Al-modified cathode showed promising cycle life under normal and high-temperature conditions. Our NMA-3 demonstrated remarkable capacity retention of ∼ 88 % at 25 °C and ∼ 81 % at 45 °C after 200 cycles at 1C, within a voltage range of 2.8–4.3 V, closely matching the performances of conventional NCM and NCA cathodes. Without cobalt, the cathodes exhibited increased cation disorder leading to inferior rate capabilities at high C-rates. In-situ transmission XRD analysis revealed that the introduction of Al has reduced the phase change and provided much-needed stability to the overall structure of the Co-free NMA-3. Altogether, the findings suggest that our aluminum-modified NMA-3 sample offers a promising approach to developing Co-free, Ni-rich cathodes, effectively paving the way toward sustainable, high-energy–density LIBs.
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institution Universiti Malaysia Pahang
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spelling ump-450472025-07-09T07:21:20Z http://umpir.ump.edu.my/id/eprint/45047/ Systematic study of Co-free LiNi0.9Mn0.07Al0.03O2 Ni-rich cathode materials to realize high-energy density Li-ion batteries Seenivasan, Manojkumar Yang, Chunchen Wu, She–Huang Chang, Jeng Kuei Jose, Rajan QC Physics TK Electrical engineering. Electronics Nuclear engineering TP Chemical technology The growing use of EVs and society's energy needs require safe, affordable, durable, and eco-friendly high-energy lithium-ion batteries (LIBs). To this end, we synthesized and investigated the removal of Co from Al-doped Ni-rich cathode materials, specifically LiNi0.9Co0.1Al0.0O2 (NCA-0), LiNi0.9Mn0.1Al0.0O2 (NMA-0), LiNi0.9Mn0.07Al0.03O2 (NMA-3), intending to enhance LIB performance and reduce the reliance on cobalt, a costly and scarce resource. Our study primarily focuses on how the removal of Co affects the material characteristics of Ni-rich cathode material and further introduces aluminum into the cathode composition to study its impacts on electrochemical properties and overall performance. Among the synthesized samples, we discovered that the NMA-3 sample, modified with 3 mol% of Al, exhibited superior battery performance, demonstrating the effectiveness of aluminum in promoting cathode stability. Furthermore, the Al-modified cathode showed promising cycle life under normal and high-temperature conditions. Our NMA-3 demonstrated remarkable capacity retention of ∼ 88 % at 25 °C and ∼ 81 % at 45 °C after 200 cycles at 1C, within a voltage range of 2.8–4.3 V, closely matching the performances of conventional NCM and NCA cathodes. Without cobalt, the cathodes exhibited increased cation disorder leading to inferior rate capabilities at high C-rates. In-situ transmission XRD analysis revealed that the introduction of Al has reduced the phase change and provided much-needed stability to the overall structure of the Co-free NMA-3. Altogether, the findings suggest that our aluminum-modified NMA-3 sample offers a promising approach to developing Co-free, Ni-rich cathodes, effectively paving the way toward sustainable, high-energy–density LIBs. Elsevier Ltd Article PeerReviewed pdf en http://umpir.ump.edu.my/id/eprint/45047/1/Systematic%20study%20of%20Co-free%20LiNi0.9Mn0.07Al0.03O2%20Ni-rich%20cathode.pdf Seenivasan, Manojkumar and Yang, Chunchen and Wu, She–Huang and Chang, Jeng Kuei and Jose, Rajan Systematic study of Co-free LiNi0.9Mn0.07Al0.03O2 Ni-rich cathode materials to realize high-energy density Li-ion batteries. Journal of Colloid and Interface Science, 661. pp. 1070-1081. ISSN 0021-9797. (Published) https://doi.org/10.1016/j.jcis.2024.02.040 https://doi.org/10.1016/j.jcis.2024.02.040
spellingShingle QC Physics
TK Electrical engineering. Electronics Nuclear engineering
TP Chemical technology
Seenivasan, Manojkumar
Yang, Chunchen
Wu, She–Huang
Chang, Jeng Kuei
Jose, Rajan
Systematic study of Co-free LiNi0.9Mn0.07Al0.03O2 Ni-rich cathode materials to realize high-energy density Li-ion batteries
title Systematic study of Co-free LiNi0.9Mn0.07Al0.03O2 Ni-rich cathode materials to realize high-energy density Li-ion batteries
title_full Systematic study of Co-free LiNi0.9Mn0.07Al0.03O2 Ni-rich cathode materials to realize high-energy density Li-ion batteries
title_fullStr Systematic study of Co-free LiNi0.9Mn0.07Al0.03O2 Ni-rich cathode materials to realize high-energy density Li-ion batteries
title_full_unstemmed Systematic study of Co-free LiNi0.9Mn0.07Al0.03O2 Ni-rich cathode materials to realize high-energy density Li-ion batteries
title_short Systematic study of Co-free LiNi0.9Mn0.07Al0.03O2 Ni-rich cathode materials to realize high-energy density Li-ion batteries
title_sort systematic study of co-free lini0.9mn0.07al0.03o2 ni-rich cathode materials to realize high-energy density li-ion batteries
topic QC Physics
TK Electrical engineering. Electronics Nuclear engineering
TP Chemical technology
url http://umpir.ump.edu.my/id/eprint/45047/
http://umpir.ump.edu.my/id/eprint/45047/
http://umpir.ump.edu.my/id/eprint/45047/
http://umpir.ump.edu.my/id/eprint/45047/1/Systematic%20study%20of%20Co-free%20LiNi0.9Mn0.07Al0.03O2%20Ni-rich%20cathode.pdf