Ceramic-polymer-carbon composite coating on the truncated octahedron-shaped LNMO cathode for high capacity and extended cycling in high-voltage lithium-ion batteries

Long-term electrochemical cycle life of the LiNi0.5Mn1.5O4 (LNMO) cathode with liquid electrolytes (LEs) and the inadequate knowledge of the cell failure mechanism are the eloquent Achilles’ heel to practical applications despite their large promise to lower the cost of lithium-ion batteries (LIBs)....

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Main Authors: Pazhaniswamy, Sivaraj, Cha, Gihoon, Joshi, Sagar A, Parameswaran, Abhilash Karuthedath, Jose, Rajan, Pechmann, Sabrina, Christiansen, Silke, Agarwal, Seema
Format: Article
Language:English
Published: American Chemical Society (ACS Publications) 2024
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Online Access:http://umpir.ump.edu.my/id/eprint/44064/
http://umpir.ump.edu.my/id/eprint/44064/1/Ceramic-polymer-carbon%20composite%20coating.pdf
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author Pazhaniswamy, Sivaraj
Cha, Gihoon
Joshi, Sagar A
Parameswaran, Abhilash Karuthedath
Jose, Rajan
Pechmann, Sabrina
Christiansen, Silke
Agarwal, Seema
author_facet Pazhaniswamy, Sivaraj
Cha, Gihoon
Joshi, Sagar A
Parameswaran, Abhilash Karuthedath
Jose, Rajan
Pechmann, Sabrina
Christiansen, Silke
Agarwal, Seema
author_sort Pazhaniswamy, Sivaraj
building UMP Institutional Repository
collection Online Access
description Long-term electrochemical cycle life of the LiNi0.5Mn1.5O4 (LNMO) cathode with liquid electrolytes (LEs) and the inadequate knowledge of the cell failure mechanism are the eloquent Achilles’ heel to practical applications despite their large promise to lower the cost of lithium-ion batteries (LIBs). Herein, a strategy for engineering the cathode–LE interface is presented to enhance the cycle life of LIBs. The direct contact between cathode-active particles and LE is controlled by encasing sol–gel-synthesized truncated octahedron-shaped LNMO particles by an ion–electron-conductive (ambipolar) hybrid ceramic–polymer electrolyte (IECHP) via a simple slot-die coating. The IECHP-coated LNMO cathode demonstrated negligible capacity fading in 250 cycles and a capacity retention of ∼90% after 1000 charge–discharge cycles, significantly exceeding that of the uncoated LNMO cathode (a capacity retention of ∼57% after 980 cycles) in 1 M LiPF6 in EC:DMC at 1 C rate. The difference in stability between the two types of cathodes after cycling is examined by focused ion beam scanning electron microscopy and time-of-flight secondary ion mass spectrometry. These studies revealed that the pristine LNMO produces an inactive layer on the cathode surface, reducing ionic transport between the cathode and the electrolyte and increasing the interface resistance. The IECHP coating successfully overcomes these limitations. Therefore, the present work underlines the adaptability of IECHP-coated LNMO as a high-voltage cathode material in a 1 M LiPF6 electrolyte for prolonged use. The proposed strategy is simple and affordable for commercial applications.
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publisher American Chemical Society (ACS Publications)
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spelling ump-440642025-03-14T04:58:38Z http://umpir.ump.edu.my/id/eprint/44064/ Ceramic-polymer-carbon composite coating on the truncated octahedron-shaped LNMO cathode for high capacity and extended cycling in high-voltage lithium-ion batteries Pazhaniswamy, Sivaraj Cha, Gihoon Joshi, Sagar A Parameswaran, Abhilash Karuthedath Jose, Rajan Pechmann, Sabrina Christiansen, Silke Agarwal, Seema QD Chemistry TP Chemical technology Long-term electrochemical cycle life of the LiNi0.5Mn1.5O4 (LNMO) cathode with liquid electrolytes (LEs) and the inadequate knowledge of the cell failure mechanism are the eloquent Achilles’ heel to practical applications despite their large promise to lower the cost of lithium-ion batteries (LIBs). Herein, a strategy for engineering the cathode–LE interface is presented to enhance the cycle life of LIBs. The direct contact between cathode-active particles and LE is controlled by encasing sol–gel-synthesized truncated octahedron-shaped LNMO particles by an ion–electron-conductive (ambipolar) hybrid ceramic–polymer electrolyte (IECHP) via a simple slot-die coating. The IECHP-coated LNMO cathode demonstrated negligible capacity fading in 250 cycles and a capacity retention of ∼90% after 1000 charge–discharge cycles, significantly exceeding that of the uncoated LNMO cathode (a capacity retention of ∼57% after 980 cycles) in 1 M LiPF6 in EC:DMC at 1 C rate. The difference in stability between the two types of cathodes after cycling is examined by focused ion beam scanning electron microscopy and time-of-flight secondary ion mass spectrometry. These studies revealed that the pristine LNMO produces an inactive layer on the cathode surface, reducing ionic transport between the cathode and the electrolyte and increasing the interface resistance. The IECHP coating successfully overcomes these limitations. Therefore, the present work underlines the adaptability of IECHP-coated LNMO as a high-voltage cathode material in a 1 M LiPF6 electrolyte for prolonged use. The proposed strategy is simple and affordable for commercial applications. American Chemical Society (ACS Publications) 2024-11-07 Article PeerReviewed pdf en cc_by_4 http://umpir.ump.edu.my/id/eprint/44064/1/Ceramic-polymer-carbon%20composite%20coating.pdf Pazhaniswamy, Sivaraj and Cha, Gihoon and Joshi, Sagar A and Parameswaran, Abhilash Karuthedath and Jose, Rajan and Pechmann, Sabrina and Christiansen, Silke and Agarwal, Seema (2024) Ceramic-polymer-carbon composite coating on the truncated octahedron-shaped LNMO cathode for high capacity and extended cycling in high-voltage lithium-ion batteries. Energy & Fuels, 38 (21). pp. 21456-21467. ISSN 0887-0624. (Published) https://pubs.acs.org/doi/10.1021/acs.energyfuels.4c02933 https://pubs.acs.org/doi/10.1021/acs.energyfuels.4c02933
spellingShingle QD Chemistry
TP Chemical technology
Pazhaniswamy, Sivaraj
Cha, Gihoon
Joshi, Sagar A
Parameswaran, Abhilash Karuthedath
Jose, Rajan
Pechmann, Sabrina
Christiansen, Silke
Agarwal, Seema
Ceramic-polymer-carbon composite coating on the truncated octahedron-shaped LNMO cathode for high capacity and extended cycling in high-voltage lithium-ion batteries
title Ceramic-polymer-carbon composite coating on the truncated octahedron-shaped LNMO cathode for high capacity and extended cycling in high-voltage lithium-ion batteries
title_full Ceramic-polymer-carbon composite coating on the truncated octahedron-shaped LNMO cathode for high capacity and extended cycling in high-voltage lithium-ion batteries
title_fullStr Ceramic-polymer-carbon composite coating on the truncated octahedron-shaped LNMO cathode for high capacity and extended cycling in high-voltage lithium-ion batteries
title_full_unstemmed Ceramic-polymer-carbon composite coating on the truncated octahedron-shaped LNMO cathode for high capacity and extended cycling in high-voltage lithium-ion batteries
title_short Ceramic-polymer-carbon composite coating on the truncated octahedron-shaped LNMO cathode for high capacity and extended cycling in high-voltage lithium-ion batteries
title_sort ceramic-polymer-carbon composite coating on the truncated octahedron-shaped lnmo cathode for high capacity and extended cycling in high-voltage lithium-ion batteries
topic QD Chemistry
TP Chemical technology
url http://umpir.ump.edu.my/id/eprint/44064/
http://umpir.ump.edu.my/id/eprint/44064/
http://umpir.ump.edu.my/id/eprint/44064/
http://umpir.ump.edu.my/id/eprint/44064/1/Ceramic-polymer-carbon%20composite%20coating.pdf