Facile synthesis of fibrous Faujasite Y supported Ni (Ni/FFY) catalyst for hydrogen production via glycerol dry reforming

In this study, the dendritic structure of Ni-supported Fibrous Faujasite Y (Ni/FFY) catalyst was successfully synthesized by employing a hydrothermal-assisted microemulsion system and subsequently tested in glycerol dry reforming to produce syngas. FFY possesses high porosity due to the formation of...

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Main Authors: Nornasuha, Abdullah, Nurul Aini, Razali, Herma Dina, Setiabudi, Asmida, Ideris, A. R., Mohamed, A. A., Jalil
Format: Article
Language:English
English
Published: Elsevier Ltd 2023
Subjects:
Online Access:http://umpir.ump.edu.my/id/eprint/40532/
http://umpir.ump.edu.my/id/eprint/40532/1/Facile%20synthesis%20of%20fibrous%20Faujasite%20Y%20supported%20Ni.pdf
http://umpir.ump.edu.my/id/eprint/40532/2/Facile%20synthesis%20of%20fibrous%20Faujasite%20Y%20supported%20Ni_FULL.pdf
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author Nornasuha, Abdullah
Nurul Aini, Razali
Herma Dina, Setiabudi
Asmida, Ideris
A. R., Mohamed
A. A., Jalil
author_facet Nornasuha, Abdullah
Nurul Aini, Razali
Herma Dina, Setiabudi
Asmida, Ideris
A. R., Mohamed
A. A., Jalil
author_sort Nornasuha, Abdullah
building UMP Institutional Repository
collection Online Access
description In this study, the dendritic structure of Ni-supported Fibrous Faujasite Y (Ni/FFY) catalyst was successfully synthesized by employing a hydrothermal-assisted microemulsion system and subsequently tested in glycerol dry reforming to produce syngas. FFY possesses high porosity due to the formation of radial wrinkle fibre observed from TEM analysis. This provides a huge amount of interparticle pores that facilitate the absorption of the molecules within the material under a minimum hindrance, hence boosting the interior surface accessibility of Ni/FFY. This exclusive morphology contributed to the enhancement in the amount of accessible Ni active sites, resulting in the good activity of Ni/FFY (C3H8O3 conversion = 56.28 %, CO yield = 70.14 %, and H2 yield = 49.80 %). The extraordinary physicochemical properties of Ni/FFY and outstanding catalytic performance in glycerol dry reforming proved its capability as a sustainable catalyst in transforming waste byproduct (glycerol) and greenhouse gas (CO2) to clean energy (H2). This finding presents a pioneering fibrous zeolite catalyst for hydrogen generation in glycerol reforming.
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publishDate 2023
publisher Elsevier Ltd
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spelling ump-405322024-02-28T06:55:02Z http://umpir.ump.edu.my/id/eprint/40532/ Facile synthesis of fibrous Faujasite Y supported Ni (Ni/FFY) catalyst for hydrogen production via glycerol dry reforming Nornasuha, Abdullah Nurul Aini, Razali Herma Dina, Setiabudi Asmida, Ideris A. R., Mohamed A. A., Jalil TP Chemical technology In this study, the dendritic structure of Ni-supported Fibrous Faujasite Y (Ni/FFY) catalyst was successfully synthesized by employing a hydrothermal-assisted microemulsion system and subsequently tested in glycerol dry reforming to produce syngas. FFY possesses high porosity due to the formation of radial wrinkle fibre observed from TEM analysis. This provides a huge amount of interparticle pores that facilitate the absorption of the molecules within the material under a minimum hindrance, hence boosting the interior surface accessibility of Ni/FFY. This exclusive morphology contributed to the enhancement in the amount of accessible Ni active sites, resulting in the good activity of Ni/FFY (C3H8O3 conversion = 56.28 %, CO yield = 70.14 %, and H2 yield = 49.80 %). The extraordinary physicochemical properties of Ni/FFY and outstanding catalytic performance in glycerol dry reforming proved its capability as a sustainable catalyst in transforming waste byproduct (glycerol) and greenhouse gas (CO2) to clean energy (H2). This finding presents a pioneering fibrous zeolite catalyst for hydrogen generation in glycerol reforming. Elsevier Ltd 2023-07 Article PeerReviewed pdf en http://umpir.ump.edu.my/id/eprint/40532/1/Facile%20synthesis%20of%20fibrous%20Faujasite%20Y%20supported%20Ni.pdf pdf en http://umpir.ump.edu.my/id/eprint/40532/2/Facile%20synthesis%20of%20fibrous%20Faujasite%20Y%20supported%20Ni_FULL.pdf Nornasuha, Abdullah and Nurul Aini, Razali and Herma Dina, Setiabudi and Asmida, Ideris and A. R., Mohamed and A. A., Jalil (2023) Facile synthesis of fibrous Faujasite Y supported Ni (Ni/FFY) catalyst for hydrogen production via glycerol dry reforming. Materials Today: Proceedings. pp. 1-7. ISSN 2214-7853. (In Press / Online First) (In Press / Online First) https://doi.org/10.1016/j.matpr.2023.06.314 https://doi.org/10.1016/j.matpr.2023.06.314
spellingShingle TP Chemical technology
Nornasuha, Abdullah
Nurul Aini, Razali
Herma Dina, Setiabudi
Asmida, Ideris
A. R., Mohamed
A. A., Jalil
Facile synthesis of fibrous Faujasite Y supported Ni (Ni/FFY) catalyst for hydrogen production via glycerol dry reforming
title Facile synthesis of fibrous Faujasite Y supported Ni (Ni/FFY) catalyst for hydrogen production via glycerol dry reforming
title_full Facile synthesis of fibrous Faujasite Y supported Ni (Ni/FFY) catalyst for hydrogen production via glycerol dry reforming
title_fullStr Facile synthesis of fibrous Faujasite Y supported Ni (Ni/FFY) catalyst for hydrogen production via glycerol dry reforming
title_full_unstemmed Facile synthesis of fibrous Faujasite Y supported Ni (Ni/FFY) catalyst for hydrogen production via glycerol dry reforming
title_short Facile synthesis of fibrous Faujasite Y supported Ni (Ni/FFY) catalyst for hydrogen production via glycerol dry reforming
title_sort facile synthesis of fibrous faujasite y supported ni (ni/ffy) catalyst for hydrogen production via glycerol dry reforming
topic TP Chemical technology
url http://umpir.ump.edu.my/id/eprint/40532/
http://umpir.ump.edu.my/id/eprint/40532/
http://umpir.ump.edu.my/id/eprint/40532/
http://umpir.ump.edu.my/id/eprint/40532/1/Facile%20synthesis%20of%20fibrous%20Faujasite%20Y%20supported%20Ni.pdf
http://umpir.ump.edu.my/id/eprint/40532/2/Facile%20synthesis%20of%20fibrous%20Faujasite%20Y%20supported%20Ni_FULL.pdf