Influence of Polyethersulfone substrate properties on the performance of thin film composite forward osmosis membrane: Effect of additive concentration, polymer concentration and casting thickness

This research seeks to optimize the impact of substrate parameters such as polyvinylpyrrolidone (PVP) additive concentration (3–11 wt%), polyethersulfone (PES) concentration (11–17 wt%), and casting thickness (100–250 μm) on the overall performances of (PES) thin film composite (TFC) FO membrane. No...

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Main Authors: Nur Aisyah, Shafie, Mazrul Nizam, Abu Seman, Syed Mohd Saufi, Tuan Chik, Abdul Wahab, Mohammad
Format: Article
Language:English
English
Published: Elsevier Ltd 2023
Subjects:
Online Access:http://umpir.ump.edu.my/id/eprint/39248/
http://umpir.ump.edu.my/id/eprint/39248/1/Influence%20of%20Polyethersulfone%20substrate%20properties.pdf
http://umpir.ump.edu.my/id/eprint/39248/2/Influence%20of%20Polyethersulfone%20substrate%20properties%20on%20the%20performance%20of%20thin%20film%20composite%20forward%20osmosis%20membrane_%20Effect%20of%20additive%20concentration%2C%20polymer%20concentration%20and%20casting%20thickness.pdf
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author Nur Aisyah, Shafie
Mazrul Nizam, Abu Seman
Syed Mohd Saufi, Tuan Chik
Abdul Wahab, Mohammad
author_facet Nur Aisyah, Shafie
Mazrul Nizam, Abu Seman
Syed Mohd Saufi, Tuan Chik
Abdul Wahab, Mohammad
author_sort Nur Aisyah, Shafie
building UMP Institutional Repository
collection Online Access
description This research seeks to optimize the impact of substrate parameters such as polyvinylpyrrolidone (PVP) additive concentration (3–11 wt%), polyethersulfone (PES) concentration (11–17 wt%), and casting thickness (100–250 μm) on the overall performances of (PES) thin film composite (TFC) FO membrane. Non-solvent induced phase separation (NIPS) method was used to fabricate the substrate membrane, which was then followed by the interfacial polymerization of m-phenylene diamine (MPD) in aqueous solution and trimesoyl chloride (TMC) in hexane-organic solvent to form the active polyamide (PA) layer. Analyses of contact angle, porosity, pore size, functional group, morphology, and surface roughness were performed on membrane substrates and TFC membrane. Membrane performance parameters such as water flux (Jw), reverse salt diffusion (RSD), and specific reverse flux (SRF) were evaluated for the fabricated TFC membranes using the FO filtration system (pure water as feed solution and NaCl as draw solution). In addition, the water permeability coefficient (A), the solute permeability coefficient (B), and the structural parameter (S) were computed mathematically. Optimized membranes were chosen using the specific reverse flux (SRF) as the principal performance indicator. The optimal membranes for each parameter were then evaluated for their antifouling and rejection properties using humic acid (HA) solution. Among the optimized membranes, 15%PES/5%PVP/100 μm membrane exhibited the best performance with high rejection and antifouling properties towards HA.
first_indexed 2025-11-15T03:33:24Z
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institution Universiti Malaysia Pahang
institution_category Local University
language English
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last_indexed 2025-11-15T03:33:24Z
publishDate 2023
publisher Elsevier Ltd
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spelling ump-392482023-11-09T01:42:47Z http://umpir.ump.edu.my/id/eprint/39248/ Influence of Polyethersulfone substrate properties on the performance of thin film composite forward osmosis membrane: Effect of additive concentration, polymer concentration and casting thickness Nur Aisyah, Shafie Mazrul Nizam, Abu Seman Syed Mohd Saufi, Tuan Chik Abdul Wahab, Mohammad T Technology (General) TP Chemical technology This research seeks to optimize the impact of substrate parameters such as polyvinylpyrrolidone (PVP) additive concentration (3–11 wt%), polyethersulfone (PES) concentration (11–17 wt%), and casting thickness (100–250 μm) on the overall performances of (PES) thin film composite (TFC) FO membrane. Non-solvent induced phase separation (NIPS) method was used to fabricate the substrate membrane, which was then followed by the interfacial polymerization of m-phenylene diamine (MPD) in aqueous solution and trimesoyl chloride (TMC) in hexane-organic solvent to form the active polyamide (PA) layer. Analyses of contact angle, porosity, pore size, functional group, morphology, and surface roughness were performed on membrane substrates and TFC membrane. Membrane performance parameters such as water flux (Jw), reverse salt diffusion (RSD), and specific reverse flux (SRF) were evaluated for the fabricated TFC membranes using the FO filtration system (pure water as feed solution and NaCl as draw solution). In addition, the water permeability coefficient (A), the solute permeability coefficient (B), and the structural parameter (S) were computed mathematically. Optimized membranes were chosen using the specific reverse flux (SRF) as the principal performance indicator. The optimal membranes for each parameter were then evaluated for their antifouling and rejection properties using humic acid (HA) solution. Among the optimized membranes, 15%PES/5%PVP/100 μm membrane exhibited the best performance with high rejection and antifouling properties towards HA. Elsevier Ltd 2023-12 Article PeerReviewed pdf en http://umpir.ump.edu.my/id/eprint/39248/1/Influence%20of%20Polyethersulfone%20substrate%20properties.pdf pdf en http://umpir.ump.edu.my/id/eprint/39248/2/Influence%20of%20Polyethersulfone%20substrate%20properties%20on%20the%20performance%20of%20thin%20film%20composite%20forward%20osmosis%20membrane_%20Effect%20of%20additive%20concentration%2C%20polymer%20concentration%20and%20casting%20thickness.pdf Nur Aisyah, Shafie and Mazrul Nizam, Abu Seman and Syed Mohd Saufi, Tuan Chik and Abdul Wahab, Mohammad (2023) Influence of Polyethersulfone substrate properties on the performance of thin film composite forward osmosis membrane: Effect of additive concentration, polymer concentration and casting thickness. Chemical Engineering Research and Design, 200. pp. 186-201. ISSN 0263-8762. (Published) https://doi.org/10.1016/j.cherd.2023.10.034 10.1016/j.cherd.2023.10.034
spellingShingle T Technology (General)
TP Chemical technology
Nur Aisyah, Shafie
Mazrul Nizam, Abu Seman
Syed Mohd Saufi, Tuan Chik
Abdul Wahab, Mohammad
Influence of Polyethersulfone substrate properties on the performance of thin film composite forward osmosis membrane: Effect of additive concentration, polymer concentration and casting thickness
title Influence of Polyethersulfone substrate properties on the performance of thin film composite forward osmosis membrane: Effect of additive concentration, polymer concentration and casting thickness
title_full Influence of Polyethersulfone substrate properties on the performance of thin film composite forward osmosis membrane: Effect of additive concentration, polymer concentration and casting thickness
title_fullStr Influence of Polyethersulfone substrate properties on the performance of thin film composite forward osmosis membrane: Effect of additive concentration, polymer concentration and casting thickness
title_full_unstemmed Influence of Polyethersulfone substrate properties on the performance of thin film composite forward osmosis membrane: Effect of additive concentration, polymer concentration and casting thickness
title_short Influence of Polyethersulfone substrate properties on the performance of thin film composite forward osmosis membrane: Effect of additive concentration, polymer concentration and casting thickness
title_sort influence of polyethersulfone substrate properties on the performance of thin film composite forward osmosis membrane: effect of additive concentration, polymer concentration and casting thickness
topic T Technology (General)
TP Chemical technology
url http://umpir.ump.edu.my/id/eprint/39248/
http://umpir.ump.edu.my/id/eprint/39248/
http://umpir.ump.edu.my/id/eprint/39248/
http://umpir.ump.edu.my/id/eprint/39248/1/Influence%20of%20Polyethersulfone%20substrate%20properties.pdf
http://umpir.ump.edu.my/id/eprint/39248/2/Influence%20of%20Polyethersulfone%20substrate%20properties%20on%20the%20performance%20of%20thin%20film%20composite%20forward%20osmosis%20membrane_%20Effect%20of%20additive%20concentration%2C%20polymer%20concentration%20and%20casting%20thickness.pdf